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Title: Nonsequential double ionization of Ar in near-single-cycle laser pulses
Using the improved quantitative rescattering (QRS) model, we simulate the correlated two-electron momentum distributions (CMD) for nonsequential double ionization (NSDI) of Ar by near-single-cycle laser pulses with a wavelength of 750 nm at an intensity of 2.8 × 1014W/cm2. With the accurate cross sections obtained from fully quantum mechanical calculations for both electron impact excitation and electron impact ionization of Ar+, we unambiguously identify the contributions from recollision direct ionization (RDI) and recollision excitation with subsequent ionization (RESI). Our analysis reveals that RESI constitutes the main contribution to NSDI of Ar under the conditions considered here. The simulated results are directly compared with experimental measurements [Bergueset al.,Nat. Commun.3,813(2012)10.1038/ncomms1807] in which each NSDI event is tagged with the carrier-envelope phase (CEP). It is found that the overall pattern of both the CEP-resolved and the CEP-averaged CMDs measured in experiment are well reproduced by the QRS model, and the cross-shaped structure in the CEP-averaged CMD is attributed to the strong forward scattering of the recolliding electron as well as the depletion effect in tunneling ionization of the electron from an excited state of the parent ion.
Using the quantitative rescattering model, we simulate the correlated two-electron momentum distributions for nonsequential double ionization of helium by 800 nm laser pulses at intensities in the range of (2 − 15) × 1014W/cm2. The experimentally observed V-shaped structure at high intensities [Phys. Rev. Lett.99,263003(2007)10.1103/PhysRevLett.99.263003] is attributed to the strong forward scattering in laser-induced recollision excitation and the asymmetric momentum distribution of electrons that are tunneling-ionized from the excited states. The final-state electron repulsion also plays an important role in forming the V-shaped structure.
Within the framework of the improved quantitative rescattering (QRS) model, we simulate the correlated two-electron momentum distributions (CMDs) for nonsequential double ionization (NSDI) of Ar by elliptically polarized laser pulses with a wavelength of 788 nm at an intensity of 0.7 × 1014W/cm2for the ellipticities ranging from 0 to 0.3. Only the CMDs for recollision excitation with subsequent ionization (RESI) are calculated and the contribution from recollision direct ionization is neglected. According to the QRS model, the CMD for RESI can be factorized as a product of the parallel momentum distribution (PMD) for the first released electron after recollision and the PMD for the second electron ionized from an excited state of the parent ion. The PMD for the first electron is obtained from the laser-free differential cross sections for electron impact excitation of Ar+calculated using state-of-the-art many-electronR-matrix theory while that for the second electron is evaluated by solving the time-dependent Schrödinger equation. The results show that the CMDs for all the ellipticities considered here exhibit distinct anticorrelated back-to-back emission of the electrons along the major polarization direction, and the anticorrelation is more pronounced with increasing ellipticity. It is found that anticorrelation is attributed to the pattern of the PMD for the second electron ionized from the excited state that, in turn, is caused by the delayed recollision time with respect to the instant of the external field crossing. Our work shows that both the ionization potential of the excited parent ion and the laser intensity play important roles in the process.
We proposed the use of relative encircled power as a measure of focusing efficiency [Optica7,252(2020)OPTIC82334-253610.1364/OPTICA.388697]. The comment [Optica8,1009(2021)OPTIC82334-253610.1364/OPTICA.416017] has raised useful questions, which we address briefly here and provide some clarifications.
Park, Bo_Kyung; Han, Sang_M; Han, Sang_Eon(
, Optical Materials Express)
Two typographical corrections are made for our recently published paper [Opt. Mater. Express12(7),2529(2022)10.1364/OME.462592]. The results, discussion, and conclusion of the paper are unaffected.
Chen, Zhangjin, Liu, Fang, Wen, Hua, Morishita, Toru, Zatsarinny, Oleg, and Bartschat, Klaus.
"Nonsequential double ionization of Ar in near-single-cycle laser pulses". Optics Express 28 (15). Country unknown/Code not available: Optical Society of America. https://doi.org/10.1364/OE.398035.https://par.nsf.gov/biblio/10170945.
@article{osti_10170945,
place = {Country unknown/Code not available},
title = {Nonsequential double ionization of Ar in near-single-cycle laser pulses},
url = {https://par.nsf.gov/biblio/10170945},
DOI = {10.1364/OE.398035},
abstractNote = {Using the improved quantitative rescattering (QRS) model, we simulate the correlated two-electron momentum distributions (CMD) for nonsequential double ionization (NSDI) of Ar by near-single-cycle laser pulses with a wavelength of 750 nm at an intensity of 2.8 × 1014W/cm2. With the accurate cross sections obtained from fully quantum mechanical calculations for both electron impact excitation and electron impact ionization of Ar+, we unambiguously identify the contributions from recollision direct ionization (RDI) and recollision excitation with subsequent ionization (RESI). Our analysis reveals that RESI constitutes the main contribution to NSDI of Ar under the conditions considered here. The simulated results are directly compared with experimental measurements [Bergueset al.,Nat. Commun.3,813(2012)10.1038/ncomms1807] in which each NSDI event is tagged with the carrier-envelope phase (CEP). It is found that the overall pattern of both the CEP-resolved and the CEP-averaged CMDs measured in experiment are well reproduced by the QRS model, and the cross-shaped structure in the CEP-averaged CMD is attributed to the strong forward scattering of the recolliding electron as well as the depletion effect in tunneling ionization of the electron from an excited state of the parent ion.},
journal = {Optics Express},
volume = {28},
number = {15},
publisher = {Optical Society of America},
author = {Chen, Zhangjin and Liu, Fang and Wen, Hua and Morishita, Toru and Zatsarinny, Oleg and Bartschat, Klaus},
}
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