Thin-film lithium-niobate-on-insulator (LNOI) has emerged as a superior integrated-photonics platform for linear, nonlinear, and electro-optics. Here we combine quasi-phase-matching, dispersion engineering, and tight mode confinement to realize nonlinear parametric processes with both high efficiency and wide wavelength tunability. On a millimeter-long, Z-cut LNOI waveguide, we demonstrate efficient ( ) and highly tunable ( ) second-harmonic generation from 1530 to 1583 nm by type-0 quasi-phase-matching. Our technique is applicable to optical harmonic generation, quantum light sources, frequency conversion, and many other photonic information processes across visible to mid-IR spectral bands.
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Ultrafast 1 MHz vacuum-ultraviolet source via highly cascaded harmonic generation in negative-curvature hollow-core fibers
Vacuum-ultraviolet (VUV) light is critical for the study of molecules and materials, but the generation of femtosecond pulses in the VUV region at high repetition rates has proven difficult. Here we demonstrate the efficient generation of VUV light at megahertz repetition rates using highly cascaded four-wave mixing processes in a negative-curvature hollow-core fiber. Both even- and odd-order harmonics are generated up to the 15th harmonic (69 nm, 18.0 eV), with high energy resolution of . In contrast to direct high harmonic generation, this highly cascaded harmonic generation process requires lower peak intensity and therefore can operate at higher repetition rates, driven by a robust fiber-laser system in a compact setup. Additionally, we present numerical simulations that explore the fundamental capabilities and spatiotemporal dynamics of highly cascaded harmonic generation. This VUV source can enhance the capabilities of spectroscopies of molecular and quantum materials, such as photoionization mass spectrometry and time-, angle-, and spin-resolved photoemission.
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- Award ID(s):
- 1734006
- PAR ID:
- 10171146
- Publisher / Repository:
- Optical Society of America
- Date Published:
- Journal Name:
- Optica
- Volume:
- 7
- Issue:
- 7
- ISSN:
- 2334-2536
- Format(s):
- Medium: X Size: Article No. 832
- Size(s):
- Article No. 832
- Sponsoring Org:
- National Science Foundation
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