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Title: Anomalous Landau Level Gaps Near Magnetic Transitions in Monolayer WSe2

First-order phase transitions produce abrupt changes to the character of both ground and excited electronic states. Here we conduct electronic compressibility measurements to map the spin phase diagram and Landau level (LL) energies of monolayerWSe2in a magnetic field. We resolve a sequence of first-order phase transitions between completely spin-polarized LLs and states with LLs of both spins. Unexpectedly, the LL gaps are roughly constant over a wide range of magnetic fields below the transitions, which we show reflects spin-polarized ground states with opposite spin excitations. These transitions also extend into compressible regimes, with a sawtooth boundary between full and partial spin polarization. We link these observations to the important influence of LL filling on the exchange energy beyond a smooth density-dependent contribution. Our results show thatWSe2realizes a unique hierarchy of energy scales where such effects induce reentrant magnetic phase transitions tuned by density and magnetic field.

Published by the American Physical Society2024 
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Award ID(s):
2103910
PAR ID:
10532103
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ;
Publisher / Repository:
American Physical Society
Date Published:
Journal Name:
Physical Review X
Volume:
14
Issue:
3
ISSN:
2160-3308
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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Retrieved from https://par.nsf.gov/biblio/10532103. <a href="https://doi.org/10.1103/PhysRevX.14.031018">https://doi.org/10.1103/PhysRevX.14.031018</a> </div> <div class="modal-footer"> <button class="btn btn-sm btn-default" data-dismiss="modal" aria-hidden="true">Close</button> </div> </div> </div> </div></li> <li class="links-format"><a href="#cite-chi" data-toggle="modal">Chicago</a> <div id="cite-chi" class="modal" tabindex="-1" role="dialog" aria-labelledby="cite-chi_label" aria-hidden="true"> <div class="modal-dialog"> <div class="modal-content"> <div class="modal-header"> <button type="button" class="close" data-dismiss="modal" aria-hidden="true">×</button> <strong id="cite-chi_label">Cite: Chicago Format</strong> </div> <div class="modal-body">Foutty, Benjamin A, Calvera, Vladimir, Han, Zhaoyu, Kometter, Carlos R, Liu, Song, Watanabe, Kenji, Taniguchi, Takashi, Hone, James C, Kivelson, Steven A, and Feldman, Benjamin E. "Anomalous Landau Level Gaps Near Magnetic Transitions in Monolayer WSe2". <em>Physical Review X</em> 14 (3). Country unknown/Code not available: American Physical Society. <a href="https://doi.org/10.1103/PhysRevX.14.031018">https://doi.org/10.1103/PhysRevX.14.031018.</a> <a href="https://par.nsf.gov/biblio/10532103">https://par.nsf.gov/biblio/10532103</a>. </div> <div class="modal-footer"> <button class="btn btn-sm btn-default" data-dismiss="modal" aria-hidden="true">Close</button> </div> </div> </div> </div></li> <li class="links-format"><a href="#cite-bib" data-toggle="modal">BibTeX</a> <div id="cite-bib" class="modal" tabindex="-1" role="dialog" aria-labelledby="cite-bib_label" aria-hidden="true"> <div class="modal-dialog"> <div class="modal-content"> <div class="modal-header"> <button type="button" class="close" data-dismiss="modal" aria-hidden="true">×</button> <strong id="cite-bib_label">Cite: BibTeX Format</strong> </div> <div class="modal-body"> @article{osti_10532103,<br/> place = {Country unknown/Code not available}, title = {Anomalous Landau Level Gaps Near Magnetic Transitions in Monolayer WSe2}, url = {https://par.nsf.gov/biblio/10532103}, DOI = {10.1103/PhysRevX.14.031018}, abstractNote = {First-order phase transitions produce abrupt changes to the character of both ground and excited electronic states. Here we conduct electronic compressibility measurements to map the spin phase diagram and Landau level (LL) energies of monolayerWSe2in a magnetic field. We resolve a sequence of first-order phase transitions between completely spin-polarized LLs and states with LLs of both spins. Unexpectedly, the LL gaps are roughly constant over a wide range of magnetic fields below the transitions, which we show reflects spin-polarized ground states with opposite spin excitations. These transitions also extend into compressible regimes, with a sawtooth boundary between full and partial spin polarization. We link these observations to the important influence of LL filling on the exchange energy beyond a smooth density-dependent contribution. Our results show thatWSe2realizes a unique hierarchy of energy scales where such effects induce reentrant magnetic phase transitions tuned by density and magnetic field. Published by the American Physical Society2024}, journal = {Physical Review X}, volume = {14}, number = {3}, publisher = {American Physical Society}, author = {Foutty, Benjamin A and Calvera, Vladimir and Han, Zhaoyu and Kometter, Carlos R and Liu, Song and Watanabe, Kenji and Taniguchi, Takashi and Hone, James C and Kivelson, Steven A and Feldman, Benjamin E}, }</div> <div class="modal-footer"> <button class="btn btn-sm btn-default" data-dismiss="modal" aria-hidden="true">Close</button> </div> </div> </div> </div></li> <li class="divider"></li> </ul> <ul class="nav nav-list" style="font-size: 14px; font-family: Arial Regular;"> <li class="nav-header header-format">Export Metadata</li> <li class="links-format"><a href="https://par.nsf.gov/endnote?osti_id=10532103">EndNote</a></li> <li class="links-format"><a href="https://par.nsf.gov/export/format:excel/osti-id:10532103">Excel</a></li> <li class="links-format"><a href="https://par.nsf.gov/export/format:csv/osti-id:10532103">CSV</a></li> <li class="links-format"><a href="https://par.nsf.gov/export/format:xml/osti-id:10532103">XML</a></li> <li class="divider"></li> </ul> <ul class="nav nav-list" style="font-size: 14px; 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