An official website of the United States government
The energetics of drop deposition are considered in the capillary-ballistic regime characterized by high Reynolds number and moderate Weber number. Experiments are performed impacting water/glycol drops onto substrates with varying wettability and contact-angle hysteresis. The impacting event is decomposed into three regimes: (i) pre-impact, (ii) inertial spreading and (iii) post contact-line (CL) pinning, conveniently framed using the theory of Dussan & Davis ( J. Fluid Mech. , vol. 173, 1986, pp. 115–130). During fast-time-scale inertial spreading, the only form of dissipation is CL dissipation ( $$\mathcal {D}_{CL}$$ ). High-speed imaging is used to resolve the stick-slip dynamics of the CL with $$\mathcal {D}_{CL}$$ measured directly from experiment using the $$\Delta \alpha$$ - $$R$$ cyclic diagram of Xia & Steen ( J. Fluid Mech. , vol. 841, 2018, pp. 767–783), representing the contact-angle deviation against the CL radius. Energy loss occurs on slip legs, and this observation is used to derive a closed-form expression for the kinetic K and interfacial $$\mathcal{A}$$ post-pinning energy $$\{K+\mathcal {A}\}_p/\mathcal {A}_o$$ independent of viscosity, only depending on the rest angle $$\alpha _p$$ , equilibrium angle $$\bar {\alpha }$$ and hysteresis $$\Delta \alpha$$ , which agrees well with experimental observation over a large range of parameters, and can be used to evaluate contact-line dissipation during inertial spreading. The post-pinning energy is found to be independent of the pre-impact energy, and it is broken into modal components with corresponding energy partitioning approximately constant for low-hysteresis surfaces with fixed pinning angle $$\alpha _p$$ . During slow-time-scale post-pinning, the liquid/gas ( $lg$ ) interface is found to vibrate with the frequencies and mode shapes predicted by Bostwick & Steen ( J. Fluid Mech. , vol. 760, 2014, pp. 5–38), irrespective of the pre-impact energy. Resonant mode decay rates are determined experimentally from fast Fourier transforms of the interface dynamics.
more »
« less
Dissipation of oscillatory contact lines using resonant mode scanning
Abstract Moving contact-lines (CLs) dissipate. Sessile droplets, mechanically driven into resonance by plane-normal forcing of the contacting substrate, can exhibit oscillatory CL motions with CL losses dominating bulk dissipation. Conventional practice measures CL dissipation based on the rate of mechanical work of the unbalanced Young’s force at the CL. Typical approaches require measurements local to the CL and assumptions about the “equilibrium” contact angle (CA). This paper demonstrates how to use scanning of forcing frequency to characterize CL dissipation without any dependence on measurements from the vicinity of the CL. The results are of immediate relevance to an International Space Station (ISS) experiment and of longer-term relevance to Earth-based wettability applications. Experiments reported here use various concentrations of a water-glycerol mixture on a low-hysteresis non-wetting substrate.
more »
« less
- Award ID(s):
- 1637960
- PAR ID:
- 10154266
- Publisher / Repository:
- Nature Publishing Group
- Date Published:
- Journal Name:
- npj Microgravity
- Volume:
- 6
- Issue:
- 1
- ISSN:
- 2373-8065
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Abstract Thermoelastic loss is an important energy dissipation mechanisms in resonant systems. A careful analysis of the thermoelastic loss is critical to the design of low-noise devices for high-precision applications, such as the mirrors used for gravitational-wave (GW) detectors. In this paper, we present analytical solutions to the thermoelastic loss due to thermoelasticity between different materials that are in contact. We find expressions for the thermoelastic loss of multimaterial coatings of finite substrates, and analyze its dependencies on material properties, mirror design and operating experimental conditions. Our results show that lower operating mirror temperature, thinner layers and higher number of interfaces in the coating, and the choice of the first layer of the coating that minimizes the thermal expansion mismatch with the substrate are strategies that reduce the thermoelastic loss and, therefore, diminish the thermal noise that limits the resolution in sensing applications. The results presented in this paper are relevant for the development of low-noise GW detectors and for other experiments sensitive to energy dissipation mechanisms when different materials are in contact.more » « less
-
Abstract Graphene's wetting transparency offers promising avenues for creating multifunctional devices by allowing real‐time wettability control on liquid substrates via the flow of different liquids beneath graphene. Despite its potential, direct measurement of floating graphene's wettability remains a challenge, hindering the exploration of these applications. The current study develops an experimental methodology to assess the wetting transparency of single‐layer graphene (SLG) on liquid substrates. By employing contact angle measurements and Neumann's Triangle model, the challenge of evaluating the wettability of floating free‐suspended single‐layer graphene is addressed. The research reveals that for successful contact angle measurements, the testing and substrate liquids must be immiscible. Using diiodomethane as the testing liquid and ammonium persulfate solution as liquid substrate, the study demonstrates the near‐complete wetting transparency of graphene. Furthermore, it successfully showcases the feasibility of real‐time wettability control using graphene on liquid substrates. This work not only advances the understanding of graphene's interaction with liquid interfaces but also suggests a new avenue for the development of multifunctional materials and devices by exploiting the unique wetting transparency of graphene.more » « less
-
PurposePowder bed density is a key parameter in powder bed additive manufacturing (AM) processes but is not easily monitored. This research evaluates the possibility of non-invasively estimating the density of an AM powder bed via its thermal properties measured using flash thermography (FT). Design/methodology/approachThe thermal diffusivity and conductivity of the samples were found by fitting an analytical model to the measured surface temperature after flash of the powder on a polymer substrate, enabling the estimation of the powder bed density. FindingsFT estimated powder bed was within 8% of weight-based density measurements and the inferred thermal properties are consistent with literature findings. However, multiple flashes were necessary to ensure precise measurements due to noise in the experimental data and the similarity of thermal properties between the powder and substrate. Originality/valueThis paper emphasizes the capability of Flash Thermography (FT) for non-contact measurement of SS 316 L powder bed density, offering a pathway to in-situ monitoring for powder bed AM methods including binder jetting (BJ) and powder bed fusion. Despite the limitations of the current approach, the density knowledge and thermal properties measurements have the potential to enhance process development and thermal modeling powder bed AM processes, aiding in understanding the powder packing and thermal behavior.more » « less
-
A mechanistic understanding of adhesion in soft materials is critical in the fields of transportation (tires, gaskets, and seals), biomaterials, microcontact printing, and soft robotics. Measurements have long demonstrated that the apparent work of adhesion coming into contact is consistently lower than the intrinsic work of adhesion for the materials, and that there is adhesion hysteresis during separation, commonly explained by viscoelastic dissipation. Still lacking is a quantitative experimentally validated link between adhesion and measured topography. Here, we used in situ measurements of contact size to investigate the adhesion behavior of soft elastic polydimethylsiloxane hemispheres (modulus ranging from 0.7 to 10 MPa) on 4 different polycrystalline diamond substrates with topography characterized across 8 orders of magnitude, including down to the angstrom scale. The results show that the reduction in apparent work of adhesion is equal to the energy required to achieve conformal contact. Further, the energy loss during contact and removal is equal to the product of the intrinsic work of adhesion and the true contact area. These findings provide a simple mechanism to quantitatively link the widely observed adhesion hysteresis to roughness rather than viscoelastic dissipation.more » « less
