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In both particle and wave descriptions of phonons, the dense, aperiodically arranged interfaces in aperiodic superlattices are expected to strongly attenuate thermal transport due to phonon-interface scattering or broken long-range coherence. However, non-trivial thermal conductivity is still observed in these structures. In this study, we reveal that incoherent modes propagating in the aperiodic superlattice can be converted, through interference, into coherent modes defined by an approximate dispersion relation. This conversion leads to high transmission across the aperiodic superlattice structure, which contains hundreds of interfaces, ultimately resulting in non-trivial thermal conductivity. Such incoherent-to-coherent mode-conversion behavior is extensively observed in periodic superlattices. This work suggests an effective strategy to manipulate the phonon dispersion relation through layer patterning or material choice, enabling precise control of phonon transmission across aperiodic superlattices.
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Evolution of Phonon Spectral Energy Density in Superlattice Structures
Superlattices are a distinctive class of artificial nanostructures formed by the periodic stacking of two or more materials. The high density of interfaces in these structures often gives rise to exotic physical properties. In the context of thermal transport, it is well established that such interfaces can significantly scatter particle-like phonons while also inducing constructive or destructive interference in wave-like phonons, depending on the relationship between the phonons’ coherence lengths and the superlattice’s period thickness. In this work, we systematically investigate the effect of temperature on the spectral energy density of phonon modes in superlattices. Additionally, we examine how variations in superlattice period thickness influence phonon lifetimes and energy density. Our findings provide critical insights into the spectral phonon properties of superlattices, particularly in terms of their coherence and lifetimes.
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- PAR ID:
- 10589500
- Publisher / Repository:
- MDPI
- Date Published:
- Journal Name:
- Crystals
- Volume:
- 15
- Issue:
- 5
- ISSN:
- 2073-4352
- Page Range / eLocation ID:
- 446
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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