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Title: Accessing bands with extended quantum metric in kagome Cs 2 Ni 3 S 4 through soft chemical processing
Flat bands that do not merely arise from weak interactions can produce exotic physical properties, such as superconductivity or correlated many-body effects. The quantum metric can differentiate whether flat bands will result in correlated physics or are merely dangling bonds. A potential avenue for achieving correlated flat bands involves leveraging geometrical constraints within specific lattice structures, such as the kagome lattice; however, materials are often more complex. In these cases, quantum geometry becomes a powerful indicator of the nature of bands with small dispersions. We present a simple, soft-chemical processing route to access a flat band with an extended quantum metric below the Fermi level. By oxidizing Ni-kagome material Cs2Ni3S4to CsNi3S4, we see a two orders of magnitude drop in the room temperature resistance. However, CsNi3S4is still insulating, with no evidence of a phase transition. Using experimental data, density functional theory calculations, and symmetry analysis, our results suggest the emergence of a correlated insulating state of unknown origin.  more » « less
Award ID(s):
2011750
PAR ID:
10585767
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ;
Publisher / Repository:
Science Advances
Date Published:
Journal Name:
Science Advances
Volume:
10
Issue:
38
ISSN:
2375-2548
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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