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1. Geochemical evolution of municipal water in a natural hydrologic system and implications for urban watershed resilience

   https://doi.org/10.1371/journal.pwat.0000327  

   Manlove, Hunter; Banner, Jay L (December 2024, PLOS Water)

   Kumar, Bimlesh (Ed.)

   Austin, Texas is among the most rapidly urbanizing regions in the U.S., posing challenges to the resilience of its water resources. Geochemical differences between stream water from relatively pristine (rural) and impacted (urban) watersheds indicate several distinct controls on stream water compositions, including extent of urbanization, extent of failure of the city’s municipal water infrastructure, and differences in bedrock composition and permeability. We focus here on the largely unstudied evolution of municipal water once it leaves the infrastructure and enters the natural hydrologic system as groundwater and/or surface water. We use the distinct Sr isotope values (⁸⁷Sr/⁸⁶Sr) and other compositional differences between municipal waters, natural stream and spring water, limestone bedrock, and soils as tracers of the sources of and processes by which four Austin-area streams and springs acquire their dissolved constituents. These processes include 1) fluid-mixing between municipal and natural surface water and groundwater, 2) multiple mineral-solution reactions, including dissolution and water-rock interaction (WRI) processes of precipitation, incongruent dissolution, and recrystallization, and 3) varying groundwater residence times. Stream water in two urbanized watersheds have high⁸⁷Sr/⁸⁶Sr values and ion compositions close to values for municipal water, whereas stream and spring water in two rural watersheds have compositions close to natural stream water. Urbanized stream water compositions can be accounted for by models of municipal water contributions followed by dissolution of bedrock minerals. By contrast, rural stream water compositions are consistent with a model sequence of dissolution followed by extensive WRI with limestone. The results of this study indicate significant contributions to streams from the municipal infrastructure. We find that the evolution of this municipal water in the natural hydrologic system comprises multiple fluid-mixing processes and mineral-solution reactions, which are influenced by differences in bedrock geology. This composite evolution advances our understanding of the complexities of “Urban Stream Syndrome”. 

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2. Positive unintended consequences of urbanization for climate-resilience of stream ecosystems

   https://doi.org/10.1038/s42949-024-00144-1  

   Banner, Jay_L; Black, Bryan_A; Tremaine, Darrel_M (March 2024, npj Urban Sustainability)

   Abstract Developing sustainable urban systems is a fundamental societal challenge for the 21st century, and central Texas faces particularly synergistic challenges of a rapidly growing urban population and a projected increasingly drought-prone climate. To assess the history of urbanization impacts on watersheds here, we analyzed 51 cores from bald cypress trees in paired urban and rural watersheds in Austin, Texas. We find a significant contrast between rural and urbanized watersheds. In the rural watershed, tree-ring-width growth histories (“chronologies”) from 1844–2018 significantly and positively correlate (p < 0.01) with (1) one another, and (2) regional instrumental and proxy records of drought. In the urbanized watershed, by contrast, chronologies weakly correlate with one another, with instrumental records of drought, and with the rural chronologies and regional records. Relatively weak drought limitations to urban tree growth are consistent with the significant present-day transfer of municipal water from urban infrastructure by leakage and irrigation to the natural hydrologic system. We infer a significant, long-term contribution from infrastructure to baseflow in urbanized watersheds. In contrast to the common negative impacts of ‘urban stream syndrome’, such sustained baseflow in watersheds with impaired or failing infrastructure may be an unintended positive consequence for stream ecosystems, as a mitigation against projected extended 21st-century droughts. Additionally, riparian trees may serve as a proxy for past impacts of urbanization on natural streams, which may inform sustainable urban development. 

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3. Expanding radiogenic strontium isotope baseline data for central Mexican paleomobility studies

   https://doi.org/10.1371/journal.pone.0229687  

   Pacheco-Forés, Sofía I.; Gordon, Gwyneth W.; Knudson, Kelly J. (February 2020, PloS one)

   null (Ed.)

