skip to main content


Search for: All records

Award ID contains: 1849762

Note: When clicking on a Digital Object Identifier (DOI) number, you will be taken to an external site maintained by the publisher. Some full text articles may not yet be available without a charge during the embargo (administrative interval).
What is a DOI Number?

Some links on this page may take you to non-federal websites. Their policies may differ from this site.

  1. Abstract

    Ocean spray aerosol formed by bubble bursting are at the core of a broad range of atmospheric processes: they are efficient cloud condensation nuclei and carry a variety of chemical, biological, and biomass material from the surface of the ocean to the atmosphere. The origin and composition of these aerosols is sensibly controlled by the detailed fluid mechanics of bubble bursting. This perspective summarizes our present-day knowledge on how bursting bubbles at the surface of a liquid pool contribute to its fragmentation, namely to the formation of droplets stripped from the pool, and associated mechanisms. In particular, we describe bounds and yields for each distinct mechanism, and the way they are sensitive to the bubble production and environmental conditions. We also underline the consequences of each mechanism on some of the many air-sea interactions phenomena identified to date. Attention is specifically payed at delimiting the known from the unknown and the certitudes from the speculations.

     
    more » « less
  2. Abstract

    Bubbles bursting at the ocean surface are an important source of ocean‐spray aerosol, with implications on radiative and cloud processes. Yet, very large uncertainties exist on the role of key physical controlling parameters, including wind speed, sea state and water temperature. We propose a mechanistic sea spray generation function that is based on the physics of bubble bursting. The number and mean droplet radius of jet and film drops is described by scaling laws derived from individual bubble bursting laboratory and numerical experiments, as a function of the bubble radius and the water physico‐chemical properties (viscosity, density and surface tension, all functions of temperature), with drops radii at production from 0.1 to 500 µm. Next, we integrate over the bubble size distribution entrained by breaking waves. Finally, the sea spray generation function is obtained by considering the volume flux of entrained bubbles due to breaking waves in the field constrained by the third moment of the breaking distribution (akin to the whitecap coverage). This mechanistic approach naturally integrates the role of wind and waves via the breaking distribution and entrained air flux, and a sensitivity to temperature via individual bubble bursting mechanisms. The resulting sea spray generation function has not been tuned or adjusted to match any existing data sets, in terms of magnitude of sea salt emissions and recently observed temperature dependencies. The remarkable coherence between the model and observations of sea salt emissions therefore strongly supports the mechanistic approach and the resulting sea spray generation function.

     
    more » « less
  3. Abstract

    Laboratory measurements of droplet size, velocity, and accelerations generated by mechanically and wind‐forced water breaking waves are reported. The wind free stream velocity is up to 12 m/s, leading to wave slopes from 0.15 to 0.35 at a fetch of 23 m. The ratio of wind free stream and wave phase speed ranges from 5.9 to 11.1, depending on the mechanical wave frequency. The droplet size distribution in all configurations can be represented by two power laws,N(d) ∝ d−1for drops from 30 to 600 μm andN(d) ∝ d−4above 600 μm. The horizontal and vertical droplet velocities appear correlated, with drops with slower horizontal speed more likely to move upward. The velocity and acceleration distributions are found to be asymmetric, with the velocity probability density functions (PDFs) being described by a normal‐inverse‐Gaussian distribution. The horizontal acceleration PDF are found to follow a shape close to the one predicted for small particles in homogeneous and isotropic turbulence, while the vertical distribution follows an asymmetric normal shape, showing that both acceleration components are controlled by different physical processes.

     
    more » « less
  4. Abstract

    Gas bubbles bursting at the sea surface produce drops, which contribute to marine aerosols. The contamination or enrichment of water by surface‐active agents, of biological or anthropogenic origin, has long been recognized as affecting the bubble bursting processes and the spray composition. However, despite an improved understanding of the physics of a single bursting event, a quantitative understanding of the role of the physico‐chemical conditions on assemblies of bursting bubbles remains elusive. We present experiments on the drop production by millimetric, collective bursting bubbles, under varying surfactant concentration and bubble density. We demonstrate that the production of supermicron droplets (with radius larger than 35 μm) is non‐monotonic as the surfactant concentration increases. The bursting efficiency is optimal for short‐lived, sparsely distributed and non‐coalescing bubbles. We identify the combined role of contamination on the surface bubble arrangement and the modification of the jet drop production process in the bursting efficiency.

