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ABSTRACT When arranged in a metasurface, the collective enhancement of field interactions within scattering elements enables precise control over the incident light phase and amplitude. In this work, we analyze collective multipolar resonances in metasurfaces that arise from the spatially extended nature of electromagnetic interactions within these structures, with particular emphasis on MXene metasurfaces. This collective scattering leads to unique and tunable resonance behaviors that reach beyond the simple dipolar approximations, thus enabling advanced manipulation of light at subwavelength scales. We also explore resonances in the scatterers and metasurfaces made of different materials, categorizing them into lossy materials, including transition metal dichalcogenides and conventional metals, and high‐refractive‐index materials, such as silicon. We observe the excitation of MXene multipolar resonances across the visible‐ and infrared‐wavelength spectra and demonstrate their control through the design of scattering elements of the metasurface. We show that periodic lattice arrays support strong localized resonances through the collective response of individual nanoresonators and that one can control multipolar resonances by engineering metasurface nanoresonators and their distribution.
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Multipolar Resonances in Electro‐Optic Metasurfaces with Moderate Refractive Index
The electro‐optic (EO) effect is one of the physical mechanisms enabling the dynamic response of metasurfaces, which motivates the analysis of nanoantenna arrays integrated with EO materials. It was shown earlier that chalcophosphate Sn2P2S6metasurfaces can enable significant shifts of multipolar resonances by enhancing the EO response near the Curie temperature. The present work explores how the refractive index of EO materials impacts resonance shifts in metasurfaces with multipolar resonances. It is numerically demonstrated that EO nanoantennas can support pronounced multipolar resonances despite their moderate refractive index, enabling strong light confinement and substantial EO tuning, and that multipolar components of even parity exhibit the highest sensitivity to variations in the refractive index of the nanoantennas. For moderate refractive indices varying from 2.3 to 3.0, it is found that, for a given resonance, the wavelength shift resulting from a refractive index change has a relatively weak dependence on the index itself. This suggests that the refractive index plays only a marginal role in enhancing the EO shift in active photonic devices, and instead, other considerations for material selection, such as the EO coefficient magnitude, the transparency window, and ease of processing, should be of primary concern.
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- Award ID(s):
- 2418519
- PAR ID:
- 10651755
- Publisher / Repository:
- Wiley Blackwell (John Wiley & Sons)
- Date Published:
- Journal Name:
- Advanced Photonics Research
- ISSN:
- 2699-9293
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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