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1. $$^{222}$$Rn  emanation measurements for the XENON1T experiment

   https://doi.org/10.1140/epjc/s10052-020-08777-z  

   Aprile, E.; Aalbers, J.; Agostini, F.; Alfonsi, M.; Althueser, L.; Amaro, F. D.; Antochi, V. C.; Angelino, E.; Angevaare, J. R.; Arneodo, F.; et al (April 2021, The European Physical Journal C)

   null (Ed.)

   Abstract The selection of low-radioactive construction materials is of utmost importance for the success of low-energy rare event search experiments. Besides radioactive contaminants in the bulk, the emanation of radioactive radon atoms from material surfaces attains increasing relevance in the effort to further reduce the background of such experiments. In this work, we present the $$^{222}$$ 222 Rn emanation measurements performed for the XENON1T dark matter experiment. Together with the bulk impurity screening campaign, the results enabled us to select the radio-purest construction materials, targeting a $$^{222}$$ 222 Rn activity concentration of $$10\,\mathrm{\,}\upmu \mathrm{Bq}/\mathrm{kg}$$ 10 μ Bq / kg in $$3.2\,\mathrm{t}$$ 3.2 t of xenon. The knowledge of the distribution of the $$^{222}$$ 222 Rn sources allowed us to selectively eliminate problematic components in the course of the experiment. The predictions from the emanation measurements were compared to data of the $$^{222}$$ 222 Rn activity concentration in XENON1T. The final $$^{222}$$ 222 Rn activity concentration of $$(4.5\pm 0.1)\,\mathrm{\,}\upmu \mathrm{Bq}/\mathrm{kg}$$ ( 4.5 ± 0.1 ) μ Bq / kg in the target of XENON1T is the lowest ever achieved in a xenon dark matter experiment. 

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2. Material radiopurity control in the XENONnT experiment

   https://doi.org/10.1140/epjc/s10052-022-10345-6  

   Aprile, E.; Abe, K.; Agostini, F.; Ahmed Maouloud, S.; Alfonsi, M.; Althueser, L.; Angelino, E.; Angevaare, J. R.; Antochi, V. C.; Antón Martin, D.; et al (July 2022, The European Physical Journal C)

   Abstract The selection of low-radioactive construction materials is of the utmost importance for rare-event searches and thus critical to the XENONnT experiment. Results of an extensive radioassay program are reported, in which material samples have been screened with gamma-ray spectroscopy, mass spectrometry, and $$^{222}$$ 222 Rn emanation measurements. Furthermore, the cleanliness procedures applied to remove or mitigate surface contamination of detector materials are described. Screening results, used as inputs for a XENONnT Monte Carlo simulation, predict a reduction of materials background ( $$\sim $$ ∼ 17%) with respect to its predecessor XENON1T. Through radon emanation measurements, the expected $$^{222}$$ 222 Rn activity concentration in XENONnT is determined to be 4.2 ( $$^{+0.5}_{-0.7}$$ - 0.7 + 0.5 )  $$\upmu $$ μ Bq/kg, a factor three lower with respect to XENON1T. This radon concentration will be further suppressed by means of the novel radon distillation system. 

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3. 3D π : three-dimensional positron imaging, a novel total-body PET scanner using xenon-doped liquid argon scintillator

   https://doi.org/10.1088/1361-6560/adbaac  

   Zabihi, Azam; Li, Xinran; Ramirez, Alejandro; Ahmad, Iftikhar; Da_Rocha_Rolo, Manuel D; Franco, Davide; Gabriele, Federico; Galbiati, Cristiano; Lai, Michela; Marlow, Daniel R; et al (March 2025, Physics in Medicine & Biology)

   Abstract Objective.This paper introduces a novel PET imaging methodology called 3-dimensional positron imaging (3Dπ), which integrates total-body coverage, time-of-flight (TOF) technology, ultra-low dose imaging capabilities, and ultra-fast readout electronics inspired by emerging technology from the DarkSide collaboration.Approach.The study evaluates the performance of 3Dπusing Monte Carlo simulations based on NEMA NU 2-2018 protocols. The methodology employs a homogenous, monolithic scintillator composed of liquid argon (LAr) doped with xenon (Xe) with silicon photomultipliers (SiPMs) operating at cryogenic temperatures.Main results.Substantial improvements in system performance are observed, with the 3Dπsystem achieving a noise equivalent count rate of 3.2 Mcps at 17.3 kBq ml⁻¹, continuing to increase up to 4.3 Mcps at 40 kBq ml⁻¹. Spatial resolution measurements show an average FWHM of 2.7 mm across both axial positions. The system exhibits superior sensitivity, with values reaching 373 kcps MBq⁻¹with a line source at the center of the field of view. Additionally, 3Dπachieves a TOF resolution of 151 ps at 5.3 kBq ml⁻¹, highlighting its potential to produce high-quality images with reduced noise levels.Significance.The study underscores the potential of 3Dπin improving PET imaging performance, offering the potential for shorter scan times and reduced radiation exposure for patients. The Xe-doped LAr offers advantages such as fast scintillation, enhanced light yield, and cost-effectiveness. Future research will focus on optimizing system geometry and further refining reconstruction algorithms to exploit the strengths of 3Dπfor clinical applications. 

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4. Radon Removal in XENONnT down to the Solar Neutrino Level

   https://doi.org/10.1103/zc1w-88p6  

   Aprile, E; Aalbers, J; Abe, K; Ahmed_Maouloud, S; Althueser, L; Andrieu, B; Angelino, E; Antón_Martin, D; Arneodo, F; Baudis, L; et al (September 2025, Physical Review X)

   The XENONnT experiment has achieved an exceptionally low 222 Rn activity concentration within its inner 5.9 tonne liquid xenon detector of (0.90±0.02 stat±0.07 syst)  μ⁢Bq kg−1, equivalent to about 430 222 Rn atoms per tonne of xenon. This was achieved by active online radon removal via cryogenic distillation after stringent material selection. The achieved 222 Rn activity concentration is 5 times lower than that in other currently operational multitonne liquid xenon detectors engaged in dark matter searches. This breakthrough enables the pursuit of various rare event searches that lie beyond the confines of the standard model of particle physics, with world-leading sensitivity. The ultralow 222 Rn levels have diminished the radon-induced background rate in the detector to a point where it is for the first time comparable to the solar neutrino-induced background, which is poised to become the primary irreducible background in liquid xenon-based detectors. 

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5. The XENONnT dark matter experiment

   https://doi.org/10.1140/epjc/s10052-024-12982-5  

   Aprile, E; Aalbers, J; Abe, K; Ahmed_Maouloud, S; Althueser, L; Andrieu, B; Angelino, E; Angevaare, J R; Antochi, V C; Antón_Martin, D; et al (August 2024, The European Physical Journal C)

   Abstract The multi-staged XENON program at INFN Laboratori Nazionali del Gran Sasso aims to detect dark matter with two-phase liquid xenon time projection chambers of increasing size and sensitivity. The XENONnT experiment is the latest detector in the program, planned to be an upgrade of its predecessor XENON1T. It features an active target of 5.9 tonnes of cryogenic liquid xenon (8.5 tonnes total mass in cryostat). The experiment is expected to extend the sensitivity to WIMP dark matter by more than an order of magnitude compared to XENON1T, thanks to the larger active mass and the significantly reduced background, improved by novel systems such as a radon removal plant and a neutron veto. This article describes the XENONnT experiment and its sub-systems in detail and reports on the detector performance during the first science run. 

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