skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.

Attention:

The NSF Public Access Repository (PAR) system and access will be unavailable from 10:00 PM ET on Thursday, February 12 until 1:00 AM ET on Friday, February 13 due to maintenance. We apologize for the inconvenience.

Explore Research Products in the PAR
It may take a few hours for recently added research products to appear in PAR search results.


Title: Néel-type skyrmion in WTe2/Fe3GeTe2 van der Waals heterostructure
Abstract The promise of high-density and low-energy-consumption devices motivates the search for layered structures that stabilize chiral spin textures such as topologically protected skyrmions. At the same time, recently discovered long-range intrinsic magnetic orders in the two-dimensional van der Waals materials provide a new platform for the discovery of novel physics and effects. Here we demonstrate the Dzyaloshinskii–Moriya interaction and Néel-type skyrmions are induced at the WTe 2 /Fe 3 GeTe 2 interface. Transport measurements show the topological Hall effect in this heterostructure for temperatures below 100 K. Furthermore, Lorentz transmission electron microscopy is used to directly image Néel-type skyrmion lattice and the stripe-like magnetic domain structures as well. The interfacial coupling induced Dzyaloshinskii–Moriya interaction is estimated to have a large energy of 1.0 mJ m −2 . This work paves a path towards the skyrmionic devices based on van der Waals layered heterostructures.  more » « less
Award ID(s):
1935362
PAR ID:
10433470
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ;
Date Published:
Journal Name:
Nature Communications
Volume:
11
Issue:
1
ISSN:
2041-1723
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. ; ; ; ; ; ; ; ; ; ; et al (, Nature Communications)
    null (Ed.)
    Abstract Room-temperature skyrmions in magnetic multilayers are considered to be promising candidates for the next-generation spintronic devices. Several approaches have been developed to control skyrmions, but they either cause significant heat dissipation or require ultrahigh electric fields near the breakdown threshold. Here, we demonstrate electric-field control of skyrmions through strain-mediated magnetoelectric coupling in ferromagnetic/ferroelectric multiferroic heterostructures. We show the process of non-volatile creation of multiple skyrmions, reversible deformation and annihilation of a single skyrmion by performing magnetic force microscopy with in situ electric fields. Strain-induced changes in perpendicular magnetic anisotropy and interfacial Dzyaloshinskii–Moriya interaction strength are characterized experimentally. These experimental results, together with micromagnetic simulations, demonstrate that strain-mediated magnetoelectric coupling (via strain-induced changes in both the perpendicular magnetic anisotropy and interfacial Dzyaloshinskii–Moriya interaction is responsible for the observed electric-field control of skyrmions. Our work provides a platform to investigate electric-field control of skyrmions in multiferroic heterostructures and paves the way towards more energy-efficient skyrmion-based spintronics. 
    more » « less
  2. ; (, Journal of Magnetism and Magnetic Materials)
    The stability and resonance spectra associated with a domain wall skyrmion embedded within a Néel skyrmion, forming a 1-kink skyrmion, has been studied using micromagnetic simulations. We show that the 1-kink skyrmion is stable over a wide range of fields at moderate strengths of the Dzyaloshinskii-Moriya interaction. By exciting these structures with a broadband magnetic field excitation, we find complex resonance behavior deviating from that of a pure Néel skyrmion. For out-of-plane excitations, the 1-kink skyrmion demonstrates an additional mode relative to that of the Néel skyrmion at reduced amplitude. These consist of low frequency and high frequency modes associated with both a breathing mode and an oscillation of the embedded domain wall skyrmion. Following an in-plane excitation, both Néel and 1-kink skyrmions exhibit a counterclockwise rotational mode with similar frequencies, as well as a higher frequency mode associated with the interaction of the structure with the ferromagnetic background state. These results may help pave the way for exploration of more complex spin structures for magnetic-based microwave devices. 
