Metasurfaces have drawn considerable attentions for their revolutionary capability of tailoring the amplitude, phase, and polarization of light. By integrating the nonlinear optical processes into metasurfaces, new wavelengths are introduced as an extra degree of freedom for further advancing the device performance. However, most of the existing nonlinear plasmonic metasurfaces are based on metallic nanoantennas as meta‐atoms, suffering from strong background transmission, low laser damage threshold and small nonlinear conversion efficiency. Here, Babinet‐inverted plasmonic metasurfaces made of C‐shaped nanoapertures as meta‐atoms are designed and demonstrated to solve these issues. Rotation‐gradient nonlinear metasurfaces are further constructed for producing spin‐selective second‐harmonic vortex beams with the orbital angular momentum (OAM) and beam diffraction angle determined by both the spin states of the fundamental wave and second‐harmonic emission. The results enable new types of functional metasurface chips for applications in spin, OAM, and wavelength multiplexed optical trapping, all‐optical communication, and optical data storage.
Wavelength, polarization and orbital angular momentum of light are important degrees of freedom for processing and encoding information in optical communication. Over the years, the generation and conversion of orbital angular momentum in nonlinear optical media has found many novel applications in the context of optical communication and quantum information processing. With that hindsight, here orbital angular momentum conversion of optical vortices through second-harmonic generation from only one atomically thin WS2monolayer is demonstrated at room temperature. Moreover, it is shown that the valley-contrasting physics associated with the nonlinear optical selection rule in WS2monolayer precisely determines the output circular polarization state of the generated second-harmonic vortex. These results pave the way for building future miniaturized valleytronic devices with atomic-scale thickness for many applications such as chiral photon emission, nonlinear beam generation, optoelectronics, and quantum computing.
more » « less- NSF-PAR ID:
- 10154147
- Publisher / Repository:
- Nature Publishing Group
- Date Published:
- Journal Name:
- Scientific Reports
- Volume:
- 9
- Issue:
- 1
- ISSN:
- 2045-2322
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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