Title: Nernst coefficient measurements in two-dimensional materials
Abstract The discovery of two-dimensional (2D) ferromagnets and antiferromagnets with topologically nontrivial electronic band structures makes the study of the Nernst effect in 2D materials of great importance and interest. To measure the Nernst coefficient of 2D materials, the detection of the temperature gradient is crucial. Although the micro-fabricated metal wires provide a simple but accurate way for temperature detection, a linear-response assumption that the temperature gradient is a constant is still necessary and has been widely used to evaluate the temperature gradient. However, with the existence of substrates, this assumption cannot be precise. In this study, we clearly show that the temperature gradient strongly depends on the distance from the heater by both thermoelectric transport and thermoreflectance measurements. Fortunately, both measurements show that the temperature gradient can be well described by a linear function of the distance from the heater. This linearity is further confirmed by comparing the measured Nernst coefficient to the value calculated from the generalized Mott’s formula. Our results demonstrate a precise way to measure the Nernst coefficient of 2D materials and would be helpful for future studies. more »« less
Van der Waals heterostructures offer great versatility to tailor unique interactions at the atomically flat interfaces between dissimilar layered materials and induce novel physical phenomena. By bringing monolayer 1 T’ WTe2, a two-dimensional quantum spin Hall insulator, and few-layer Cr2Ge2Te6, an insulating ferromagnet, into close proximity in an heterostructure, we introduce a ferromagnetic order in the former via the interfacial exchange interaction. The ferromagnetism in WTe2manifests in the anomalous Nernst effect, anomalous Hall effect as well as anisotropic magnetoresistance effect. Using local electrodes, we identify separate transport contributions from the metallic edge and insulating bulk. When driven by an AC current, the second harmonic voltage responses closely resemble the anomalous Nernst responses to AC temperature gradient generated by nonlocal heater, which appear as nonreciprocal signals with respect to the induced magnetization orientation. Our results from different electrodes reveal spin-polarized edge states in the magnetized quantum spin Hall insulator.
Hankiewicz, Janusz H.; Celinski, Zbigniew; Camley, Robert E.(
, Medical Physics)
AbstractPurpose
One standard method, proton resonance frequency shift, for measuring temperature using magnetic resonance imaging (MRI), in MRI‐guided surgeries, fails completely below the freezing point of water. Because of this, we have developed a new methodology for monitoring temperature with MRI below freezing. The purpose of this paper is to show that a strong temperature dependence of the nuclear relaxation timeT1in soft silicone polymers can lead to temperature‐dependent changes of MRI intensity acquired withT1weighting. We propose the use of silicone filaments inserted in tissue for measuring temperature during MRI‐guided cryoablations.
Methods
The temperature dependence ofT1in bio‐compatible soft silicone polymers was measured using nuclear magnetic resonance spectroscopy and MRI. Phantoms, made of bulk silicone materials and put in an MRI‐compatible thermal container with dry ice, allowed temperature measurements ranging from –60°C to + 20°C.T1‐weighted gradient echo images of the phantoms were acquired at spatially uniform temperatures and with a gradient in temperature to determine the efficacy of using these materials as temperature indicators in MRI. Ex vivo experiments on silicone rods, 4 mm in diameter, inserted in animal tissue were conducted to assess the practical feasibility of the method.
Results
Measurements of nuclear relaxation times of protons in soft silicone polymers show a monotonic, nearly linear, change with temperature (R2 > 0.98) and have a significant correlation with temperature (Pearson'sr > 0.99,p < 0.01). Similarly, the intensity of the MR images in these materials, taken with a gradient echo sequence, are also temperature dependent. There is again a monotonic change in MRI intensity that correlates well with the measured temperature (Pearson'sr < ‐0.98 andp < 0.01). The MRI experiments show that a temperature change of 3°C can be resolved in a distance of about 2.5 mm. Based on MRI images and external sensor calibrations for a sample with a gradient in temperature, temperature maps with 3°C isotherms are created for a bulk phantom. Experiments demonstrate that these changes in MRI intensity with temperature can also be seen in 4 mm silicone rods embedded in ex vivo animal tissue.
Conclusions
We have developed a new method for measuring temperature in MRI that potentially could be used during MRI‐guided cryoablation operations, reducing both procedure time and cost, and making these surgeries safer.
As spin caloritronic measurements become increasingly common techniques for characterizing material properties, it is important to quantify potentially confounding effects. We report measurements of the Nernst–Ettingshausen response from room temperature to 5 K in thin film wires of Pt and W, metals commonly used as inverse spin Hall detectors in spin Seebeck characterization. Johnson–Nyquist noise thermometry is used to assess the temperature change in the metals with heater power at low temperatures, and the thermal path is analyzed via finite-element modeling. The Nernst–Ettingshausen response of W is found to be approximately temperature-independent, while the response of Pt increases at low temperatures. These results are discussed in the context of theoretical expectations and the possible role of magnetic impurities in Pt.
