Abstract The anomalous Hall effect (AHE), typically observed in ferromagnetic (FM) metals with broken time-reversal symmetry, depends on electronic and magnetic properties. In Co3Sn2-xInxS2, a giant AHE has been attributed to Berry curvature associated with the FM Weyl semimetal phase, yet recent studies report complicated magnetism. We use neutron scattering to determine the spin dynamics and structures as a function ofxand provide a microscopic understanding of the AHE and magnetism interplay. Spin gap and stiffness indicate a contribution from Weyl fermions consistent with the AHE. The magnetic structure evolves fromc-axis ferromagnetism at$$x = 0$$ to a canted antiferromagnetic (AFM) structure with reducedc-axis moment and in-plane AFM order at$$x = 0.12$$ and further reducedc-axis FM moment at$$x = 0.3$$ . Since noncollinear spins can induce non-zero Berry curvature in real space acting as a fictitious magnetic field, our results revealed another AHE contribution, establishing the impact of magnetism on transport.
more »
« less
Anomalous Landau quantization in intrinsic magnetic topological insulators
Abstract The intrinsic magnetic topological insulator, Mn(Bi1−xSbx)2Te4, has been identified as a Weyl semimetal with a single pair of Weyl nodes in its spin-aligned strong-field configuration. A direct consequence of the Weyl state is the layer dependent Chern number,$$C$$ . Previous reports in MnBi2Te4thin films have shown higher$$C$$ states either by increasing the film thickness or controlling the chemical potential. A clear picture of the higher Chern states is still lacking as data interpretation is further complicated by the emergence of surface-band Landau levels under magnetic fields. Here, we report a tunable layer-dependent$$C$$ = 1 state with Sb substitution by performing a detailed analysis of the quantization states in Mn(Bi1−xSbx)2Te4dual-gated devices—consistent with calculations of the bulk Weyl point separation in the doped thin films. The observed Hall quantization plateaus for our thicker Mn(Bi1−xSbx)2Te4films under strong magnetic fields can be interpreted by a theory of surface and bulk spin-polarised Landau level spectra in thin film magnetic topological insulators.
more »
« less
- PAR ID:
- 10439932
- Publisher / Repository:
- Nature Publishing Group
- Date Published:
- Journal Name:
- Nature Communications
- Volume:
- 14
- Issue:
- 1
- ISSN:
- 2041-1723
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Abstract Relativistic Weyl fermion quasiparticles in Weyl semimetal bring the electron’s chirality degree of freedom into the electrical transport and give rise to exotic phenomena. A topological phase transition from a topological trivial phase to a topological non-trivial phase offers a route to control electronic devices through its topological properties. Here, we report the Weyl semimetal phase in hydrothermally grown two-dimensional Tellurium (2D Te) induced by high hydrostatic pressure (up to 2.47 GPa). The unique chiral crystal structure gives rise to chiral fermions with different topological chiral charges ($${{C}}=-{{1}},+{{1}},{{and}}-{{2}}$$ ). The highly tunable chemical potential in 2D Te provides comprehensive information for understanding the pressure-dependent electron band structure. The pressure-induced insulator-to-metal transition, two-carrier transport, and the non-trivial π Berry phase shift in quantum oscillations are observed in the 2D Te Weyl semimetal phase. Our work demonstrates the pressure-induced bandgap closing in the inversion asymmetric narrow bandgap semiconductor 2D Te.more » « less
-
Abstract The presence of topological flat minibands in moiré materials provides an opportunity to explore the interplay between topology and correlation. In this work, we study moiré minibands in topological insulator films with two hybridized surface states under a moiré superlattice potential created by two-dimensional insulating materials. We show the lowest conduction (highest valence) Kramers’ pair of minibands can be$${{\mathbb{Z}}}_{2}$$ non-trivial when the minima (maxima) of moiré potential approximately form a hexagonal lattice with six-fold rotation symmetry. Coulomb interaction can drive the non-trivial Kramers’ minibands into the quantum anomalous Hall state when they are half-filled, which is further stabilized by applying external gate voltages to break inversion. We propose the monolayer Sb2on top of Sb2Te3films as a candidate based on first principles calculations. Our work demonstrates the topological insulator based moiré heterostructure as a potential platform for studying interacting topological phases.more » « less
-
Abstract We study the effect of strain on the magnetic properties and magnetization configurations in nanogranular FexGe films ( ) with and without B20 FeGe nanocrystals surrounded by an amorphous structure. Relaxed films on amorphous silicon nitride membranes reveal a disordered skyrmion phase while films near and on top of a rigid substrate favor ferromagnetism and an anisotropic hybridization of Fedlevels and spin-polarized Gespband states. The weakly coupled topological states emerge at room temperature and become more abundant at cryogenic temperatures without showing indications of pinning at defects or confinement to individual grains. These results demonstrate the possibility to control magnetic exchange and topological magnetism by strain and inform magnetoelasticity-mediated voltage control of topological phases in amorphous quantum materials.more » « less
-
Abstract Initially, vanadium dioxide seems to be an ideal first-order phase transition case study due to its deceptively simple structure and composition, but upon closer inspection there are nuances to the driving mechanism of the metal-insulator transition (MIT) that are still unexplained. In this study, a local structure analysis across a bulk powder tungsten-substitution series is utilized to tease out the nuances of this first-order phase transition. A comparison of the average structure to the local structure using synchrotron x-ray diffraction and total scattering pair-distribution function methods, respectively, is discussed as well as comparison to bright field transmission electron microscopy imaging through a similar temperature-series as the local structure characterization. Extended x-ray absorption fine structure fitting of thin film data across the substitution-series is also presented and compared to bulk. Machine learning technique, non-negative matrix factorization, is applied to analyze the total scattering data. The bulk MIT is probed through magnetic susceptibility as well as differential scanning calorimetry. The findings indicate the local transition temperature ($$T_c$$ ) is less than the average$$T_c$$ supporting the Peierls-Mott MIT mechanism, and demonstrate that in bulk powder and thin-films, increasing tungsten-substitution instigates local V-oxidation through the phase pathway VO$$_2\, \rightarrow$$ V$$_6$$ O$$_{13} \, \rightarrow$$ V$$_2$$ O$$_5$$ .more » « less