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1. Radiative decay of the ${}^{229m}\mathrm{Th}$ nuclear clock isomer in different host materials

   https://doi.org/10.1103/PhysRevResearch.7.013052  

   Pineda, S V; Chhetri, P; Bara, S; Elskens, Y; Casci, S; Alexandrova, A N; Au, M; Athanasakis-Kaklamanakis, M; Bartokos, M; Beeks, K; et al (January 2025, Physical Review Research)

   A comparative vacuum ultraviolet spectroscopy study conducted at ISOLDE-CERN of the radiative decay of the ${}^{229m}\mathrm{Th}$nuclear clock isomer embedded in different host materials is reported. The ratio of the number of radiative decay photons and the number of ${}^{229m}\mathrm{Th}$embedded are determined for single crystalline ${\mathrm{CaF}}_2, {\mathrm{MgF}}_2, {\mathrm{LiSrAlF}}_6$, AlN, and amorphous ${\mathrm{SiO}}_2$. For the latter two materials, no radiative decay signal was observed and an upper limit of the ratio is reported. The radiative decay wavelength was determined in ${\mathrm{LiSrAlF}}_6$and ${\mathrm{CaF}}_2$, reducing its uncertainty by a factor of 2.5 relative to our previous measurement. This value is in agreement with the recently reported improved values from laser excitation. Published by the American Physical Society2025 

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2. Reduction of spectroscopic overlap across the $Z=8$ shell in neutron-rich nuclei

   https://doi.org/10.1103/PhysRevC.109.054325  

   Redpath, T; Guèye, P; Baumann, T; Brown, B A; Cunningham, A; DeYoung, P A; Frank, N; Hoffman, C R; Kuchera, A N; Godoy, B Monteagudo; et al (May 2024, Physical Review C)

   Zhang, Lin (Ed.)

   The recent discovery and spectroscopic measurements of ${}^{27}\mathrm{O}$and ${}^{28}\mathrm{O}$suggests the disappearance of the $N=20$shell structure in these neutron-rich oxygen isotopes. We measured one- and two-proton removal cross sections from ${}^{27}\mathrm{F}$and ${}^{29}\mathrm{Ne}$, respectively, extracting spectroscopic factors and comparing them to shell model overlap functions coupled with eikonal reaction model calculations. The invariant mass technique was used to reconstruct the two-body ( ${}^{24}\mathrm{O}+n$) and three-body ( ${}^{24}\mathrm{O}+2n$) decay energies from knockout reactions of ${}^{27}\mathrm{F}$(106.2 MeV/u) and ${}^{29}\mathrm{Ne}$(112.8 MeV/u) beams impinging on a ${}^9\mathrm{Be}$target. The one-proton removal from ${}^{27}\mathrm{F}$strongly populated the ground state of ${}^{26}\mathrm{O}$and the extracted cross section of $3.4_{-1.5}^{+0.3}$mb agrees with eikonal model calculations that are normalized by the shell model spectroscopic factors and account for the systematic reduction factor observed for single nucleon removal reactions within the models used. For the two-proton removal reaction from ${}^{29}\mathrm{Ne}$an upper limit of 0.08 mb was extracted for populating states in ${}^{27}\mathrm{O}$decaying though the ground state of ${}^{26}\mathrm{O}$. The measured upper limit for the population of the ground state of ${}^{26}\mathrm{O}$in the two-proton removal reaction from ${}^{29}\mathrm{Ne}$indicates a significant difference in the underlying nuclear structure of ${}^{27}\mathrm{F}$and ${}^{29}\mathrm{Ne}$. Published by the American Physical Society2024 

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3. Measurement of the Isolated Nuclear Two-Photon Decay in ${}^{72}\mathrm{Ge}$

   https://doi.org/10.1103/PhysRevLett.133.022502  

   Freire-Fernández, D; Korten, W; Chen, R J; Litvinov, S; Litvinov, Yu A; Sanjari, M S; Weick, H; Akinci, F C; Albers, H M; Armstrong, M; et al (July 2024, Physical Review Letters)

   The nuclear two-photon or double-gamma ( $2\gamma$) decay is a second-order electromagnetic process whereby a nucleus in an excited state emits two gamma rays simultaneously. To be able to directly measure the $2\gamma$decay rate in the low-energy regime below the electron-positron pair-creation threshold, we combined the isochronous mode of a storage ring with Schottky resonant cavities. The newly developed technique can be applied to isomers with excitation energies down to $\sim 100\mathrm{keV}$and half-lives as short as $\sim 10\mathrm{ms}$. The half-life for the $2\gamma$decay of the first-excited $0^{+}$state in bare ${}^{72}\mathrm{Ge}$ions was determined to be 23.9(6) ms, which strongly deviates from expectations. Published by the American Physical Society2024 

