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Title: Advancing Reverse Electrowetting‐on‐Dielectric from Planar to Rough Surface Electrodes for High Power Density Energy Harvesting
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Award ID(s):
1933502
PAR ID:
10446144
Author(s) / Creator(s):
 ;  ;  ;  ;  ;  
Publisher / Repository:
Wiley Blackwell (John Wiley & Sons)
Date Published:
Journal Name:
Energy Technology
Volume:
10
Issue:
3
ISSN:
2194-4288
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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  1. Dutta, Achyut K. ; Balaya, Palani ; Xu, Sheng (Ed.)
    Monitoring human health in real-time using wearable and implantable electronics (WIE) has become one of the most promising and rapidly growing technologies in the healthcare industry. In general, these electronics are powered by batteries that require periodic replacement and maintenance over their lifetime. To prolong the operation of these electronics, they should have zero post-installation maintenance. On this front, various energy harvesting technologies to generate electrical energy from ambient energy sources have been researched. Many energy harvesters currently available are limited by their power output and energy densities. With the miniaturization of wearable and implantable electronics, the size of the harvesters must be miniaturized accordingly in order to increase the energy density of the harvesters. Additionally, many of the energy harvesters also suffer from limited operational parameters such as resonance frequency and variable input signals. In this work, low frequency motion energy harvesting based on reverse electrowetting-ondielectric (REWOD) is examined using perforated high surface area electrodes with 38 µm pore diameters. Total available surface area per planar area was 8.36 cm2 showing a significant surface area enhancement from planar to porous electrodes and proportional increase in AC voltage density from our previous work. In REWOD energy harvesting, high surface area electrodes significantly increase the capacitance and hence the power density. An AC peak-to-peak voltage generation from the electrode in the range from 1.57-3.32 V for the given frequency range of 1-5 Hz with 0.5 Hz step is demonstrated. In addition, the unconditioned power generated from the harvester is converted to a DC power using a commercial off-theshelf Schottky diode-based voltage multiplier and low dropout regulator (LDO) such that the sensors that use this technology could be fully self-powered. The produced charge is then converted to a proportional voltage by using a commercial charge amplifier to record the features of the motion activities. A transceiver radio is also used to transmit the digitized data from the amplifier and the built-in analog-to-digital converter (ADC) in the micro-controller. This paper proposes the energy harvester acting as a self-powered motion sensor for different physical activities for wearable and wireless healthcare devices. 
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  2. Abstract

    Increasing demand for self-powered wearable sensors has spurred an urgent need to develop energy harvesting systems that can reliably and sufficiently power these devices. Within the last decade, reverse electrowetting-on-dielectric (REWOD)-based mechanical motion energy harvesting has been developed, where an electrolyte is modulated (repeatedly squeezed) between two dissimilar electrodes under an externally applied mechanical force to generate an AC current. In this work, we explored various combinations of electrolyte concentrations, dielectrics, and dielectric thicknesses to generate maximum output power employing REWOD energy harvester. With the objective of implementing a fully self-powered wearable sensor, a “zero applied-bias-voltage” approach was adopted. Three different concentrations of sodium chloride aqueous solutions (NaCl-0.1 M, NaCl-0.5 M, and NaCl-1.0 M) were used as electrolytes. Likewise, electrodes were fabricated with three different dielectric thicknesses (100 nm, 150 nm, and 200 nm) of Al2O3and SiO2with an additional layer of CYTOP for surface hydrophobicity. The REWOD energy harvester and its electrode–electrolyte layers were modeled using lumped components that include a resistor, a capacitor, and a current source representing the harvester. Without using any external bias voltage, AC current generation with a power density of 53.3 nW/cm2was demonstrated at an external excitation frequency of 3 Hz with an optimal external load. The experimental results were analytically verified using the derived theoretical model. Superior performance of the harvester in terms of the figure-of-merit comparing previously reported works is demonstrated. The novelty of this work lies in the combination of an analytical modeling method and experimental validation that together can be used to increase the REWOD harvested power extensively without requiring any external bias voltage.

     
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    The technological promise of soft devices—wearable electronics, implantables, soft robotics, sensors—has accelerated the demand for deformable energy sources. Devices that can convert mechanical energy to electrical energy can enable self‐powered, tetherless, and sustainable devices. This work presents a completely soft and stretchable (>400% strain) energy harvester based on variable‐area electrical‐double‐layer (EDL) capacitors (≈40 µF cm−2). Mechanically varying the EDL area, and thus the capacitance, disrupts equilibrium and generates a driving force for charge movement through an external circuit. Prior EDL capacitors varied the contact area by depressing water droplets between rigid electrodes. In contrast, here, the harvester consists of liquid‐metal electrodes encased in a hydrogel. Deforming the device by ≈25% strain generates a power density ≈0.5 mW m−2. This unconventional approach is attractive because: (1) it does not need an external voltage supply to provide charge; (2) the electrodes themselves deform; and (3) it can work under various modes of deformation such as pressing, stretching, bending, and twisting. The unique ability of the harvester to operate underwater shows promising applications in wearables that contact sweat, underwater sensing, and blue energy harvesting.

     
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