Abstract Coherence delocalization has been investigated on a coupled‐cavity molecular polariton platform in time, frequency, and spatial domains, enabled by ultrafast two‐dimensional infrared hyperspectral imaging. Unidirectional coherence delocalization (coherence prepared in one cavity transferred to another cavity) has been observed in frequency and real space. This directionality is enabled by the dissipation of delocalized photon from high‐energy to low‐energy modes, described by Lindblad dynamics. Further experiments show that when coherences are directly prepared between polaritons from different cavities, only energetically nearby polaritons can form coherences that survive the long‐range environmental fluctuation. Together with the Lindblad dynamics, this result implies that coherences delocalize through a one‐step mechanism where photons transfer from one cavity to another, shedding light to coherence evolution in natural and artificial quantum systems. This new optical platform based on molecular vibrational polariton thus demonstrates a way of combining photon and molecular modes to simulate coherence dynamics in the infrared regime.
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Smart quantum statistical imaging beyond the Abbe-Rayleigh criterion
Abstract The wave nature of light imposes limits on the resolution of optical imaging systems. For over a century, the Abbe-Rayleigh criterion has been utilized to assess the spatial resolution limits of imaging instruments. Recently, there has been interest in using spatial projective measurements to enhance the resolution of imaging systems. Unfortunately, these schemes require a priori information regarding the coherence properties of “unknown” light beams and impose stringent alignment conditions. Here, we introduce a smart quantum camera for superresolving imaging that exploits the self-learning features of artificial intelligence to identify the statistical fluctuations of unknown mixtures of light sources at each pixel. This is achieved through a universal quantum model that enables the design of artificial neural networks for the identification of photon fluctuations. Our protocol overcomes limitations of existing superresolution schemes based on spatial mode projections, and consequently provides alternative methods for microscopy, remote sensing, and astronomy.
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- Award ID(s):
- 2225986
- PAR ID:
- 10484105
- Editor(s):
- Mary Francina
- Publisher / Repository:
- Nature Publishing Group
- Date Published:
- Journal Name:
- npj Quantum Information
- Edition / Version:
- 1
- Volume:
- 8
- Issue:
- 1
- ISSN:
- 2056-6387
- Page Range / eLocation ID:
- 1
- Subject(s) / Keyword(s):
- Quantum Imaging
- Format(s):
- Medium: X Size: 8 Other: pdf
- Size(s):
- 8
- Sponsoring Org:
- National Science Foundation
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