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Unidirectionally propagated electromagnetic waves are rare in nature but heavily sought after due to their potential applications in backscatter-free optical information processing setups. It was theoretically shown that the distinct bulk optical band topologies of a gyrotropic metal and an isotropic metal can enable topologically protected unidirectional surface plasmon polaritons (SPPs) at their interface. Here, we experimentally identify such interfacial modes at terahertz frequencies. Launching the interfacial SPPs via a tailored grating coupler, the far-field spectroscopy data obtained reveals strongly nonreciprocal SPP dispersions that are highly consistent with the theoretical predictions. The directionality of the interfacial SPPs studied here is flexibly tunable by either varying the external field or adjusting the metallic characteristics of the bulk materials. The experimental realization of actively tunable unidirectional SPPs sets the foundation for developing nanophotonic information processing devices based on topologically protected interfacial waves.
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This content will become publicly available on December 1, 2026
Engineering anisotropic electrodynamics at the graphene/CrSBr interface
Abstract Graphene is a privileged 2D platform for hosting confined light-matter excitations known as surface plasmon polaritons (SPPs), as it possesses low intrinsic losses and a high degree of optical confinement. However, the isotropic nature of graphene limits its ability to guide and focus SPPs, making it less suitable than anisotropic elliptical and hyperbolic materials for polaritonic lensing and canalization. Here, we present graphene/CrSBr as an engineered 2D interface that hosts highly anisotropic SPP propagation across mid-infrared and terahertz energies. Using scanning tunneling microscopy, scattering-type scanning near-field optical microscopy, and first-principles calculations, we demonstrate mutual doping in excess of 1013 cm–2holes/electrons between the interfacial layers of graphene/CrSBr. SPPs in graphene activated by charge transfer interact with charge-induced electronic anisotropy in the interfacial doped CrSBr, leading to preferential SPP propagation along the quasi-1D chains that compose each CrSBr layer. This multifaceted proximity effect both creates SPPs and endows them with anisotropic propagation lengths that differ by an order-of-magnitude between the in-plane crystallographic axes of CrSBr.
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- Award ID(s):
- 2308979
- PAR ID:
- 10579167
- Author(s) / Creator(s):
- ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; more »
- Publisher / Repository:
- Nature
- Date Published:
- Journal Name:
- Nature Communications
- Volume:
- 16
- Issue:
- 1
- ISSN:
- 2041-1723
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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