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Site U1590 (proposed Site CSK-03A) is located 5 km northwest of the submarine Kolumbo crater on its flank in the Anhydros Basin at 397 meters below sea level (mbsl) (Figure F1). It lies on the intersection of Seismic Lines HH06-22 and HH06-34 (Figure F2). Drilling took place in two holes (U1590A and U1590B) to a maximum recovery depth of 627.8 meters below seafloor (mbsf) (all depths below seafloor are given using the core depth below seafloor, Method A [CSF-A], scale, except in Operations, where the drilling depth below seafloor [DSF] scale is used). Average core recovery in Hole U1590A was moderate (61%), but recovery in Hole U1590B was poor (14%). The seismic profiles across the Kolumbo edifice reveal five units interpreted as Kolumbo-derived volcaniclastics (K1–K5, from the base up; Figure F2) with Unit K5 representing the 1650 Common Era (CE) eruption (Hübscher et al., 2015; Preine et al., 2022). The submarine cones northeast of Kolumbo postdate Unit K2 on seismic profiles, but their products are not expected to be prominent in our drill cores. The aim of drilling on the flanks of Kolumbo was to penetrate the different seismically recognized volcanic eruption units from that volcano (K1, K2, K3, and K5 or their thin, lateral equivalents) as well as many eruption units from Santorini and traces from the submarine cones northeast of Kolumbo. This enabled characterization of the products of the Kolumbo eruptions and construction of a coherent stratigraphy for Santorini and the submarine Kolumbo volcano chain together. The anticipated lithologies were volcaniclastics, muds, and turbidites. Site U1590 lies at the foot of the Kolumbo edifice; it allowed us to drill Seismic Units K1, K2, K3, and K5 and therefore nearly the entire history of Kolumbo Volcano. Intercalated seismic units are believed to contain the products of Santorini eruptions, including potentially those of smaller magnitude than recorded at the more distal basin sites.
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Revisiting Néel 60 years on: The magnetic anisotropy of L10 FeNi (tetrataenite)
The magnetocrystalline anisotropy energy of atomically ordered L10 FeNi (the meteoritic mineral tetrataenite) is studied within a first-principles electronic structure framework. Two compositions are examined: equiatomic Fe0.5Ni0.5 and an Fe-rich composition, Fe0.56Ni0.44. It is confirmed that, for the single crystals modeled in this work, the leading-order anisotropy coefficient K1 dominates the higher-order coefficients K2 and K3. To enable comparison with experiment, the effects of both imperfect atomic long-range order and finite temperature are included. While our computational results initially appear to undershoot the measured experimental values for this system, careful scrutiny of the original analysis due to Néel et al. [J. Appl. Phys. 35, 873 (1964)] suggests that our computed value of K1 is, in fact, consistent with experimental values, and that the noted discrepancy has its origins in the nanoscale polycrystalline, multivariant nature of experimental samples, that yields much larger values of K2 and K3 than expected a priori. These results provide fresh insight into the existing discrepancies in the literature regarding the value of tetrataenite’s uniaxial magnetocrystalline anisotropy in both natural and synthetic samples.
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- Award ID(s):
- 2118164
- PAR ID:
- 10594040
- Publisher / Repository:
- American Institute of Physics
- Date Published:
- Journal Name:
- Journal of Applied Physics
- Volume:
- 134
- Issue:
- 16
- ISSN:
- 0021-8979
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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Abstract The production of locally atomically ordered FeNi (known by its meteoric mineral name, tetrataenite) is confirmed in bulk samples by simultaneous conversion X‐ray and backscattered γ‐ray57Fe Mössbauer spectroscopy. Up to 22 volume percent of the tetragonal tetrataenite phase is quantified in samples thermally treated under simultaneous magnetic‐ and stress‐field conditions for a period of 6 weeks, with the remainder identified as the cubic FeNi alloy. In contrast, all precursor samples consist only of the cubic FeNi alloy. Data from the processed alloys are validated using Mössbauer parameters derived from natural meteoritic tetrataenite. The meteoritic tetrataenite exhibits a substantially higher degree of atomic order than do the processed samples, consistent with their low uniaxial magnetocrystalline anisotropy energy of ≈1 kJ·m−3. These results suggest that targeted refinements to the processing conditions of FeNi will foster greater atomic order and increased magnetocrystalline anisotropy, leading to an enhanced magnetic energy product. These outcomes also suggest that deductions concerning paleomagnetic conditions of the solar system, as derived from meteoritic data, may warrant re‐examination and re‐evaluation. Additionally, this work strengthens the argument that tetrataenite may indeed become a member of the advanced permanent magnet portfolio, helping to meet rapidly escalating green energy imperatives.more » « less
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