The application of high-power, few-cycle, long-wave infrared (LWIR, 8–20 µm) pulses in strong-field physics is largely unexplored due to the lack of suitable sources. However, the generation of intense pulses with >6 µm wavelength range is becoming increasingly feasible with the recent advances in high-power ultrashort lasers in the middle-infrared range that can serve as a pump for optical parametric amplifiers (OPA). Here we experimentally demonstrate the feasibility of this approach by building an OPA pumped at 2.4 µm that generates 93 µJ pulses at 9.5 µm, 1 kHz repetition rate with sub-two-cycle pulse duration, 1.6 GW peak power, and excellent beam quality. The results open a wide range of applications in attosecond physics (especially for studies of condensed phase samples), remote sensing, and biophotonics.
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Cryogenically cooled Fe:ZnSe-based chirped pulse amplifier at 4.07 µm
A femtosecond chirped pulse amplifier based on cryogenically cooled Fe:ZnSe was demonstrated at 333 Hz—33 times higher than previous results achieved at near-room-temperature. The long upper-state lifetime allows free-running, diode-pumped Er:YAG lasers to be used as pump lasers. 250-fs, 4.59-mJ pulses are produced with a center wavelength of 4.07 µm, which avoids strong atmospheric CO 2 absorption that cuts on around 4.2 µm. It is therefore possible to operate the laser in ambient air with good beam quality. By focusing the 18-GW beam in air, harmonics up to the ninth order were observed indicating its potential for use in strong-field experimentation.
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- Award ID(s):
- 2207674
- PAR ID:
- 10430694
- Date Published:
- Journal Name:
- Optics Express
- Volume:
- 31
- Issue:
- 8
- ISSN:
- 1094-4087
- Page Range / eLocation ID:
- 13447
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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