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Abstract Most brown dwarfs show some level of photometric or spectral variability. However, finding the most variable dwarfs more suited for a thorough variability monitoring campaign remained a challenge until a few years ago with the design of spectral indices to find the most likely L and T dwarfs using their near-infrared (NIR) single-epoch spectrum. In this work, we designed and tested NIR spectral indices to preselect the most likely variable L4–L8 dwarfs, complementing the indices presented by Ashraf et al. and Oliveros-Gomez et al. We used time-resolved NIR Hubble Space Telescope Wide Field Camera 3 spectra of an L6.0 dwarf, LP 261–75b, to design our novel spectral indices. We tested these spectral indices on 75 L4.0–L8.0 NIR SpeX/IRTF spectra, providing 27 new variable candidates. Our indices have a recovery rate of ∼80% and a false negative rate of ∼25%. All the known nonvariable brown dwarfs were found to be nonvariable by our indices. We estimated the variability fraction of our sample to be ${51}_{-38}^{+4}$%, which agrees with the variability fractions provided by Buenzli et al., Radigan et al., and Metchev et al. for L4–L8 dwarfs. These spectral indices may support the future selection of the most likely variable directly imaged exoplanets for studies with the James Webb Space Telescope and as well as the 30 m telescopes. 

Abstract Exoplanet and brown dwarf atmospheres commonly show signs of disequilibrium chemistry. In the James Webb Space Telescope (JWST) era, high-resolution spectra of directly imaged exoplanets will allow the characterization of their atmospheres in more detail, and allow systematic tests for the presence of chemical species that deviate from thermochemical equilibrium in these atmospheres. Constraining the presence of disequilibrium chemistry in these atmospheres as a function of parameters such as their effective temperature and surface gravity will allow us to place better constraints on the physics governing these atmospheres. This paper is part of a series of works presenting the Sonora grid of atmosphere models. In this paper, we present a grid of cloud-free, solar metallicity atmospheres for brown dwarfs and wide-separation giant planets with key molecular species such as CH 4 , H 2 O, CO, and NH 3 in disequilibrium. Our grid covers atmospheres with T eff ∈ [500 K, 1300 K], log g ∈ [3.0, 5.5] (cgs) and an eddy diffusion parameter of log K zz = 2 , 4 and 7 (cgs). We study the effect of different parameters within the grid on the temperature and composition profiles of our atmospheres. We discuss their effect on the near-infrared colors of our model atmospheres and the detectability of CH 4 , H 2 O, CO, and NH 3 using the JWST. We compare our models against existing MKO and Spitzer observations of brown dwarfs and verify the importance of disequilibrium chemistry for T dwarf atmospheres. Finally, we discuss how our models can help constrain the vertical structure and chemical composition of these atmospheres.