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Great progress has been made in recent years towards understanding the properties of disordered electronic systems. In part, this is made possible by recent advances in quantum effective medium methods which enable the study of disorder and electron-electronic interactions on equal footing. They include dynamical mean-field theory and the Coherent Potential Approximation, and their cluster extension, the dynamical cluster approximation. Despite their successes, these methods do not enable the first-principles study of the strongly disordered regime, including the effects of electronic localization. The main focus of this review is the recently developed typical medium dynamical cluster approximation for disordered electronic systems. This method has been constructed to capture disorder-induced localization and is based on a mapping of a lattice onto a quantum cluster embedded in an effective typical medium, which is determined self-consistently. Unlike the average effective medium-based methods mentioned above, typical medium-based methods properly capture the states localized by disorder. The typical medium dynamical cluster approximation not only provides the proper order parameter for Anderson localized states, but it can also incorporate the full complexity of Density-Functional Theory (DFT)-derived potentials into the analysis, including the effect of multiple bands, non-local disorder, and electron-electron interactions. After a brief historical review of other numerical methods for disordered systems, we discuss coarse-graining as a unifying principle for the development of translationally invariant quantum cluster methods. Together, the Coherent Potential Approximation, the Dynamical Mean-Field Theory and the Dynamical Cluster Approximation may be viewed as a single class of approximations with a much-needed small parameter of the inverse cluster size which may be used to control the approximation. We then present an overview of various recent applications of the typical medium dynamical cluster approximation to a variety of models and systems, including single and multiband Anderson model, and models with local and off-diagonal disorder. We then present the application of the method to realistic systems in the framework of the DFT and demonstrate that the resulting method can provide a systematic first-principles method validated by experiment and capable of making experimentally relevant predictions. We also discuss the application of the typical medium dynamical cluster approximation to systems with disorder and electron-electron interactions. Most significantly, we show that in the limits of strong disorder and weak interactions treated perturbatively, that the phenomena of 3D localization, including a mobility edge, remains intact. However, the metal-insulator transition is pushed to larger disorder values by the local interactions. We also study the limits of strong disorder and strong interactions capable of producing moment formation and screening, with a non-perturbative local approximation. Here, we find that the Anderson localization quantum phase transition is accompanied by a quantum-critical fan in the energy-disorder phase diagram.
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Nonequilibrium steady state full counting statistics in the noncrossing approximation
Quantum transport is often characterized not just by mean observables like the particle or energy current but by their fluctuations and higher moments, which can act as detailed probes of the physical mechanisms at play. However, relatively few theoretical methods are able to access the full counting statistics (FCS) of transport processes through electronic junctions in strongly correlated regimes. While most experiments are concerned with steady state properties, most accurate theoretical methods rely on computationally expensive propagation from a tractable initial state. Here, we propose a simple approach for computing the FCS through a junction directly at the steady state, utilizing the propagator noncrossing approximation. Compared to time propagation, our method offers reduced computational cost at the same level of approximation, but the idea can also be used within other approximations or as a basis for numerically exact techniques. We demonstrate the method’s capabilities by investigating the impact of lead dimensionality on electronic transport in the nonequilibrium Anderson impurity model at the onset of Kondo physics. Our results reveal a distinct signature of one dimensional leads in the noise and Fano factor not present for other dimensionalities, showing the potential of FCS measurements as a probe of the environment surrounding a quantum dot.
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- Award ID(s):
- 2401159
- PAR ID:
- 10616823
- Publisher / Repository:
- American Institute of Physics
- Date Published:
- Journal Name:
- The Journal of Chemical Physics
- Volume:
- 161
- Issue:
- 16
- ISSN:
- 0021-9606
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
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Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1063/5.0233876
