The rheology of lavas and magmas exerts a strong control on the dynamics and hazards posed by volcanic eruptions. Magmas and lavas are complex mixtures of silicate melt, suspended crystals, and gas bubbles. To improve the understanding of the dynamics and effective rheology of magmas and lavas, we performed dam‐break flow experiments using suspensions of silicone oil, sesame seeds, and N2O bubbles. Experiments were run inside a magnetic resonance imaging (MRI) scanner to provide imaging of the flow interior. We varied the volume fraction of sesame seeds between 0 and 0.48, and of bubbles between 0 and 0.21. MRI phase‐contrast velocimetry was used to measure liquid velocity. We fit an effective viscosity to the velocity data by approximating the stress using lubrication theory and the imaged shape of the free surface. In experiments with both particles and bubbles (three‐phase suspensions), we observed shear banding in which particle‐poor regions deform with a lower effective viscosity and dominate flow propagation speed. Our observations demonstrate the importance of considering variations in phase distributions within magmatic fluids and their implications on the dynamics of volcanic eruptions.
Multiphase suspensions are complex systems where microscopic interactions between suspended bubbles, particles, and liquids can significantly alter bulk behavior. Observing the internal mechanics of such suspensions can help constrain the dynamics of natural multiphase flows. To capture these internal processes at high speed and in three dimensions, we propose the use of Swept Confocally Aligned Planar Excitation (SCAPE) microscopy in analog experiments. This imaging technique, developed for neuroscience and biology, uses a sweeping light sheet to illuminate and image fluorophores within a sample. We performed experiments using water and various oils as the liquid phases, glass or PMMA particles for solids, and air or CO2for gas, which we imaged at rates >50 volumes per second, over a volume size of ∼1 × 1 × 0.4 mm. We focused on three case studies: (1) bubble nucleation, growth, and rise in sparkling water, where we found that bubble detachment from angular PMMA particles left residual bubbles that also grew and detached, generating more bubbles compared to smooth particles; (2) flow of immiscible liquids (water droplets suspended in canola oil) in a porous matrix of PMMA beads, which highlighted the importance of pore and throat sizes on droplet velocities; and (3) injection of air bubbles into concentrated suspensions of glass beads or crushed PMMA particles in a refractive‐index‐matched liquid, which revealed particle motion and strong alterations of the bubble shape. We conclude that SCAPE microscopy is a powerful tool to study the dynamics of multiphase systems.
more » « less- NSF-PAR ID:
- 10453770
- Publisher / Repository:
- DOI PREFIX: 10.1029
- Date Published:
- Journal Name:
- Geochemistry, Geophysics, Geosystems
- Volume:
- 22
- Issue:
- 3
- ISSN:
- 1525-2027
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
more » « less
Abstract -
Three-phase suspensions, of liquid that suspends dispersed solid particles and gas bubbles, are common in both natural and industrial settings. Their rheology is poorly constrained, particularly for high total suspended fractions (≳0.5). We use a dam-break consistometer to characterize the rheology of suspensions of (Newtonian) corn syrup, plastic particles and CO 2 bubbles. The study is motivated by a desire to understand the rheology of magma and lava. Our experiments are scaled to the volcanic system: they are conducted in the non-Brownian, non-inertial regime; bubble capillary number is varied across unity; and bubble and particle fractions are 0 ≤ ϕ gas ≤ 0.82 and 0 ≤ ϕ solid ≤ 0.37, respectively. We measure flow-front velocity and invert for a Herschel–Bulkley rheology model as a function of ϕ gas , ϕ solid , and the capillary number. We find a stronger increase in relative viscosity with increasing ϕ gas in the low to intermediate capillary number regime than predicted by existing theory, and find both shear-thinning and shear-thickening effects, depending on the capillary number. We apply our model to the existing community code for lava flow emplacement, PyFLOWGO, and predict increased viscosity and decreased velocity compared with current rheological models, suggesting existing models may not adequately account for the role of bubbles in stiffening lavas.more » « less
-
more » « less
Abstract The ignition of plasmas in liquids has applications from medical instrumentation to manipulation of liquid chemistry. Formation of plasmas directly in a liquid often requires prohibitively large voltages to initiate breakdown. Producing plasma streamers in bubbles submerged in a liquid with higher permittivity can significantly lower the voltage needed to initiate a discharge by reducing the electric field required to produce breakdown. The proximity of the bubble to the electrodes and the shape of the bubbles play critical roles in the manner in which the plasma is produced in, and propagates through, the bubble. In this paper, we discuss results from a three-dimensional direct numerical simulation (DNS) used to investigate the shapes of bubbles formed by injection of air into water. Comparisons are made to results from a companion experiment. A two-dimensional plasma hydrodynamics model was then used to capture the plasma streamer propagation in the bubble using a static bubble geometry generated by the DNS The simulations showed two different modes for streamer formation depending on the bubble shape. In an elliptical bubble, a short electron avalanche triggered a surface ionization wave (SIWs) resulting in plasma propagating along the surface of the bubble. In a circular bubble, an electron avalanche first traveled through the middle of the bubble before two SIWs began to propagate from the point closest to the grounded electrode where a volumetric streamer intersected the surface. In an elliptical bubble approaching a powered electrode in a pin-to-pin configuration, we experimentally observed streamer behavior that qualitatively corresponds with computational results. Optical emission captured over the lifetime of the streamer curve along the path of deformed bubbles, suggesting propagation of the streamer along the liquid/gas boundary interface. Plasma generation supported by the local field enhancement of the deformed bubble surface boundaries is a mechanism that is likely responsible for initiating streamer formation.