     
    more » « less
  5. We investigate wind wave growth by direct numerical simulations solving for the two-phase Navier–Stokes equations. We consider the ratio of the wave speed $c$ to the wind friction velocity $u_*$ from $c/u_*= 2$ to 8, i.e. in the slow to intermediate wave regime; and initial wave steepness $ak$ from 0.1 to 0.3; the two being varied independently. The turbulent wind and the travelling, nearly monochromatic waves are fully coupled without any subgrid-scale models. The wall friction Reynolds number is 720. The novel fully coupled approach captures the simultaneous evolution of the wave amplitude and shape, together with the underwater boundary layer (drift current), up to wave breaking. The wave energy growth computed from the time-dependent surface elevation is in quantitative agreement with that computed from the surface pressure distribution, which confirms the leading role of the pressure forcing for finite amplitude gravity waves. The phase shift and the amplitude of the principal mode of surface pressure distribution are systematically reported, to provide direct evidence for possible wind wave growth theories. Intermittent and localised airflow separation is observed for steep waves with small wave age, but its effect on setting the phase-averaged pressure distribution is not drastically different from that of non-separated sheltering. We find that the wave form drag force is not a strong function of wave age but closely related to wave steepness. In addition, the history of wind wave coupling can affect the wave form drag, due to the wave crest shape and other complex coupling effects. The normalised wave growth rate we obtain agrees with previous studies. We make an effort to clarify various commonly adopted underlying assumptions, and to reconcile the scattering of the data between different previous theoretical, numerical and experimental results, as we revisit this longstanding problem with new numerical evidence. 
    more » « less
  6. We present high-resolution three-dimensional (3-D) direct numerical simulations of breaking waves solving for the two-phase Navier–Stokes equations. We investigate the role of the Reynolds number ( Re , wave inertia relative to viscous effects) and Bond number ( Bo , wave scale over the capillary length) on the energy, bubble and droplet statistics of strong plunging breakers. We explore the asymptotic regimes at high Re and Bo , and compare with laboratory breaking waves. Energetically, the breaking wave transitions from laminar to 3-D turbulent flow on a time scale that depends on the turbulent Re up to a limiting value $Re_\lambda \sim 100$ , consistent with the mixing transition in other canonical turbulent flows. We characterize the role of capillary effects on the impacting jet and ingested main cavity shape and subsequent fragmentation process, and extend the buoyant-energetic scaling from Deike et al. ( J. Fluid Mech. , vol. 801, 2016, pp. 91–129) to account for the cavity shape and its scale separation from the Hinze scale, $r_H$ . We confirm two regimes in the bubble size distribution, $N(r/r_H)\propto (r/r_H)^{-10/3}$ for $r>r_H$ , and $\propto (r/r_H)^{-3/2}$ for $r more » « less
  7. Breaking waves modulate the transfer of energy, momentum, and mass between the ocean and atmosphere, controlling processes critical to the climate system, from gas exchange of carbon dioxide and oxygen to the generation of sea spray aerosols that can be transported in the atmosphere and serve as cloud condensation nuclei. The smallest components, i.e., drops and bubbles generated by breaking waves, play an outsize role. This fascinating problem is characterized by a wide range of length scales, from wind forcing the wave field at scales of [Formula: see text](1 km–0.1 m) to the dynamics of wave breaking at [Formula: see text](10–0.1 m); air bubble entrainment, dynamics, and dissolution in the water column at [Formula: see text](1 m–10 μm); and bubbles bursting at [Formula: see text](10 mm–1 μm), generating sea spray droplets at [Formula: see text](0.5 mm–0.5 μm) that are ejected into atmospheric turbulent boundary layers. I discuss recent progress to bridge these length scales, identifying the controlling processes and proposing a path toward mechanistic parameterizations of air–sea mass exchange that naturally accounts for sea state effects. 
    more » « less