A comprehensive study of the exciton fine structure (EFS) is presented in 2D‐phenethylammonium lead iodide films using magnetic field‐induced polarization of photoluminescence (PL) in both Faraday and Voigt configurations at fields up to 25 Tesla. Three exciton bands are identified in the PL spectrum associated with bound, dark, and bright excitons, respectively. Under a high magnetic field in Faraday/Voigt configuration, large field‐induced circular/linear polarization is observed in the PL band related to the dark exciton, which is magnetically activated. Furthermore, it is found that the dark exciton has an anomalous field‐induced circular polarization, which cannot be explained by the classical Boltzmann distribution of spin‐polarized species. These findings are well explained by an effective mass model that includes exchange terms unique to the monoclinic symmetry as a perturbation of the EFS in the approximate tetragonal symmetry. It is also confirmed that the field‐induced linear polarization is sensitive to the monoclinic exchange term, whereas the field‐induced circular polarization is immune to such term.
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Non-Hermitian Hamiltonians may still have real eigenvalues, provided that a combined parity-time (ƤƮ) symmetry exists. The prospect of ƤƮ symmetry has been explored in several physical systems such as photonics, acoustics, and electronics. The eigenvalues in these systems undergo a transition from real to complex at exceptional points (EPs), where the ƤƮ symmetry is broken. Here, we demonstrate the existence of EP in magnonic devices composed of two coupled magnets with different magnon losses. The eigenfrequencies and damping rates change from crossing to anti-crossing at the EP when the coupling strength increases. The magnonic dispersion includes a strong “acoustic-like” mode and a weak “optic-like” mode. Moreover, upon microwave radiation, the ƤƮ magnonic devices act as magnon resonant cavity with unique response compared to conventional magnonic systems.more » « less
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We have investigated spin related processes in fullerene C 60 devices using several experimental techniques, which include magnetic field effect of photocurrent and electroluminescence in C 60 -based diodes; spin polarized carrier injection in C 60 -based spin-valves; and pure spin current generation in NiFe/C 60 /Pt trilayer devices. We found that the ‘curvature-related spin orbit coupling’ in C 60 plays a dominant role in the obtained spin-related phenomena. The measured magneto-photocurrent and magneto-electroluminescence responses in C 60 diodes are dominated by the difference in the g -values of hole and electron polarons in the fullerene molecules. We also obtained giant magneto-resistance of ∼10% at 10 K in C 60 spin-valve devices, where spin polarized holes are injected into the C 60 interlayer. In addition, using the technique of spin-pumping in NiFe/C 60 /Pt trilayer devices with various C 60 interlayer thicknesses we determined the spin diffusion length in C 60 films to be 13 ± 2 nm at room temperature.more » « less