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Abstract The hope for a futuristic global quantum internet that provides robust and high-capacity quantum information transfer lies largely on qudits, the fundamental quantum information carriers prepared in high-dimensional superposition states. However, preparing and manipulating N-dimensional flying qudits as well as subsequently establishing their entanglement are still challenging tasks, which require precise and simultaneous maneuver of 2 (N-1) parameters across multiple degrees of freedom. Here, using an integrated approach, we explore the synergy from two degrees of freedom of light, spatial mode and polarization, to generate, encode, and manipulate flying structured photons and their formed qudits in a four-dimensional Hilbert space with high quantum fidelity, intrinsically enabling enhanced noise resilience and higher quantum data rates. The four eigen spin–orbit modes of our qudits possess identical spatial–temporal characteristics in terms of intensity distribution and group velocity, thereby preserving long-haul coherence within the entirety of the quantum data transmission link. Judiciously leveraging the bi-photon entanglement, which is well preserved in the integrated manipulation process, we present versatile spin–orbit cluster states in an extensive dimensional Hilbert space. Such cluster states hold the promise for quantum error correction which can further bolster the channel robustness in long-range quantum communication. 

Abstract Coherent control and manipulation of quantum degrees of freedom such as spins forms the basis of emerging quantum technologies. In this context, the robust valley degree of freedom and the associated valley pseudospin found in two‐dimensional transition metal dichalcogenides is a highly attractive platform. Valley polarization and coherent superposition of valley states have been observed in these systems even up to room temperature. Control of valley coherence is an important building block for the implementation of valley qubit. Large magnetic fields or high‐power lasers have been used in the past to demonstrate the control (initialization and rotation) of the valley coherent states. Here, the control of layer–valley coherence via strong coupling of valley excitons in bilayer WS₂to microcavity photons is demonstrated by exploiting the pseudomagnetic field arising in optical cavities owing to the transverse electric–transverse magnetic (TE–TM)mode splitting. The use of photonic structures to generate pseudomagnetic fields which can be used to manipulate exciton‐polaritons presents an attractive approach to control optical responses without the need for large magnets or high‐intensity optical pump powers. 

Abstract On-chip integrated laser sources of structured light carrying fractional orbital angular momentum (FOAM) are highly desirable for the forefront development of optical communication and quantum information–processing technologies. While integrated vortex beam generators have been previously demonstrated in different optical settings, ultrafast control and sweep of FOAM light with low-power control, suitable for high-speed optical communication and computing, remains challenging. Here we demonstrate fast control of the FOAM from a vortex semiconductor microlaser based on fast transient mixing of integer laser vorticities induced by a control pulse. A continuous FOAM sweep between charge 0 and charge +2 is demonstrated in a 100 ps time window, with the ultimate speed limit being established by the carrier recombination time in the gain medium. Our results provide a new route to generating vortex microlasers carrying FOAM that are switchable at GHz frequencies by an ultrafast control pulse.