    more » « less
  3. ; ; ; ; ; ; ; ; ; ; et al (, Advanced Materials)
    Abstract Magnetic skyrmions are topologically nontrivial chiral spin textures that have potential applications in next‐generation energy‐efficient and high‐density spintronic devices. In general, the chiral spins of skyrmions are stabilized by the noncollinear Dzyaloshinskii–Moriya interaction (DMI), originating from the inversion symmetry breaking combined with the strong spin–orbit coupling (SOC). Here, the strong SOC from topological insulators (TIs) is utilized to provide a large interfacial DMI in TI/ferrimagnet heterostructures at room temperature, resulting in small‐size (radius ≈ 100 nm) skyrmions in the adjacent ferrimagnet. Antiferromagnetically coupled skyrmion sublattices are observed in the ferrimagnet by element‐resolved scanning transmission X‐ray microscopy, showing the potential of a vanishing skyrmion Hall effect and ultrafast skyrmion dynamics. The line‐scan spin profile of the single skyrmion shows a Néel‐type domain wall structure and a 120 nm size of the 180° domain wall. This work demonstrates the sizable DMI and small skyrmions in TI‐based heterostructures with great promise for low‐energy spintronic devices. 
    more » « less
  4. ; ; ; ; ; ; ; ; ; ; et al (, Small)
    Abstract Topological spin textures (e.g., skyrmions) can be stabilized by interfacial Dzyaloshinskii‐Moriya interaction (DMI) in the magnetic multilayer, which has been intensively studied. Recently, Bloch‐type magnetic skyrmions stabilized by composition gradient‐induced DMI (g‐DMI) have been observed in 10‐nm thick CoPt single layer. However, magnetic anisotropy in gradient‐composition engineered CoPt (g‐CoPt) films is highly sensitive to both the relative Co/Pt composition and the film thickness, leading to a complex interplay with g‐DMI. The stability of skyrmions under the combined influence of magnetic anisotropy and g‐DMI is crucial yet remains poorly understood. Here, we condcut a systematic study on the characteristics of magnetic skyrmions as a function of gradient polarity and effective gradient (defined as gradient/thickness) in g‐CoPt single layers (thickness of 10–30 nm) using magnetic force microscopy (MFM), bulk magnetometry, and topological Hall effect measurements. Brillouin light scattering spectroscopy confirms that both the sign and magnitude of g‐DMI depend on the polarity and amplitude of the composition gradient in g‐CoPt films. MFM reveals that skyrmion size and density vary with g‐CoPt film thickness, gradient polarity, and applied magnetic field. An increased skyrmion density is observed in samples exhibiting higher magnetic anisotropy, in agreement with micromagnetic simulations and energy barrier calculations. 
    more » « less
  5. ; ; ; ; ; ; ; ; ; ; et al (, Advanced Physics Research)
    Abstract Magnetic van der Waals (vdW) materials are a promising platform for producing atomically thin spintronic and optoelectronic devices. The A‐type antiferromagnet CrSBr has emerged as a particularly exciting material due to its high magnetic ordering temperature, semiconducting electrical properties, and enhanced chemical stability compared to other vdW magnets. Exploring mechanisms to tune its magnetic properties will facilitate the development of nanoscale devices based on vdW materials with designer magnetic properties. Here it is investigated how the magnetic properties of CrSBr change under pressure and ligand substitution. Pressure compresses the unit cell, increasing the interlayer exchange energy while lowering the Néel temperature. Ligand substitution, realized synthetically through Cl alloying, anisotropically compresses the unit cell and suppresses the Cr‐halogen covalency, reducing the magnetocrystalline anisotropy energy and decreasing the Néel temperature. A detailed structural analysis combined with first‐principles calculations reveals that alterations in the magnetic properties are intricately related to changes in direct Cr–Cr exchange interactions and the Cr–anion superexchange pathways. Further, it is demonstrated that Cl alloying enables chemical tuning of the interlayer coupling from antiferromagnetic to ferromagnetic, which is unique among known two‐dimensional magnets. 
    more » « less
  • Citation Formats
  • MLA
  • APA
  • Chicago
  • BibTeX
  • Text Encoded Conversion
  • XML
  • Save / Share this Record
  • Send to Email