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Creators/Authors contains: "Li, Xiaosong"

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  1. ; ; ; ; ; ; ( , Nature Communications)
    Abstract

    Understanding the fluorescence resonance energy transfer (FRET) of metal nanoparticles at the atomic level has long been a challenge due to the lack of accurate systems with definite distance and orientation of molecules. Here we present the realization of achieving FRET between two atomically precise copper nanoclusters through cocrystallization-induced spatial confinement. In this study, we demonstrate the establishment of FRET in a cocrystallized Cu8(p-MBT)8(PPh3)4@Cu10(p-MBT)10(PPh3)4system by exploiting the overlapping spectra between the excitation of the Cu10(p-MBT)10(PPh3)4cluster and the emission of the Cu8(p-MBT)8(PPh3)4cluster, combined with accurate control over the confined space between the two nanoclusters. Density functional theory is employed to provide deeper insights into the role of the distance and dipole orientations of molecules to illustrate the FRET procedure between two cluster molecules at the electronic structure level.

     
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    Free, publicly-accessible full text available December 1, 2025
  2. ; ; ; ; ( , Journal of Chemical Theory and Computation)
    Free, publicly-accessible full text available September 10, 2025
  3. ; ; ; ( , The Journal of Physical Chemistry Letters)
    Free, publicly-accessible full text available June 13, 2025
  4. ; ; ; ( , The Journal of Physical Chemistry Letters)
    Free, publicly-accessible full text available April 18, 2025
  5. ; ; ; ; ( , Journal of the American Chemical Society)
    Free, publicly-accessible full text available April 22, 2025
  6. ; ; ; ; ; ( , The Journal of Physical Chemistry A)
    Free, publicly-accessible full text available April 23, 2025
  7. ; ; ; ; ; ; ( , The Journal of Physical Chemistry A)
    Free, publicly-accessible full text available March 28, 2025
  8. ; ; ; ; ( , Journal of Chemical Theory and Computation)
    Free, publicly-accessible full text available December 26, 2024
  9. ; ; ; ; ; ( , The Journal of Physical Chemistry A)
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  10. ; ; ; ( , Journal of Chemical Theory and Computation)
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