The suppression of ferroquadrupolar order in TmVO4in a magnetic field is well-described by the transverse field Ising model, enabling detailed studies of critical dynamics near the quantum phase transition. We describe nuclear magnetic resonance measurements in pure and Y-doped single crystals. The non-Kramers nature of the ground state doublet leads to a unique form of the hyperfine coupling that exclusively probes the transverse field susceptibility. Our results show that this quantity diverges at the critical field, in contrast to the mean-field prediction. Furthermore, we find evidence for quantum critical fluctuations present near Tm-rich regions in Y-doped crystals at levels beyond which long-range order is suppressed, suggesting the presence of quantum Griffiths phases.
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Critical behaviour of the quasi-periodic quantum Ising chain
Abstract The interplay of correlated spatial modulation and symmetry breaking leads to quantum critical phenomena intermediate between those of the clean and randomly disordered cases. By performing a detailed analytic and numerical case study of the quasi-periodically (QP) modulated transverse field Ising chain, we provide evidence for the conjectures of reference (Crowleyet al2018Phys. Rev. Lett.120175702) regarding the QP-Ising universality class. In the generic case, we confirm that the logarithmic wandering coefficientwgoverns both the macroscopic critical exponents and the energy-dependent localisation length of the critical excitations. However, for special values of the phase difference Δ between the exchange and transverse field couplings, the QP-Ising transition has different properties. For Δ = 0, a generalised Aubry–André duality prevents the finite energy excitations from localising despite the presence of logarithmic wandering. For Δ such that the fields and couplings are related by a lattice shift, the wandering coefficientwvanishes. Nonetheless, the presence of small couplings leads to non-trivial exponents and localised excitations. Our results add to the rich menagerie of quantum Ising transitions in the presence of spatial modulation.
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- Award ID(s):
- 1752759
- PAR ID:
- 10546478
- Publisher / Repository:
- IOP Publishing
- Date Published:
- Journal Name:
- Journal of Statistical Mechanics: Theory and Experiment
- Volume:
- 2022
- Issue:
- 8
- ISSN:
- 1742-5468
- Page Range / eLocation ID:
- 083102
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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