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1. Two-fold symmetric superconductivity in few-layer NbSe2

   https://doi.org/10.1038/s41567-021-01219-x  

   Hamill, Alex; Heischmidt, Brett; Sohn, Egon; Shaffer, Daniel; Tsai, Kan-Ting; Zhang, Xi; Xi, Xiaoxiang; Suslov, Alexey; Berger, Helmuth; Forró, László; et al (April 2021, Nature Physics)

   null (Ed.)

   The strong Ising spin–orbit coupling in certain two-dimensional transition metal dichalcogenides can profoundly affect the superconducting state in few-layer samples. For example, in NbSe2, this effect combines with the reduced dimensionality to stabilize the superconducting state against magnetic fields up to ~35 T, and could lead to topological superconductivity. Here we report a two-fold rotational symmetry of the superconducting state in few-layer NbSe2 under in-plane external magnetic fields, in contrast to the three-fold symmetry of the lattice. Both the magnetoresistance and critical field exhibit this two-fold symmetry, and it also manifests deep inside the superconducting state in NbSe2/CrBr3 superconductor-magnet tunnel junctions. In both cases, the anisotropy vanishes in the normal state, demonstrating that it is an intrinsic property of the superconducting phase. We attribute the behaviour to the mixing between two closely competing pairing instabilities, namely the conventional s-wave instability typical of bulk NbSe2 and an unconventional d- or p-wave channel that emerges in few-layer NbSe2. Our results demonstrate the unconventional character of the pairing interaction in few-layer transition metal dichalcogenides and highlight the exotic superconductivity in this family of two-dimensional materials. 

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2. Strongly correlated and topological states in [111] grown transition metal oxide thin films and heterostructures

   https://doi.org/10.1063/5.0009092  

   Chakhalian, Jak; Liu, Xiaoran; Fiete, Gregory_A (May 2020, APL Materials)

   We highlight recent advances in the theory, materials fabrication, and experimental characterization of strongly correlated and topological states in [111] oriented transition metal oxide thin films and heterostructures, which are notoriously difficult to realize compared to their [001] oriented counterparts. We focus on two classes of complex oxides, with the chemical formulas ABO3 and A2B2O7, where the B sites are occupied by an open-shell transition metal ion with a local moment and the A sites are typically a rare earth element. The [111] oriented quasi-two-dimensional lattices derived from these parent compound lattices can exhibit peculiar geometries and symmetries, namely, a buckled honeycomb lattice, as well as kagome and triangular lattices. These lattice motifs form the basis for emergent strongly correlated and topological states expressed in exotic magnetism, various forms of orbital ordering, topological insulators, topological semimetals, quantum anomalous Hall insulators, and quantum spin liquids. For transition metal ions with high atomic number, spin–orbit coupling plays a significant role and may give rise to additional topological features in the electronic band structure and in the spectrum of magnetic excitations. We conclude this perspective by articulating open challenges and opportunities in this actively developing field. 

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3. Dynamical criticality of spin-shear coupling in van der Waals antiferromagnets

   https://doi.org/10.1038/s41467-022-34376-5  

   Zhou, Faran; Hwangbo, Kyle; Zhang, Qi; Wang, Chong; Shen, Lingnan; Zhang, Jiawei; Jiang, Qianni; Zong, Alfred; Su, Yifan; Zajac, Marc; et al (December 2022, Nature Communications)

   Abstract The interplay between a multitude of electronic, spin, and lattice degrees of freedom underlies the complex phase diagrams of quantum materials. Layer stacking in van der Waals (vdW) heterostructures is responsible for exotic electronic and magnetic properties, which inspires stacking control of two-dimensional magnetism. Beyond the interplay between stacking order and interlayer magnetism, we discover a spin-shear coupling mechanism in which a subtle shear of the atomic layers can have a profound effect on the intralayer magnetic order in a family of vdW antiferromagnets. Using time-resolved X-ray diffraction and optical linear dichroism measurements, interlayer shear is identified as the primary structural degree of freedom that couples with magnetic order. The recovery times of both shear and magnetic order upon optical excitation diverge at the magnetic ordering temperature with the same critical exponent. The time-dependent Ginzburg-Landau theory shows that this concurrent critical slowing down arises from a linear coupling of the interlayer shear to the magnetic order, which is dictated by the broken mirror symmetry intrinsic to the monoclinic stacking. Our results highlight the importance of interlayer shear in ultrafast control of magnetic order via spin-mechanical coupling. 

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4. Dielectric catastrophe at the Wigner-Mott transition in a moiré superlattice

   https://doi.org/10.1038/s41467-022-32037-1  

   Tang, Yanhao; Gu, Jie; Liu, Song; Watanabe, Kenji; Taniguchi, Takashi; Hone, James C.; Mak, Kin Fai; Shan, Jie (December 2022, Nature Communications)

   Abstract The bandwidth-tuned Wigner-Mott transition is an interaction-driven phase transition from a generalized Wigner crystal to a Fermi liquid. Because the transition is generally accompanied by both magnetic and charge-order instabilities, it remains unclear if a continuous Wigner-Mott transition exists. Here, we demonstrate bandwidth-tuned metal-insulator transitions at fixed fractional fillings of a MoSe 2 /WS 2 moiré superlattice. The bandwidth is controlled by an out-of-plane electric field. The dielectric response is probed optically with the 2s exciton in a remote WSe 2 sensor layer. The exciton spectral weight is negligible for the metallic state with a large negative dielectric constant. It continuously vanishes when the transition is approached from the insulating side, corresponding to a diverging dielectric constant or a ‘dielectric catastrophe’ driven by the critical charge dynamics near the transition. Our results support the scenario of continuous Wigner-Mott transitions in two-dimensional triangular lattices and stimulate future explorations of exotic quantum phases in their vicinities. 

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5. Angular dependence of spin-orbit torque in monolayer ${\mathrm{Fe}}_3{\mathrm{GeTe}}_2$

   https://doi.org/10.1103/PhysRevB.108.144422  

   Xue, Fei; Stiles, Mark D.; Haney, Paul M. (October 2023, Physical Review B)

   In ferromagnetic systems lacking inversion symmetry, an applied electric field can control the ferromagnetic order parameters through the spin-orbit torque. The prototypical example is a bilayer heterostructure composed of a ferromagnet and a heavy metal that acts as a spin current source. In addition to such bilayers, spin-orbit coupling can mediate spin-orbit torques in ferromagnets that lack bulk inversion symmetry. A recently discovered example is the two-dimensional monolayer ferromagnet Fe3GeTe2. In this paper, we use first-principles calculations to study the spin-orbit torque and ensuing magnetic dynamics in this material. By expanding the torque versus magnetization direction as a series of vector spherical harmonics, we find that higher order terms (up to ℓ=4) are significant and play important roles in the magnetic dynamics. They give rise to deterministic, magnetic field-free electrical switching of perpendicular magnetization. 

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