   Radiogenic strontium isotopes (87Sr/86Sr) have long been used in analyses of paleomobility within Mesoamerica. While considerable effort has been expended developing 87Sr/86Sr baseline values across the Maya region, work in central Mexico is primarily focused on the Classic period urban center of Teotihuacan. This study adds to this important dataset by presenting bioavailable 87Sr/86Sr values across central Mexico focusing on the Basin of Mexico. This study therefore serves to expand the utility of strontium isotopes across a wider geographic region. A total of 63 plant and water samples were collected from 13 central Mexican sites and analyzed for 87Sr/86Sr on a Thermo-Finnigan Neptune multi-collector inductively coupled plasma mass spectrometer (MC-ICP-MS). These data were analyzed alongside 16 published 87Sr/86Sr values from two additional sites within the region of interest. A five-cluster k-means model was then generated to determine which regions of the Basin of Mexico and greater central Mexico can and cannot be distinguished isotopically using 87Sr/86Sr values. Although the two clusters falling within the Basin of Mexico overlap in their local 87Sr/86Sr ranges, many locations within the Basin are distinguishable using 87Sr/86Sr values at the site-level. This study contributes to paleomobility studies within central Mexico by expanding knowledge of strontium isotope variability within the region, ultimately allowing researchers to detect intra-regional residential mobility and gain a greater understanding of the sociopolitical interactions between the Basin of Mexico and supporting outlying regions of central Mexico. 

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4. Dryland irrigation increases accumulation rates of pedogenic carbonate and releases soil abiotic CO2

   https://doi.org/10.1038/s41598-021-04226-3  

   Ortiz, Anna C.; Jin, Lixin; Ogrinc, Nives; Kaye, Jason; Krajnc, Bor; Ma, Lin (January 2022, Scientific Reports)

   Abstract Agricultural fields in drylands are challenged globally by limited freshwater resources for irrigation and also by elevated soil salinity and sodicity. It is well known that pedogenic carbonate is less soluble than evaporate salts and commonly forms in natural drylands. However, few studies have evaluated how irrigation loads dissolved calcium and bicarbonate to agricultural fields, accelerating formation rates of secondary calcite and simultaneously releasing abiotic CO₂to the atmosphere. This study reports one of the first geochemical and isotopic studies of such “anthropogenic” pedogenic carbonates and CO₂from irrigated drylands of southwestern United States. A pecan orchard and an alfalfa field, where flood-irrigation using the Rio Grande river is a common practice, were compared to a nearby natural dryland site. Strontium and carbon isotope ratios show that bulk pedogenic carbonates in irrigated soils at the pecan orchard primarily formed due to flood-irrigation, and that approximately 20–50% of soil CO₂in these irrigated soils is calcite-derived abiotic CO₂instead of soil-respired or atmospheric origins. Multiple variables that control the salt buildup in this region are identified and impact the crop production and soil sustainability regionally and globally. Irrigation intensity and water chemistry (irrigation water quantity and quality) dictate salt loading, and soil texture governs water infiltration and salt leaching. In the study area, agricultural soils have accumulated up to 10 wt% of calcite after just about 100 years of cultivation. These rates will likely increase in the future due to the combined effects of climate variability (reduced rainfall and more intense evaporation), use of more brackish groundwater for irrigation, and reduced porosity in soils. The enhanced accumulation rates of pedogenic carbonate are accompanied by release of large amounts of abiotic CO₂from irrigated drylands to atmosphere. Extensive field studies and modelling approaches are needed to further quantify these effluxes at local, regional and global scales. 

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5. Irrigated urban trees exhibit greater functional trait plasticity compared to natural stands

   https://doi.org/10.1098/rsbl.2022.0448  

   Ibsen, Peter C.; Santiago, Louis S.; Shiflett, Sheri A.; Chandler, Mark; Jenerette, G. Darrel (January 2023, Biology Letters)

   Urbanization creates novel ecosystems comprised of species assemblages and environments with no natural analogue. Moreover, irrigation can alter plant function compared to non-irrigated systems. However, the capacity of irrigation to alter functional trait patterns across multiple species is unknown but may be important for the dynamics of urban ecosystems. We evaluated the hypothesis that urban irrigation influences plasticity in functional traits by measuring carbon-gain and water-use traits of 30 tree species planted in Southern California, USA spanning a coastal-to-desert gradient. Tree species respond to irrigation through increasing the carbon-gain trait relationship of leaf nitrogen per specific leaf area compared to their native habitat. Moreover, most species shift to a water-use strategy of greater water loss through stomata when planted in irrigated desert-like environments compared to coastal environments, implying that irrigated species capitalize on increased water availability to cool their leaves in extreme heat and high evaporative demand conditions. Therefore, irrigated urban environments increase the plasticity of trait responses compared to native ecosystems, allowing for novel response to climatic variation. Our results indicate that trees grown in water-resource-rich urban ecosystems can alter their functional traits plasticity beyond those measured in native ecosystems, which can lead to plant trait dynamics with no natural analogue. 

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