-
more » « less
Natural aquatic environments such as oceans, lakes, and rivers are home to a tremendous diversity of microorganisms. Some may cross the air-water interface within droplets and become airborne, with the potential to impact the Earth’s radiation budget, precipitation processes, and spread of disease. Larger droplets are likely to return to the water or adjacent land, but smaller droplets may be suspended in the atmosphere for transport over long distances. Here, we report on a series of controlled laboratory experiments to quantify wind-driven droplet production from a freshwater source for low wind speeds. The rate of droplet production increased quadratically with wind speed above a critical value (10-m equivalent 5.7 m/s) where droplet production initiated. Droplet diameter and ejection speeds were fit by a gamma distribution. The droplet mass flux and momentum flux increased with wind speed. Two mechanisms of droplet production, bubble bursting and fragmentation, yielded different distributions for diameter, speed, and angle. At a wind speed of about 3.5 m/s, aqueous suspensions of the ice-nucleating bacterium
Pseudomonas syringae were collected at rates of 283 cells m−2 s−1at 5 cm above the water surface, and at 14 cells m−2 s−1at 10 cm above the water surface. At a wind speed of about 4.0 m/s, aqueous suspensions ofP. syringae were collected at rates of 509 cells m−2 s−1at 5 cm above the water surface, and at 81 cells m−2 s−1at 10 cm above the water surface. The potential for microbial flux into the atmosphere from aquatic environments was calculated using known concentrations of bacteria in natural freshwater systems. Up to 3.1 × 104 cells m−2 s−1of water surface were estimated to leave the water in potentially suspended droplets (diameters <100 µm). Understanding the sources and mechanisms for bacteria to aerosolize from freshwater aquatic sources may aid in designing management strategies for pathogenic bacteria, and could shed light on how bacteria are involved in mesoscale atmospheric processes. -
Recent studies in polymer physics have created macro-scale analogs to solute microscopic polymer chains like DNA by inducing diffusive motion on a chain of beads. These bead chains have persistence lengths of O(10) links and undergo diffusive motion under random fluctuations like vibration. We present a bead chain model within a new stochastic forcing system: an air fluidizing bed of granular media. A chain of spherical 6 mm resin beads crimped onto silk thread are buffeted randomly by the multiphase flow of grains and low density rising air “bubbles”. We “thermalize” bead chains of various lengths at different fluidizing airflow rates, while X-ray imaging captures a projection of the chains’ dynamics within the media. With modern 3D printing techniques, we can better represent complex polymers by geometrically varying bead connections and their relative strength, e.g., mimicking the variable stiffness between adjacent nucleotide pairs of DNA. We also develop Discrete Element Method (DEM) simulations to study the 3D motion of the bead chain, where the bead chain is represented by simulated spherical particles connected by linear and angular spring-like bonds. In experiment, we find that the velocity distributions of the beads follow exponential distributions rather than the Gaussian distributions expected from polymers in solution. Through use of the DEM simulation, we find that this difference can likely be attributed to the distributions of the forces imparted onto the chain from the fluidized bed environment. We anticipate expanding this study in the future to explore a wide range of chain composition and confinement geometry, which will provide insights into the physics of large biopolymers.more » « less
