Abstract The intensity of tropical cyclones is sensitive to the air-sea fluxes of enthalpy and momentum. Sea spray plays a critical role in mediating enthalpy and momentum fluxes over the ocean’s surface at high wind speeds, and parameterizing the influence of sea spray is a crucial component of any air-sea interaction scheme used for the high wind regime where sea spray is ubiquitous. Many studies have proposed parameterizations of air-sea flux that incorporate the microphysics of sea spray evaporation and the mechanics of sea spray stress. Unfortunately, there is not yet a consensus on which parameterization best represents air-sea exchange in tropical cyclones, and the different proposed parameterizations can yield substantially different tropical cyclone intensities. This paper seeks to review the developments in parameterizations of the sea spray-mediated enthalpy and momentum fluxes for the high wind speed regime and to synthesize key findings that are common across many investigations.
more »
« less
Constraining the Surface Flux of Sea Spray Particles From the Southern Ocean
Abstract Modeling the shortwave radiation balance over the Southern Ocean region remains a challenge for Earth system models. To investigate whether this is related to the representation of aerosol‐cloud interactions, we compared measurements of the total number concentration of sea spray‐generated particles within the Southern Ocean region to model predictions thereof. Measurements were conducted from a container laboratory aboard the R/VTangaroathroughout an austral summer voyage to the Ross Sea. We used source‐receptor modeling to calculate the sensitivity of our measurements to upwind surface fluxes. From this approach, we could constrain empirical parameterizations of sea spray surface flux based on surface wind speed and sea surface temperature. A newly tuned parameterization for the flux of sea spray particles based on the near‐surface wind speed is presented. Comparisons to existing model parameterizations revealed that present model parameterizations led to overestimations of sea spray concentrations. In contrast to previous studies, we found that including sea surface temperature as an explanatory variable did not substantially improve model‐measurement agreement. To test whether or not the parameterization may be applicable globally, we conducted a regression analysis using a database of in situ whitecap measurements. We found that the key fitting parameter within this regression agreed well with the parameterization of sea spray flux. Finally, we compared calculations from the best model of surface flux to boundary layer measurements collected onboard an aircraft throughout the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES), finding good agreement overall.
more »
« less
- Award ID(s):
- 1660537
- PAR ID:
- 10455530
- Publisher / Repository:
- DOI PREFIX: 10.1029
- Date Published:
- Journal Name:
- Journal of Geophysical Research: Atmospheres
- Volume:
- 125
- Issue:
- 4
- ISSN:
- 2169-897X
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Abstract. Sea salt aerosols play an important role in the radiationbudget and atmospheric composition over the Arctic, where the climate israpidly changing. Previous observational studies have shown that Arctic sea ice leads are an important source of sea salt aerosols, and modeling efforts have also proposed blowing snow sublimation as a source. In this study,size-resolved atmospheric particle number concentrations and chemicalcomposition were measured at the Arctic coastal tundra site ofUtqiaġvik, Alaska, during spring (3 April–7 May 2016). Blowing snow conditions were observed during 25 % of the 5-week study period andwere overpredicted by a commonly used blowing snow parameterization based solely on wind speed and temperature. Throughout the study, open leads werepresent locally. During periods when blowing snow was observed, significantincreases in the number concentrations of 0.01–0.06 µm particles(factor of 6, on average) and 0.06–0.3 µm particles (67 %, on average) and a significant decrease (82 %, on average) in 1–4 µmparticles were observed compared to low wind speed periods. These size distribution changes were likely caused by the generation of ultrafineparticles from leads and/or blowing snow, with scavenging of supermicronparticles by blowing snow. At elevated wind speeds, both submicron andsupermicron sodium and chloride mass concentrations were enhanced,consistent with wind-dependent local sea salt aerosol production. Atmoderate wind speeds below the threshold for blowing snow as well as during observed blowing snow, individual sea spray aerosol particles were measured.These individual salt particles were enriched in calcium relative to sodiumin seawater due to the binding of this divalent cation with organic matter in the sea surface microlayer and subsequent enrichment during seawaterbubble bursting. The chemical composition of the surface snowpack alsoshowed contributions from sea spray aerosol deposition. Overall, theseresults show the contribution of sea spray aerosol production from leads onboth aerosols and the surface snowpack. Therefore, if blowing snowsublimation contributed to the observed sea salt aerosol, the snow beingsublimated would have been impacted by sea spray aerosol deposition rather than upward brine migration through the snowpack. Sea spray aerosol production from leads is expected to increase, with thinning and fracturingof sea ice in the rapidly warming Arctic.more » « less
