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Abstract Excitons, bound electron–hole pairs, in two-dimensional hybrid organic inorganic perovskites (2D HOIPs) are capable of forming hybrid light-matter states known as exciton-polaritons (E–Ps) when the excitonic medium is confined in an optical cavity. In the case of 2D HOIPs, they can self-hybridize into E–Ps at specific thicknesses of the HOIP crystals that form a resonant optical cavity with the excitons. However, the fundamental properties of these self-hybridized E–Ps in 2D HOIPs, including their role in ultrafast energy and/or charge transfer at interfaces, remain unclear. Here, we demonstrate that >0.5 µm thick 2D HOIP crystals on Au substrates are capable of supporting multiple-orders of self-hybridized E–P modes. These E–Ps have high Q factors (>100) and modulate the optical dispersion for the crystal to enhance sub-gap absorption and emission. Through varying excitation energy and ultrafast measurements, we also confirm energy transfer from higher energy E–Ps to lower energy E–Ps. Finally, we also demonstrate that E–Ps are capable of charge transport and transfer at interfaces. Our findings provide new insights into charge and energy transfer in E–Ps opening new opportunities towards their manipulation for polaritonic devices. 

Correlated quantum many-body phenomena in lattice models have been identified as a set of physically interesting problems that cannot be solved classically. Analog quantum simulators, in photonics and microwave superconducting circuits, have emerged as near-term platforms to address these problems. An important ingredient in practical quantum simulation experiments is the tomography of the implemented Hamiltonians—while this can easily be performed if we have individual measurement access to each qubit in the simulator, this could be challenging to implement in many hardware platforms. In this paper, we present a scheme for tomography of quantum simulators which can be described by a Bose-Hubbard Hamiltonian while having measurement access to only some sites on the boundary of the lattice. We present an algorithm that uses the experimentally routine transmission and two-photon correlation functions, measured at the boundary, to extract the Hamiltonian parameters at the standard quantum limit. Furthermore, by building on quantum enhanced spectroscopy protocols that, we show that with the additional ability to switch on and off the on-site repulsion in the simulator, we can sense the Hamiltonian parameters beyond the standard quantum limit. Published by the American Physical Society2024 

The wave nature of light sets a fundamental diffraction limit that challenges confinement and control of light in nanoscale structures with dimensions significantly smaller than the wavelength. Here, we study light–matter interaction in van der Waals MoS₂nanophotonic devices. We show that light can be coupled and guided in structures with dimensions as small as ≃λ/16 (∼60nm at 1000 nm excitation wavelength), while offering unprecedented optical field confinement. This deep subwavelength optical field confinement is achieved by exploiting strong lightwave dispersion in MoS₂. We further study the performance of a range of nanophotonic integrated devices via far- and near-field measurements. Our near-field measurements reveal detailed imaging of excitation, evolution, and guidance of fields in nanostructured MoS₂, whereas our far-field study examines light excitation and coupling to highly confined integrated photonics. Nanophotonics at a fraction of a wavelength demonstrated here could dramatically reduce the size of integrated photonic devices and opto-electronic circuits with potential applications in optical information science and engineering.