Context. As primary anchors of the distance scale, Cepheid stars play a crucial role in our understanding of the distance scale of the Universe because of their period-luminosity relation. Determining precise and consistent parameters (radius, temperature, color excess, and projection factor) of Cepheid pulsating stars is therefore very important. Aims. With the high-precision parallaxes delivered by the early third Gaia data release (EDR3), we aim to derive various parameters of Cepheid stars in order to calibrate the period-luminosity and period-radius relations and to investigate the relation of period to p -factor. Methods. We applied an implementation of the parallax-of-pulsation method through the algorithm called spectro-photo-interferometry of pulsating stars (SPIPS), which combines all types of available data for a variable star (multiband and multicolor photometry, radial velocity, effective temperature, and interferometry measurements) in a global modeling of its pulsation. Results. We present the SPIPS modeling of a sample of 63 Galactic Cepheids. Adopting Gaia EDR3 parallaxes as an input associated with the best available dataset, we derive consistent values of parameters for these stars such as the radius, multiband apparent magnitudes, effective temperatures, color excesses, period changes, Fourier parameters, and the projection factor. Conclusions. Using the best set of data and the most precise distances for Milky Way Cepheids, we derive new calibrations of the period-luminosity and period-radius relations: M K S = −5.529 ±0.015 − 3.141 ±0.050 (log P − 0.9) and log R = 1.763 ±0.003 + 0.653 ±0.012 (log P − 0.9). After investigating the dependences of the projection factor on the parameters of the stars, we find a high dispersion of its values and no evidence of its correlation with the period or with any other parameters such as radial velocity, temperature, or metallicity. Statistically, the p -factor has an average value of p = 1.26 ± 0.07, but with an unsatisfactory agreement ( σ = 0.15). In absence of any clear correlation between the p -factor and other quantities, the best agreement is obtained under the assumption that the p -factor can take any value in a band with a width of 0.15. This result highlights the need for a further examination of the physics behind the p -factor.
Cannon, Taylor M.; Bouma, Brett E.; Uribe-Patarroyo, Néstor(
, Biomedical Optics Express)
Structural optical coherence tomography (OCT) images of tissue stand to benefit from greater functionalization and quantitative interpretation. The OCT attenuation coefficientµ, an analogue of the imaged sample’s scattering coefficient, offers potential functional contrast based on the relationship ofµto sub-resolution physical properties of the sample. Attenuation coefficients are computed either by fitting a representativeµover several depth-wise pixels of a sample’s intensity decay, or by using previously-developed depth-resolved attenuation algorithms by Girardet al.[Invest. Ophthalmol. Vis. Sci.52,7738(2011).10.1167/iovs.10-6925] and Vermeeret al.[Biomed. Opt. Express5,322(2014).10.1364/BOE.5.000322]. However, the former method sacrifices axial information in the tomogram, while the latter relies on the stringent assumption that the sample’s backscattering fraction, another optical property, does not vary along depth. This assumption may be violated by layered tissues commonly observed in clinical imaging applications. Our approach preserves the full depth resolution of the attenuation map but removes its dependence on backscattering fraction by performing signal analysis inside individual discrete layers over which the scattering properties (e.g., attenuation and backscattering fraction) vary minimally. Although this approach necessitates the detection of these layers, it removes the constant-backscattering-fraction assumption that has constrained quantitative attenuation coefficient analysis in the past, and additionally yields a layer-resolved backscattering fraction, providing complementary scattering information to the attenuation coefficient. We validate our approach using automated layer detection in layered phantoms, for which the measured optical properties were in good agreement with theoretical values calculated with Mie theory, and show preliminary results in tissue alongside corresponding histological analysis. Together, accurate backscattering fraction and attenuation coefficient measurements enable the estimation of both particle density and size, which is not possible from attenuation measurements alone. We hope that this improvement to depth-resolved attenuation coefficient measurement, augmented by a layer-resolved backscattering fraction, will increase the diagnostic power of quantitative OCT imaging.
@article{osti_10415148,
place = {Country unknown/Code not available},
title = {Nernst coefficient measurements in two-dimensional materials},
url = {https://par.nsf.gov/biblio/10415148},
DOI = {10.1088/1361-6463/ac923f},
abstractNote = {Abstract The discovery of two-dimensional (2D) ferromagnets and antiferromagnets with topologically nontrivial electronic band structures makes the study of the Nernst effect in 2D materials of great importance and interest. To measure the Nernst coefficient of 2D materials, the detection of the temperature gradient is crucial. Although the micro-fabricated metal wires provide a simple but accurate way for temperature detection, a linear-response assumption that the temperature gradient is a constant is still necessary and has been widely used to evaluate the temperature gradient. However, with the existence of substrates, this assumption cannot be precise. In this study, we clearly show that the temperature gradient strongly depends on the distance from the heater by both thermoelectric transport and thermoreflectance measurements. Fortunately, both measurements show that the temperature gradient can be well described by a linear function of the distance from the heater. This linearity is further confirmed by comparing the measured Nernst coefficient to the value calculated from the generalized Mott’s formula. Our results demonstrate a precise way to measure the Nernst coefficient of 2D materials and would be helpful for future studies.},
journal = {Journal of Physics D: Applied Physics},
volume = {55},
number = {45},
author = {Feng, Qi and Zhu, Tianhui and Jian, Yu and Yuan, Wei and Peng, Huimin and Zhong, Jinrui and Duan, Junxi and Zebarjadi, Mona},
}
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