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4. Shedding Light on the Origin of ${}^{204}\mathrm{Pb}$ , the Heaviest $s$ -Process–Only Isotope in the Solar System

   https://doi.org/10.1103/PhysRevLett.133.052702  

   Casanovas-Hoste, A; Domingo-Pardo, C; Lerendegui-Marco, J; Guerrero, C; Tarifeño-Saldivia, A; Krtička, M; Pignatari, M; Calviño, F; Schumann, D; Heinitz, S; et al (July 2024, Physical Review Letters)

   Asymptotic giant branch stars are responsible for the production of most of the heavy isotopes beyond Sr observed in the solar system. Among them, isotopes shielded from the $r$-process contribution by their stable isobars are defined as $s$-only nuclei. For a long time the abundance of ${}^{204}\mathrm{Pb}$, the heaviest $s$-only isotope, has been a topic of debate because state-of-the-art stellar models appeared to systematically underestimate its solar abundance. Besides the impact of uncertainties from stellar models and galactic chemical evolution simulations, this discrepancy was further obscured by rather divergent theoretical estimates for the neutron capture cross section of its radioactive precursor in the neutron-capture flow, ${}^{204}\mathrm{Tl}$( $t_{1/2}=3.78\mathrm{yr}$), and by the lack of experimental data on this reaction. We present the first ever neutron capture measurement on ${}^{204}\mathrm{Tl}$, conducted at the CERN neutron time-of-flight facility n_TOF, employing a sample of only 9 mg of ${}^{204}\mathrm{Tl}$produced at the Institute Laue Langevin high flux reactor. By complementing our new results with semiempirical calculations we obtained, at the $s$-process temperatures of $kT\approx 8\mathrm{keV}$and $kT\approx 30\mathrm{keV}$, Maxwellian-averaged cross sections (MACS) of 580(168) mb and 260(90) mb, respectively. These figures are about 3% lower and 20% higher than the corresponding values widely used in astrophysical calculations, which were based only on theoretical calculations. By using the new ${}^{204}\mathrm{Tl}$MACS, the uncertainty arising from the ${}^{204}\mathrm{Tl}(\mathrm{n},\gamma )$cross section on the $s$-process abundance of ${}^{204}\mathrm{Pb}$has been reduced from $\sim 30\%$down to $+8\%/-6\%$, and the $s$-process calculations are in agreement with the latest solar system abundance of ${}^{204}\mathrm{Pb}$reported by K. Lodders in 2021. Published by the American Physical Society2024 

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5. Spectroscopy and Modeling of ${}^{171}\mathrm{Yb}$ Rydberg States for High-Fidelity Two-Qubit Gates

   https://doi.org/10.1103/PhysRevX.15.011009  

   Peper, Michael; Li, Yiyi; Knapp, Daniel Y; Bileska, Mila; Ma, Shuo; Liu, Genyue; Peng, Pai; Zhang, Bichen; Horvath, Sebastian P; Burgers, Alex P; et al (January 2025, Physical Review X)

   Highly excited Rydberg states and their interactions play an important role in quantum computing and simulation. These properties can be predicted accurately for alkali atoms with simple Rydberg level structures. However, an extension of these methods to more complex atoms such as alkaline-earth atoms has not been demonstrated or experimentally validated. Here, we present multichannel quantum defect models for highly excited ${}^{174}\mathrm{Yb}$and ${}^{171}\mathrm{Yb}$Rydberg states with $L\le 2$. The models are developed using a combination of existing literature data and new, high-precision laser and microwave spectroscopy in an atomic beam, and validated by detailed comparison with experimentally measured Stark shifts and magnetic moments. We then use these models to compute interaction potentials between two Yb atoms, and find excellent agreement with direct measurements in an optical tweezer array. From the computed interaction potential, we identify an anomalous Förster resonance that likely degraded the fidelity of previous entangling gates in ${}^{171}\mathrm{Yb}$using $F=3/2$Rydberg states. We then identify a more suitable $F=1/2$state, and achieve a state-of-the-art controlled- gate fidelity of $\mathcal{F}=0.994\left(1\right)$, with the remaining error fully explained by known sources. This work establishes a solid foundation for the continued development of quantum computing, simulation, and entanglement-enhanced metrology with Yb neutral atom arrays. Published by the American Physical Society2025 

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