Abstract The search for new elementary particles is one of the most basic pursuits in physics, spanning from subatomic physics to quantum materials. Magnons are the ubiquitous elementary quasiparticle to describe the excitations of fully-ordered magnetic systems. But other possibilities exist, including fractional and multipolar excitations. Here, we demonstrate that strong quantum interactions exist between three flavors of elementary quasiparticles in the uniaxial spin-one magnet FeI2. Using neutron scattering in an applied magnetic field, we observe spontaneous decay between conventional and heavy magnons and the recombination of these quasiparticles into a super-heavy bound-state. Akin to other contemporary problems in quantum materials, the microscopic origin for unusual physics in FeI2is the quasi-flat nature of excitation bands and the presence of Kitaev anisotropic magnetic exchange interactions.
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Uniaxial stress effect on the electronic structure of quantum materials
Uniaxial stress has proven to be a powerful experimental tuning parameter for effectively controlling lattice, charge, orbital, and spin degrees of freedom in quantum materials. In addition, its ability to manipulate the symmetry of materials has garnered significant attention. Recent technical progress to combine uniaxial stress cells with quantum oscillation and angle-resolved photoemission techniques allowed to study the electronic structure as function of uniaxial stress. This review provides an overview on experimental advancements in methods and examines studies on diverse quantum materials, encompassing the semimetal WTe2, the unconventional superconductor Sr2RuO4, Fe-based superconductors, and topological materials.
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- Award ID(s):
- 2337535
- PAR ID:
- 10575545
- Publisher / Repository:
- Frontiers
- Date Published:
- Journal Name:
- Frontiers in Electronic Materials
- Volume:
- 4
- ISSN:
- 2673-9895
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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Abstract We perform nuclear magnetic resonance (NMR) measurements of the oxygen-17 Knight shifts for Sr2RuO4, while subjected to uniaxial stress applied along [100] direction. The resulting strain is associated with a strong variation of the temperature and magnetic field dependence of the inferred magnetic response. A quasiparticle description based on density-functional theory calculations, supplemented by many-body renormalizations, is found to reproduce our experimental results, and highlights the key role of a van-Hove singularity. The Fermi-liquid coherence scale is shown to be tunable by strain, and driven to low values as the associated Lifshitz transition is approached.more » « less
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