An official website of the United States government
Frequency domain nonlinear spectroscopies are a useful probe of linear and non-linear transitions in a variety of biological, chemical, and materials systems. They require scanning of optical parametric amplifiers (OPAs). Each OPA contains multiple motors that move to prerecorded positions to optimize output at each desired color. OPA optimization and color accuracy are crucial for frequency domain experiments, where OPA color is scanned. Such performance is highly sensitive to environmental fluctuations, so motor positions must be regularly optimized and tuned. Despite the widespread availability of motorized OPAs, this frequent maintenance can make frequency domain spectroscopy a cumbersome and time-consuming process. We have found that fully automated approaches to tuning are invaluable when scanning OPAs. Here, we report four algorithms that accurately and robustly tune a variety of ultrafast laser systems—picosecond and femtosecond, homebuilt and commercial OPAs. Using case studies from previously published work, we illustrate how these four algorithms can be combined to tune all motors of an ultrafast laser system. These algorithms are available through open-source software and can be applied to existing instruments, significantly lowering the threshold for executing frequency domain spectroscopy.
more »
« less
This content will become publicly available on July 1, 2026
Calibration of optical parametric amplifiers for frequency-domain ultrafast coherent multidimensional spectroscopic studies
Frequency-domain ultrafast coherent multidimensional spectroscopy has made possible a family of fully coherent spectroscopies that can create and interrogate characteristic superpositions of the quantum-mechanical states of a system under investigation. Typical applications include the resolution of couplings and dynamics among multiple electronic states in atoms, molecules, and materials. These methods require scanning the wavelengths of multiple, ultrafast light sources—often optical parametric amplifiers (OPAs). Spectral calibration of the OPA output (a.k.a. wavelength-tuning) involves optimizing the OPA output intensity by adjusting the angles of its component nonlinear crystals and motorized delay stages. When the spectral range addressed in the experiment is large, optimization and control of the one or more OPAs become complex. This work describes an automated calibration strategy that measures the multidimensional configuration-space of a typical 800-nm OPA over all angular and delay degrees-of-freedom in order to create a global tuning curve that spans its dynamic spectral range with optimal power and smooth interpolation. To accomplish this task, the optimization assesses the wavelength-dependent variations to the temporal and spatial characteristics of the OPA output caused by material dispersion so that compensations may be applied during a wavelength scan.
more »
« less
- Award ID(s):
- 2203290
- PAR ID:
- 10635008
- Publisher / Repository:
- AIP Publishing1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501
- Date Published:
- Journal Name:
- Review of Scientific Instruments
- Volume:
- 96
- Issue:
- 7
- ISSN:
- 0034-6748
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Floquet state spectroscopy is an optical analogue of multiple quantum coherence nuclear magnetic resonance (MQC-NMR). Tunable ultrafast excitation pulses resonantly excite multiple states in a sample to form the Floquet state. The Floquet state emits multiple coherent beams at frequencies and in directions that conserve energy and momenta. The different output beams differ in the time ordering and coherences created by the excitation beams. They correspond to the different methodologies in the NMR family. Isolating a specific beam and monitoring the output intensity as a function of excitation frequencies creates multidimensional spectra containing cross-peaks between coupled states. The frequency range of the multidimensional spectra is limited by phase matching constraints. This paper presents a new, to the best of our knowledge, active phase matching strategy that increases the versatility of multidimensional Floquet state spectroscopy through both longer sample path lengths and larger spectral ranges.more » « less
-
Integrated optical phased arrays (OPAs) have enabled cutting-edge applications where optical beam steering can benefit from chip-scale integration. However, the majority of integrated OPA demonstrations to date have been limited to showing far-field beam forming and steering. There are, however, many emerging applications of integrated photonics where emission of focused light from a chip is desirable, such as in integrated optical tweezers for biophotonics, chip-based 3D printers, and trapped-ion quantum systems. To address this need, we have recently demonstrated the first near-field-focusing integrated OPAs; however, this preliminary demonstration was limited to emission at only one focal plane above the chip. In this paper, we show the first, to the best of our knowledge, spiral integrated OPAs, enabling emission of focusing beams with tunable variable focal heights for the first time. In the process, we develop the theory, explore the design parameters, and propose feed-structure architectures for such OPAs. Finally, we experimentally demonstrate an example spiral integrated OPA system fabricated in a standard silicon-photonics process, showing wavelength-tunable variable-focal-height focusing emission. This work introduces a first-of-its-kind integrated OPA architecture not previously explored or demonstrated in literature and, as such, enables new functionality for emerging applications of OPAs that require focusing operation.more » « less
-
In this Letter, we present the first, to the best of our knowledge, liquid-crystal-based integrated optical phased arrays (OPAs) that enable visible-light beam forming and steering. A cascaded OPA architecture is developed and experimentally shown to emit a beam in the far field at a 632.8-nm wavelength with a power full width at half maximum of 0.4°×1.6° and 7.2° beam-steering range within ±3.4 V. Furthermore, we show the first visible-light integrated-OPA-based free-space-optical-communications transmitter and use it to demonstrate the first integrated-OPA-based underwater-wireless-optical-communications link. We experimentally demonstrate a 1-Gbps on–off-keying link through water and an electronically-switchable point-to-multipoint link with channel selectivity greater than 19 dB through a water-filled tank.more » « less
-
Optical phased arrays (OPAs) which beam-steer in two dimensions (2D) are currently limited to grating row spacings well above a half wavelength. This gives rise to grating lobes along one axis which limit the field of view (FOV), introduce return signal ambiguity, and reduce the optical efficiency in lidar applications. We demonstrate a Vernier transceiver scheme which uses paired transmit and receive phased arrays with different row periodicities, leading to mismatched grating lobe angular spacings and only a single aligned pair of transmit and receive lobes. This permits a return signal from a target in the desired lobe to be efficiently coupled back into the receive OPA while back-scatter from the other grating lobes is rejected, removing the ambiguity. Our proposal goes beyond previously considered Vernier schemes in other domains like RF and sound, to enable adynamic Vernierwhere all beam directions are simultaneously Vernier aligned, and allow ultra-fast scanning, or multi-beam, operation with Vernier lobe suppression. We analyze two variants of grating lobe suppressing beam-steering configurations, one of which eliminates the FOV limitation, and find the conditions for optimal lobe suppression. We present the first, to the best of our knowledge, experimental demonstration of an OPA Vernier transceiver, including grating lobe suppression of 6.4 dB and beam steering across 5.5°. The demonstration is based on a pair of 2D-wavelength-steered serpentine OPAs. These results address the pervasive issue of grating lobes in integrated photonic lidar schemes, opening the way to larger FOVs and reduced complexity 2D beam-steering designs.more » « less