-
Abstract Supercooled liquid clouds are ubiquitous over the Southern Ocean (SO), even to temperatures below −20°C, and comprise a large fraction of the marine boundary layer (MBL) clouds. Earth system models and reanalysis products have struggled to reproduce the observed cloud phase distribution and occurrence of cloud ice in the region. Recent simulations found the microphysical representation of ice nucleation and growth has a large impact on these properties, however, measurements of SO ice nucleating particles (INPs) to validate simulations are sparse. This study presents measurements of INPs from simultaneous aircraft and ship campaigns conducted over the SO in austral summer 2018, which include the first in situ observations in and above cloud in the region. Our results confirm recent observations that INP concentrations are uniformly lower than measurements made in the late 1960s. While INP concentrations below and above cloud are similar, higher ice nucleation efficiency above cloud supports model simulations that the dominant INP composition varies with height. Model parameterizations based solely on aerosol properties capture the mean relationship between INP concentration and temperature but not the observed variability, which is likely related to the only modest correlations observed between INPs and environmental or aerosol metrics. Including wind speed in addition to activation temperature in a marine INP parameterization reduces bias but does not explain the large range of observed INP concentrations. Direct and indirect inference of marine INP size suggests MBL INPs, at least during Austral summer, are dominated by particles with diameters smaller than 500 nm.more » « less
-
Abstract The abundance and sources of ice‐nucleating particles, particles required for heterogeneous ice nucleation, are long‐standing sources of uncertainty in quantifying aerosol‐cloud interactions. In this study, we demonstrate near closure between immersion freezing ice‐nucleating particle number concentration (nINPs) observations andnINPscalculated from simulated sea spray aerosol and dust. The Community Atmospheric Model with constrained meteorology was used to simulate aerosol concentrations at the Mace Head Research Station (North Atlantic) and over the Southern Ocean to the south of Tasmania (Clouds, Aerosols, Precipitation, Radiation, and atmospherIc Composition Over the southeRN ocean campaign). Model‐predictednINPswere within a factor of 10 ofnINPsobserved with an off‐line ice spectrometer at Mace Head Research Station and Clouds, Aerosols, Precipitation, Radiation, and atmospherIc Composition Over the southeRN ocean campaign, for 93% and 69% of observations, respectively. Simulated vertical profiles ofnINPsreveal that transported dust may be critical tonINPsin remote regions and that sea spray aerosol may be the dominate contributor to primary ice nucleation in Southern Ocean low‐level mixed‐phase clouds.more » « less
-
In winter, the Northwest Tropical Atlantic Ocean can be characterized by various wave age-based interactions among ocean current, surface wind and surface waves, which are critical for accurately describing surface wind stress. In this work, coupled wave-ocean-atmosphere model simulations are conducted using two different wave roughness parameterizations within COARE3.5, including one that relies solely on wind speed and another that uses wave age and wave slope as inputs. Comparisons with the directly measured momentum fluxes during the ATOMIC/EUREC4A experiments in winter 2020 show that, for sea states dominated by short wind waves under moderate to strong winds, the wave-based formulation (WBF) increases the surface roughness length in average by 25% compared to the wind-speed-based approach. For sea states dominated by remotely generated swells under moderate to strong wind intensity, the WBF predicts significantly lower roughness length and surface stress (≈15%), resulting in increased near-surface wind speed above the constant flux layer (≈5%). Further investigation of the mixed sea states in the model and data indicates that the impact of swell on wind stress is over-emphasized in the COARE3.5 WBF, especially under moderate wind regimes. Various approaches are explored to alleviate this deficiency by either introducing directional alignment between wind and waves or using the mean wave period instead of the wave period corresponding to the spectral peak to compute the wave age. The findings of this study are likely to be site-dependent, and mostly concern specific regimes of wind and waves where the original parameterization was deficient.more » « less
An official website of the United States government
