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Abstract Marine cloud brightening (MCB) is proposed to offset global warming by emitting sea salt aerosols to the tropical marine boundary layer, which increases aerosol and cloud albedo. Sea salt aerosol is the main source of tropospheric reactive chlorine (Cly) and bromine (Bry). The effects of additional sea salt on atmospheric chemistry have not been explored. We simulate sea salt aerosol injections for MCB under two scenarios (212–569 Tg/a) in the GEOS‐Chem global chemical transport model, only considering their impacts as a halogen source. Globally, tropospheric Clyand Bryincrease (20–40%), leading to decreased ozone (−3 to −6%). Consequently, OH decreases (−3 to −5%), which increases the methane lifetime (3–6%). Our results suggest that the chemistry of the additional sea salt leads to minor total radiative forcing compared to that of the sea salt aerosol itself (~2%) but may have potential implications for surface ozone pollution in tropical coastal regions.
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Physical science research needed to evaluate the viability and risks of marine cloud brightening
Marine cloud brightening (MCB) is the deliberate injection of aerosol particles into shallow marine clouds to increase their reflection of solar radiation and reduce the amount of energy absorbed by the climate system. From the physical science perspective, the consensus of a broad international group of scientists is that the viability of MCB will ultimately depend on whether observations and models can robustly assess the scale-up of local-to-global brightening in today’s climate and identify strategies that will ensure an equitable geographical distribution of the benefits and risks associated with projected regional changes in temperature and precipitation. To address the physical science knowledge gaps required to assess the societal implications of MCB, we propose a substantial and targeted program of research—field and laboratory experiments, monitoring, and numerical modeling across a range of scales.
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- Award ID(s):
- 2133229
- PAR ID:
- 10523948
- Author(s) / Creator(s):
- ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; more »
- Publisher / Repository:
- Science Advances
- Date Published:
- Journal Name:
- Science Advances
- Volume:
- 10
- Issue:
- 12
- ISSN:
- 2375-2548
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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Since its publication, the authors of Wang et al. (2021) have brought to our attention an error in their article. A grant awarded by the National Science Foundation (grant no. MCB 1817985) to author Elizabeth Vierling was omitted from the Acknowledgements section. The correct Acknowledgements section is shown below. Acknowledgements We thank Suiwen Hou (Lanzhou University) and Zhaojun Ding (Shandong University) for providing the seeds used in this study. We thank Xiaoping Gou (Lanzhou University) and Ravishankar Palanivelu (University of Arizona) for critically reading the manuscript and for suggestions regarding the article. This work was supported by grants from National Natural Science Foundation of China (31870298) to SX, the US Department of Agriculture (USDA-CSREES-NRI-001030) and the National Science Foundation (MCB 1817985) to EV, and the Youth 1000-Talent Program of China (A279021801) to LY.more » « less
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- Free Publicly Accessible Full Text
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Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1126/sciadv.adi8594
