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1. Mid-IR spectroscopy of Er ³⁺ doped low-phonon CsCdCl ₃ and CsPbCl ₃ crystals

   https://doi.org/10.1364/JOSAB.470152  

   Brown, Ei_Ei; Fleischman, Zackery_D; McKay, Jason; Hommerich, Uwe; Kabir, Al_Amin; Riggins, Jazmine; Trivedi, Sudhir; Dubinskii, Mark (September 2022, Journal of the Optical Society of America B)

   The mid-IR spectroscopic properties of ${\mathrm{E}\mathrm{r}}^{3+}$doped low-phonon ${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$and ${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$crystals grown by the Bridgman technique have been investigated. Using optical excitations at $\sim <\#comment/>800\mathrm{n}\mathrm{m}$and $\sim <\#comment/>660\mathrm{n}\mathrm{m}$, both crystals exhibited IR emissions at $\sim <\#comment/>1.55$, $\sim <\#comment/>2.75$, $\sim <\#comment/>3.5$, and $\sim <\#comment/>4.5\text{µ<\#comment/>}\mathrm{m}$at room temperature. The mid-IR emission at 4.5 µm, originating from the ${}^4{\mathrm{I}}_{9/2}\to <\#comment/>{}^4{\mathrm{I}}_{11/2}$transition, showed a long emission lifetime of $\sim <\#comment/>11.6\mathrm{m}\mathrm{s}$for ${\mathrm{E}\mathrm{r}}^{3+}$doped ${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$, whereas ${\mathrm{E}\mathrm{r}}^{3+}$doped ${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$exhibited a shorter lifetime of $\sim <\#comment/>1.8\mathrm{m}\mathrm{s}$. The measured emission lifetimes of the ${}^4{\mathrm{I}}_{9/2}$state were nearly independent of the temperature, indicating a negligibly small nonradiative decay rate through multiphonon relaxation, as predicted by the energy-gap law for low-maximum-phonon energy hosts. The room temperature stimulated emission cross sections for the ${}^4{\mathrm{I}}_{9/2}\to <\#comment/>{}^4{\mathrm{I}}_{11/2}$transition in ${\mathrm{E}\mathrm{r}}^{3+}$doped ${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$and ${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$were determined to be $\sim <\#comment/>0.14\times <\#comment/>{10}^{-<\#comment/>20}{\mathrm{c}\mathrm{m}}^2$and $\sim <\#comment/>0.41\times <\#comment/>{10}^{-<\#comment/>20}{\mathrm{c}\mathrm{m}}^2$, respectively. The results of Judd–Ofelt analysis are presented and discussed. 

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2. Determination of size and complex index of refraction of single particles with elastic light scattering

   https://doi.org/10.1364/AO.413675  

   Waez, Mir_Seliman; Eckels, Steven_J; Sorensen, Christopher_M (January 2021, Applied Optics)

   We show that for spherical particles greater than ca. 5 µm, the differential scattering cross section is only weakly dependent on the real and imaginary parts of the refractive index ( $m=n+i\mathrm{\kappa <\#comment/>}$) when integrated over angle ranges near $37\pm <\#comment/>5^{\circ <\#comment/>}$and $115\pm <\#comment/>5^{\circ <\#comment/>}$, respectively. With this knowledge, we set up an arrangement that collects scattered light in the ranges $37\pm <\#comment/>5^{\circ <\#comment/>}$, $115\pm <\#comment/>5^{\circ <\#comment/>}$, and $80\pm <\#comment/>5^{\circ <\#comment/>}$. The weak functionality on refractive index for the first two angle ranges simplifies the inversion of scattering to the particle properties of diameter and the real and imaginary refractive indices. Our setup also uses a diamond-shaped incident beam profile that allows us to determine when a particle went through the exact center of the beam. Application of our setup to droplets of an absorbing liquid successfully determined the diameter and complex refractive index to accuracies ranging from a few to ten percent. Comparisons to simulated data derived from the Mie equations yielded similar results. 

