High-intensity pulse-beams are ubiquitous in scientific investigations and industrial applications ranging from the generation of secondary radiation sources (e.g., high harmonic generation, electrons) to material processing (e.g., micromachining, laser-eye surgery). Crucially, pulse-beams can only be controlled to the degree to which they are characterized, necessitating sophisticated measurement techniques. We present a reference-free, full-field, single-shot spatiospectral measurement technique called broadband single-shot ptychography (BBSSP). BBSSP provides the complex wavefront for each spectral and polarization component in an ultrafast pulse-beam and should be applicable across the electromagnetic spectrum. BBSSP will dramatically improve the application and mitigation of spatiospectral pulse-beam structure. 
                        more » 
                        « less   
                    
                            
                            Single-pulse, reference-free, spatiotemporal characterization of ultrafast laser pulse beams via broadband ptychography
                        
                    
    
            Ultrafast laser pulse beams are four-dimensional, space–time phenomena that can exhibit complicated, coupled spatial and temporal profiles. Tailoring the spatiotemporal profile of an ultrafast pulse beam is necessary to optimize the focused intensity and to engineer exotic spatiotemporally shaped pulse beams. Here we demonstrate a single-pulse, reference-free spatiotemporal characterization technique based on two colocated synchronized measurements: (1) broadband single-shot ptychography and (2) single-shot frequency resolved optical gating. We apply the technique to measure the nonlinear propagation of an ultrafast pulse beam through a fused silica window. Our spatiotemporal characterization method represents a major contribution to the growing field of spatiotemporally engineered ultrafast laser pulse beams. 
        more » 
        « less   
        
    
                            - Award ID(s):
- 2206807
- PAR ID:
- 10425211
- Publisher / Repository:
- Optical Society of America
- Date Published:
- Journal Name:
- Optics Letters
- Volume:
- 48
- Issue:
- 13
- ISSN:
- 0146-9592; OPLEDP
- Format(s):
- Medium: X Size: Article No. 3455
- Size(s):
- Article No. 3455
- Sponsoring Org:
- National Science Foundation
More Like this
- 
            
- 
            Ultrafast pulse-beam characterization is critical for diverse scientific and industrial applications from micromachining to generating the highest intensity laser pulses. The four-dimensional structure of a pulse-beam, , can be fully characterized by coupling spatiospectral metrology with spectral phase measurement. When temporal pulse dynamics are not of primary interest, spatiospectral characterization of a pulse-beam provides crucial information even without spectral phase. Here we demonstrate spatiospectral characterization of pulse-beams via multiplexed broadband ptychography. The complex spatial profiles of multiple spectral components, , from modelocked Ti:sapphire and from extreme ultra-violet pulse-beams are reconstructed with minimum intervening optics and no refocusing. Critically, our technique does not require spectral filters, interferometers, or reference pulses.more » « less
- 
            We present a single-shot detection method of terahertz correlated second harmonic generation in plasma-based sources by directly mixing an optical probe into femtosecond laser-induced plasma filaments in air. The single-shot second harmonic trace is obtained by measuring a second harmonic generation on a conventional CCD with a spatiotemporally distorted probe beam. The system shows a spectrometer resolution of 22 fs/pixel on the CCD and a true resolution on the order of the probe pulse duration. With considerable THz peak electric field strength, this formalism can open the door to single-shot THz detection without bandwidth limitations.more » « less
- 
            Ultrafast laser systems, those with a pulse duration on the order of picoseconds or less, have enabled advancements in a wide variety of fields. Of particular interest to this work, these laser systems are the key component to many High Energy Density (HED) physics experiments. Despite this, previous studies on the shape of the laser pulse within the HED community have focused primarily on pulse duration due to the relationship between pulse duration and peak intensity, while leaving the femtosecond scale structure of the pulse shape largely unstudied. To broaden the variety of potential pulses available for study, a method of reliably adjusting the pulse shape at the femtosecond scale using sub-nanometer resolution Direct Phase Control has been developed. This paper examines the capabilities of this new method compared to more commonplace dispersion-based pulse shaping methods. It also will detail the capabilities of the core algorithm driving this technique when used in conjunction with the WIZZLER and DAZZLER instruments that are common in high intensity laser labs. Performance of the method and instrumentation is examined using data taken with a single shot FROG system. Finally, some discussion is given to possible applications on how the Direct Phase Control pulse shaping technique will be implemented in the future.more » « less
- 
            Field-resolved measurements of few-cycle laser waveforms allow access to ultrafast electron dynamics in light–matter interactions and are key to future lightwave electronics. Recently, sub-cycle gating based on nonlinear excitation in active pixel sensors has allowed the first single-shot measurements of mid-infrared optical fields. Extending the techniques to shorter wavelengths, however, is not feasible using silicon-based detectors with bandgaps in the near-infrared. Here, we demonstrate an all-optical sampling technique for near-infrared laser fields, wherein an intense fundamental field generates a sub-cycle gate through nonlinear excitation of a wide-bandgap crystal, in this case, ZnO, which can sample the electric field of a weak perturbing pulse. By using a crossed-beam geometry, the temporal evolution of the perturbing field is mapped onto a transverse spatial axis of the nonlinear medium, and the waveform is captured in a single measurement of the spatially resolved fluorescence emission from the crystal. The technique is demonstrated through field-resolved measurements of the field reshaping during nonlinear propagation in the ZnO detection crystal.more » « less
 An official website of the United States government
An official website of the United States government 
				
			 
					 
					
