Magnetic tunnel junctions (MTJs) that are comprised of epitaxially-grown complex oxides offer a versatile platform to control the symmetry of tunneling states and tailor magnetic anisotropy useful for practical applications. This work employs thin films of SrTiO3 as an insulating barrier deposited between two ferromagnetic SrRuO3 electrodes to form fully epitaxial MTJs and demonstrate these functionalities. Transport measurements demonstrate large tunneling magnetoresistance (TMR), significantly exceeding previously found values of TMR in MTJs based on SrRuO3 electrodes. These results are explained by perpendicular magnetic anisotropy of SrRuO3 and matching (mismatching) between symmetry and spin across the SrTiO3/SrRuO3 (001) interface for the parallel (antiparallel) MTJ magnetization state, supported by density functional (DFT) calculations. The angular varia- tion of TMR indicates that the SrRuO3 electrodes contain multiple magnetic domains, allowing the devices to exhibit at least three stable resistance states.
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Tunneling magnetoresistance in magnetic tunnel junctions with a single ferromagnetic electrode
Magnetic tunnel junctions (MTJs) are key components of spintronic devices, such as magnetic random-access memories. Normally, MTJs consist of two ferromagnetic (FM) electrodes separated by an insulating barrier layer. Their key functional property is tunneling magnetoresistance (TMR), which is a change in MTJ's resistance when magnetization of the two electrodes alters from parallel to antiparallel. Here, we demonstrate that TMR can occur in MTJs with a single FM electrode, provided that the counter electrode is an antiferromagnetic (AFM) metal that supports a spin-split band structure and/or a Néel spin current. Using RuO2 as a representative example of such antiferromagnet and CrO2 as a FM metal, we design all-rutile RuO2/TiO2/CrO2 MTJs to reveal a non-vanishing TMR. Our first-principles calculations predict that magnetization reversal in CrO2 significantly changes conductance of the MTJs stacked in the (110) or (001) planes. The predicted giant TMR effect of about 1000% in the (110)-oriented MTJs stems from spin-dependent conduction channels in CrO2 (110) and RuO2 (110), whose matching alters with CrO2 magnetization orientation, while TMR in the (001)-oriented MTJs originates from the Néel spin currents and different effective TiO2 barrier thickness for two magnetic sublattices that can be engineered by the alternating deposition of TiO2 and CrO2 monolayers. Our results demonstrate a possibility of a sizable TMR in MTJs with a single FM electrode and offer a practical test for using the antiferromagnet RuO2 in functional spintronic devices.
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- Award ID(s):
- 2316665
- PAR ID:
- 10523798
- Publisher / Repository:
- American Physical Society
- Date Published:
- Journal Name:
- Physical Review B
- Volume:
- 109
- Issue:
- 17
- ISSN:
- 2469-9950
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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