skip to main content


Title: Enhanced optical mode coherence in exchange coupled soft magnetic multilayers
We report on an all-optical investigation of coupled spin excitation modes in a series of magnetic trilayer structures. Using time-resolved magneto-optic Kerr effect (tr-MOKE) magnetometry, we observe multi-mode coherent spin excitations in [Formula: see text]/Ru/[Formula: see text] multilayers even though the tr-MOKE optical detection is sensitive only to the [Formula: see text] magnetization dynamics. Frequency shifts of the different modes indicate that the coupling between the [Formula: see text] and [Formula: see text] layers varies from anti-ferromagnetic to ferromagnetic to uncoupled as the Ru spacer layer thickness is increased from 8 Å to 200 Å. The lifetime of the high frequency coherent oscillations in the [Formula: see text] layer increases by over 200%–300% even in the case of uncoupled [Formula: see text] and [Formula: see text] layers with a 200 Å thick Ru spacer. The results suggest an additional method to decrease the damping of high-moment alloys in layered magnetic nanostructures.  more » « less
Award ID(s):
1952957
PAR ID:
10409815
Author(s) / Creator(s):
; ; ; ;
Date Published:
Journal Name:
Journal of Applied Physics
Volume:
131
Issue:
21
ISSN:
0021-8979
Page Range / eLocation ID:
213902
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Abstract

    In this work high-frequency magnetization dynamics and statics of artificial spin-ice lattices with different geometric nanostructure array configurations are studied where the individual nanostructures are composed of ferromagnetic/non-magnetic/ferromagnetic trilayers with different non-magnetic thicknesses. These thickness variations enable additional control over the magnetic interactions within the spin-ice lattice that directly impacts the resulting magnetization dynamics and the associated magnonic modes. Specifically the geometric arrangements studied are square, kagome and trigonal spin ice configurations, where the individual lithographically patterned nanomagnets (NMs) are trilayers, made up of two magnetic layers ofNi81Fe19of 30 nm and 70 nm thickness respectively, separated by a non-magnetic copper layer of either 2 nm or 40 nm. We show that coupling via the magnetostatic interactions between the ferromagnetic layers of the NMs within square, kagome and trigonal spin-ice lattices offers fine-control over magnetization states and magnetic resonant modes. In particular, the kagome and trigonal lattices allow tuning of an additional mode and the spacing between multiple resonance modes, increasing functionality beyond square lattices. These results demonstrate the ability to move beyond quasi-2D single magnetic layer nanomagnetics via control of the vertical interlayer interactions in spin ice arrays. This additional control enables multi-mode magnonic programmability of the resonance spectra, which has potential for magnetic metamaterials for microwave or information processing applications.

     
    more » « less
  2. Efficient manipulation of antiferromagnetically coupled materials that are integration-friendly and have strong perpendicular magnetic anisotropy (PMA) is of great interest for low-power, fast, dense magnetic storage and computing. Here, we report a distinct, giant bulk damping-like spin–orbit torque in strong-PMA ferrimagnetic Fe 100− x Tb x single layers that are integration-friendly (composition-uniform, amorphous, and sputter-deposited). For sufficiently thick layers, this bulk torque is constant in the efficiency per unit layer thickness, [Formula: see text]/ t, with a record-high value of 0.036 ± 0.008 nm −1 , and the damping-like torque efficiency [Formula: see text] achieves very large values for thick layers, up to 300% for 90 nm layers. This giant bulk torque by itself switches tens of nm thick Fe 100− x Tb x layers that have very strong PMA and high coercivity at current densities as low as a few MA/cm 2 . Surprisingly, for a given layer thickness, [Formula: see text] shows strong composition dependence and becomes negative for composition where the total angular momentum is oriented parallel to the magnetization rather than antiparallel. Our findings of giant bulk spin torque efficiency and intriguing torque-compensation correlation will stimulate study of such unique spin–orbit phenomena in a variety of ferrimagnetic hosts. This work paves a promising avenue for developing ultralow-power, fast, dense ferrimagnetic storage and computing devices. 
    more » « less
  3. Magneto-intersubband resistance oscillations (MISOs) of highly mobile 2D electrons in symmetric GaAs quantum wells with two populated subbands are studied in magnetic fields [Formula: see text] tilted from the normal to the 2D electron layer at different temperatures [Formula: see text]. The in-plane component ([Formula: see text]) of the field [Formula: see text] induces magnetic entanglement between subbands, leading to beating in oscillating density of states (DOS) and to MISO suppression. Model of the MISO suppression is proposed. Within the model, a comparison of MISO amplitude in the entangled and disentangled ([Formula: see text]) 2D systems yields both difference frequency of DOS oscillations, [Formula: see text], and strength of the electron–electron interaction, described by parameter [Formula: see text], in the 2D system. These properties are analyzed using two methods, yielding consistent but not identical results for both [Formula: see text] and [Formula: see text]. The analysis reveals an additional angular dependent factor of MISO suppression. The factor is related to spin splitting of quantum levels in magnetic fields. 
    more » « less
  4. The strong spin–orbit coupling (SOC) in lead halide perovskites, when inversion symmetry is lifted, has provided opportunities for investigating the Rashba effect in these systems. Moreover, the strong orbital moment, which, in turn, impacts the spin-pair in singlet and triplet electronic states, plays a significant role in enhancing the optoelectronic properties in the presence of external magnetic fields in lead halide perovskites. Here, we investigate the effect of weak magnetic fields (<1 T) on the photoluminescence (PL) properties of [Formula: see text] nanocrystals with and without Ruddlesden–Popper (RP) faults and single crystals of [Formula: see text]. Along with an enhancement in the PL intensity as a function of an external magnetic field, which is observed in both lead bromide perovskites, the PL emission red-shifts in [Formula: see text] nanocrystals. Density-functional theory calculations of the electronic band-edge in [Formula: see text] show almost no change in the energy gap as a function of the external magnetic field. The experimental results, thus, suggest the role of mixing of the triplet and singlet excitonic states under weak magnetic fields. This is further deduced from an enhancement in PL lifetimes as a function of the field in [Formula: see text]. In [Formula: see text], an increase in PL intensity is observed under weak magnetic fields; however, no changes in the peak energy or PL lifetimes are observed. The internal magnetic fields due to SOC are characterized for all three samples and found to be the highest for [Formula: see text] nanocrystals with RP faults.

     
    more » « less
  5. Abstract

    Thin ferromagnetic films possessing perpendicular magnetic anisotropy derived from the crystal lattice can deliver the requisite magnetocrystalline anisotropy density for thermally stable magnetic memory and logic devices at the single-digit-nm lateral size. Here, we demonstrate that an epitaxial synthetic antiferromagnet can be formed from L10FePd, a candidate material with large magnetocrystalline anisotropy energy, through insertion of an ultrathin Ir spacer. Tuning of the Ir spacer thickness leads to synthetic antiferromagnetically coupled FePd layers, with an interlayer exchange field upwards of 0.6 T combined with a perpendicular magnetic anisotropy energy of 0.95 MJ/m3and a low Gilbert damping of 0.01. Temperature-dependent ferromagnetic resonance measurements show that the Gilbert damping is mostly insensitive to temperature over a range of 20 K up to 300 K. In FePd|Ir|FePd trilayers with lower interlayer exchange coupling, optic and acoustic dynamic ferromagnetic resonance modes are explored as a function of temperature. The ability to engineer low damping and large interlayer exchange coupling in FePd|Ir|FePd synthetic antiferromagnets with high perpendicular magnetic anisotropy could prove useful for high performance spintronic devices.

     
    more » « less