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3. Rapid acquisition of broadband two-dimensional electronic spectra by continuous scanning with conventional delay lines

   https://doi.org/10.1364/OL.391360  

   Spencer, Austin_P; Chen, Lin_X (May 2020, Optics Letters)

   A passively phase-stable, broadband ( $\sim <\#comment/>7\mathrm{f}\mathrm{s}$, $><\#comment/>2000{\mathrm{c}\mathrm{m}}^{-<\#comment/>1}$) two-dimensional (2D) electronic spectroscopy apparatus that achieves rapid acquisition rates by continuously—rather than step-wise—scanning the Fourier-transform dimension is demonstrated for the first time, to the best of our knowledge. This is made possible through use of a partially common path interferometer design in which the coherence time $\mathrm{\tau <\#comment/>}$is sampled in a “rotating frame.” Rapid, continuous scanning of $\mathrm{\tau <\#comment/>}$increases the duty cycle of signal collection, rejects the majority of excitation pulse scatter, and enables the measurement of a complete 2D spectrum in 92 ms, which minimizes the influence of pulse intensity and delay fluctuations on the 2D spectrum. In practice, these improvements make possible the acquisition of hundreds of 2D spectra in tens of minutes, which opens the door to dense sampling of ultrafast relaxation dynamics and to generating extremely broadband 3D Fourier-transform spectra. 

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4. High-resolution and compact serpentine integrated grating spectrometer

   https://doi.org/10.1364/JOSAB.423968  

   Brand, Michael; Zhang, Bohan; Onural, Deniz; Al_Qubaisi, Kenaish; Popović, Miloš; Dostart, Nathan; Wagner, Kelvin (June 2021, Journal of the Optical Society of America B)

   Integrated astrophotonic spectrometers are integrated variants of conventional free-space spectrometers that offer significantly reduced size, weight, and cost and immunity to alignment errors, and can be readily integrated with other astrophotonic instruments such as nulling interferometers. Current integrated dispersive astrophotonic spectrometers are one-dimensional devices such as arrayed waveguide gratings or planar echelle gratings. These devices have been limited to ${10}^4$resolving powers and $<<\#comment/>1000$spectral bins due to having limited total optical delay paths and 1D detector array pixel densities. In this paper, we propose and demonstrate a high-resolution and compact astrophotonic serpentine integrated grating (SIG) spectrometer design based on a 2D dispersive serpentine optical phased array. The SIG device combines a 5.2 cm long folded delay line with grating couplers to create a large optical delay path along two dimensions in a compact integrated device footprint. Analogous to free-space crossed-dispersion high-resolution spectrometers, the SIG spectrometer maps spectral content to a 2D wavelength-beam-steered folded-raster emission pattern focused onto a 2D detector array. We demonstrate a SIG spectrometer with $\sim <\#comment/>100\mathrm{k}$resolving power and $\sim <\#comment/>6750$spectral bins, which are approximately an order of magnitude higher than previous integrated photonic designs that operate over a wide bandwidth, in a $0.4{\mathrm{m}\mathrm{m}}^2$footprint. We measure a Rayleigh resolution of $1.93\pm <\#comment/>0.07\mathrm{G}\mathrm{H}\mathrm{z}$and an operational bandwidth from 1540 nm to 1650 nm. Finally, we discuss refinements of the SIG spectrometer that improve its resolution, bandwidth, and throughput. These results show that SIG spectrometer technology provides a path towards miniaturized, high-resolution spectrometers for applications in astronomy and beyond. 

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5. Ultralow-threshold thin-film lithium niobate optical parametric oscillator

   https://doi.org/10.1364/OPTICA.418984  

   Lu, Juanjuan; Al_Sayem, Ayed; Gong, Zheng; Surya, Joshua_B; Zou, Chang-Ling; Tang, Hong_X (April 2021, Optica)

   Materials with strong second-order ( ${\mathrm{\chi <\#comment/>}}^{\left(2\right)}$) optical nonlinearity, especially lithium niobate, play a critical role in building optical parametric oscillators (OPOs). However, chip-scale integration of low-loss ${\mathrm{\chi <\#comment/>}}^{\left(2\right)}$materials remains challenging and limits the threshold power of on-chip ${\mathrm{\chi <\#comment/>}}^{\left(2\right)}$OPO. Here we report an on-chip lithium niobate optical parametric oscillator at the telecom wavelengths using a quasi-phase-matched, high-quality microring resonator, whose threshold power ( $\sim <\#comment/>30\text{µ<\#comment/>}\mathrm{W}$) is 400 times lower than that in previous ${\mathrm{\chi <\#comment/>}}^{\left(2\right)}$integrated photonics platforms. An on-chip power conversion efficiency of 11% is obtained from pump to signal and idler fields at a pump power of 93 µW. The OPO wavelength tuning is achieved by varying the pump frequency and chip temperature. With the lowest power threshold among all on-chip OPOs demonstrated so far, as well as advantages including high conversion efficiency, flexibility in quasi-phase-matching, and device scalability, the thin-film lithium niobate OPO opens new opportunities for chip-based tunable classical and quantum light sources and provides a potential platform for realizing photonic neural networks. 

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