An official website of the United States government
We have demonstrated that plasmonic metasurfaces composed of arrays of Au bowtie nanoantennas can support an infrared bidirectional superscattering state. This state arises when the nanoantennas are coherently coupled together, forming a surface lattice resonance that efficiently guides the infrared range (1–1.6 μm) of incident broadband white light along the plane of the arrays. This process exhibits strong polarization dependence, offering an “OFF” state where a 90° rotation of the incident light polarization effectively suppresses in-plane scattering from all sides. Stokes parameters analysis is used to study the states of polarization of the scattering, demonstrating transformation into a complete depolarized state. The results emphasize the significant influence of the multipolar modes of these nanoantennas on the interference processes associated with such scattering phenomena, and their potential applications in polarization optical switching and unique beamsplitting.
more »
« less
Spin-polarization control of in-plane scattering in arrays of asymmetric U-shaped nanoantennas
Abstract We study projection-enabled enhancement of asymmetric optical responses of plasmonic metasurfaces for photon-spin control of their far field scattering. Such a process occurs by detecting the light scattered by arrays of asymmetric U-shaped nanoantennas along their planes (in-plane scattering). The nanoantennas are considered to have relatively long bases and two unequal arms. Therefore, as their view angles along the planes of the arrays are changed, they offer an extensive range of shape and size projections, providing a wide control over the contributions of plasmonic near fields and multipolar resonances to the far field scattering of the arrays. We show that this increases the degree of the asymmetric spin-polarization responses of the arrays to circularly polarized light, offering a large amount of chirality. In particular, our results show the in-plane scattering of such metasurfaces can support opposite handedness, offering the possibility of photon spin-dependent directional control of energy routing.
more »
« less
- Award ID(s):
- 1917544
- PAR ID:
- 10480180
- Publisher / Repository:
- Instittue of Physics
- Date Published:
- Journal Name:
- Nanotechnology
- Volume:
- 34
- Issue:
- 41
- ISSN:
- 0957-4484
- Page Range / eLocation ID:
- 415201
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
When a metallic U-shaped nanoantenna (split ring resonator) is observed from its sides, variations in the viewing angle can lead to significantly different size and shape projections. In this study, we demonstrate that plasmonic metasurfaces consisting of arrays of such nanoantennas can support unique side (in-plane) scattering switching and routing processes. These processes encompass a polarization switching centered at 1.6 μm, which is driven by the coherent excitation of the nanoantennas’ multipolar modes. They also include spectrally broadband (0.5–1.6 μm) directional control of the flow of in-plane light scattering. Such a process includes a total prohibition of light emerging from one side of the metasurface for a given polarization of the incident light. However, when such polarization is rotated by 90°, the flow of the in-plane scattering opens with high efficiency. We further discuss the impact of the formation of surface lattice resonance on the coherent amplification of infrared scattering around 1.6 μm and its switching process. The results underscore the influence of variations in asymmetry, associated with the sizes and shape projections, on interference processes. They also showcase how in-plane scattering has the capacity to transfer distinct characteristics of plasmonic near-field asymmetries induced by optical fields into far-field scattering.more » « less
-
Plasmonic metastructures have become valuable platforms for manipulating light based on polarization. While traditional approaches have focused on sorting light through front- or back-scattering, recent advances underscore the potential of in-plane light routing—guiding and separating photons across the surface of the metastructure itself. In this study, we investigate how lateral asymmetry in nanoantenna design—introduced along the direction of in-plane light propagation rather than the axis of illumination—can be leveraged for efficient polarization sorting. We focus on metasurfaces composed of arrays of both symmetric and asymmetric gold nanoantennas. Our results reveal that such structural asymmetry enables two distinct modes of operation: in one, photons with different polarizations are directed along separate in-plane paths; in the other, they follow the same axis but are emitted at different angles depending on their polarization. We further examine the spectral dependence of this sorting behavior and demonstrate that asymmetric metastructures can realize four-way polarization sorting, each with unique anisotropic characteristics. Our simulation results provide insight into how phase modulation of the scattered light—coupled into the substrate beneath the metasurface—is influenced by nanoantenna asymmetry. These findings pave the way for compact, on-chip implementations of the planar spin Hall effect and for simplified metasurfaces suited to sensing, optical switching, and beam steering applications.more » « less
-
Abstract Optical metasurfaces have been widely investigated in recent years as a means to tailor the wavefronts of externally incident light for passive device applications. At the same time, their use in active optoelectronic devices such as light emitters is far less established. This work explores their ability to control the radiation properties of a nearby continuous ensemble of randomly oriented incoherent dipole sources via near‐field interactions. Specifically, a film of colloidal quantum dots is deposited on a plasmonic metasurface consisting of a 1D array of metallic nanoantennas on a metal film. The array is designed to introduce a linear phase profile upon reflection, and a bi‐periodic nanoparticle arrangement is introduced to ensure adequate sampling of the desired phase gradient. Highly directional radiation patterns are correspondingly obtained from the quantum dots at an enhanced emission rate. The underlying radiation mechanism involves the near‐field excitation of surface plasmon polaritons at the metal film, and their selective diffractive scattering by the metasurface into well‐collimated beams along predetermined geometrically tunable directions. These results underscore the distinctive ability of metasurfaces to control radiation properties directly at the source level, which is technologically significant for the continued miniaturization and large‐scale integration of optoelectronic devices.more » « less
-
It is known that the spontaneous emission of semiconductor quantum dots is mostly unpolarized when they are excited off-resonantly. The complete loss of polarization memory is associated with the ultrafast carrier scattering, leading to complete spin polarization relaxation. We study the application of metal-oxide plasmonic double-junction structures to transfer the excitation polarization memory of quantum dots to their spontaneous emission. These structures consist of arrays of metallic nanoantennas in the presence of heterostructures consisting of Au/Si Schottky junctions and Si/Al-oxide charge barriers. Our results show that by using such double-junction structures, one can control the states of polarization and intensity of the emission of quantum dots using the state of polarization of an off-resonant laser field. For achieving this, we explore the optical control of exciton–plasmon coupling using optical lattice modes caused by the arrays of metallic nanoantennas, and the application of the electrostatic field generated by the hot electrons captured at the Au/Si Schottky junction.more » « less
- Free Publicly Accessible Full Text
-
Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1088/1361-6528/ace725
