Metasurfaces are two-dimensional nanoantenna arrays that can control the propagation of light at will. In particular, plasmonic metasurfaces feature ultrathin thicknesses, ease of fabrication, field confinement beyond the diffraction limit, superior nonlinear properties, and ultrafast performances. However, the technological relevance of plasmonic metasurfaces operating in the transmission mode at optical frequencies is questionable due to their limited efficiency. The state-of-the-art efficiency of geometric plasmonic metasurfaces at visible and near-infrared frequencies, for example, is ≤10%. Here, we report a multipole-interference-based transmission-type geometric plasmonic metasurface with a polarization conversion efficiency that reaches 42.3% at 744 nm, over 400% increase over the state of the art. The efficiency is augmented by breaking the scattering symmetry due to simultaneously approaching the generalized Kerker condition for two orthogonal polarizations. In addition, the design of the metasurface proposed in this study introduces an air gap between the antennas and the surrounding media that confines the field within the gap, which mitigates the crosstalk between meta-atoms and minimizes metallic absorption. The proposed metasurface is broadband, versatile, easy to fabricate, and highly tolerant to fabrication errors. We highlight the technological relevance of our plasmonic metasurface by demonstrating a transmission-type beam deflector and hologram with record efficiencies.
Metasurfaces have drawn considerable attentions for their revolutionary capability of tailoring the amplitude, phase, and polarization of light. By integrating the nonlinear optical processes into metasurfaces, new wavelengths are introduced as an extra degree of freedom for further advancing the device performance. However, most of the existing nonlinear plasmonic metasurfaces are based on metallic nanoantennas as meta‐atoms, suffering from strong background transmission, low laser damage threshold and small nonlinear conversion efficiency. Here, Babinet‐inverted plasmonic metasurfaces made of C‐shaped nanoapertures as meta‐atoms are designed and demonstrated to solve these issues. Rotation‐gradient nonlinear metasurfaces are further constructed for producing spin‐selective second‐harmonic vortex beams with the orbital angular momentum (OAM) and beam diffraction angle determined by both the spin states of the fundamental wave and second‐harmonic emission. The results enable new types of functional metasurface chips for applications in spin, OAM, and wavelength multiplexed optical trapping, all‐optical communication, and optical data storage.
more » « less- NSF-PAR ID:
- 10063627
- Publisher / Repository:
- Wiley Blackwell (John Wiley & Sons)
- Date Published:
- Journal Name:
- Advanced Optical Materials
- Volume:
- 6
- Issue:
- 19
- ISSN:
- 2195-1071
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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