Light carries both spin angular momentum (SAM) and orbital angular momentum (OAM), which can be used as potential degrees of freedom for quantum information processing. Quantum emitters are ideal candidates towards on-chip control and manipulation of the full SAM–OAM state space. Here, we show coupling of a spin-polarized quantum emitter in a monolayer with the whispering gallery mode of a ring resonator. The cavity mode carries a transverse SAM of in the evanescent regions, with the sign depending on the orbital power flow direction of the light. By tailoring the cavity–emitter interaction, we couple the intrinsic spin state of the quantum emitter to the SAM and propagation direction of the cavity mode, which leads to spin–orbit locking and subsequent chiral single-photon emission. Furthermore, by engineering how light is scattered from the WGM, we create a high-order Bessel beam which opens up the possibility to generate optical vortex carrying OAM states.
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Effect of emitter orientation on the outcoupling efficiency of perovskite light-emitting diodes
Metal halide perovskite light-emitting diodes (PeLEDs) have experienced a rapid advancement in the last several years with the external quantum efficiencies (EQEs) reaching over 20%, comparable to the state-of-the-art organic LEDs and quantum dot LEDs. The photoluminescence quantum yields of perovskite films have also been approaching 100%. Therefore, the next step to improving the EQE of PeLEDs should be focused on boosting light extraction. In this Letter, we demonstrate the emitter dipole orientation as a key parameter in determining the outcoupling efficiency of PeLEDs. We find that the emitter has a slightly preferred orientation with the horizontal-to-vertical dipole ratio of 0.41:0.59, as compared to 0.33:0.67 in the isotropic case. A theoretical analysis predicts that a purely anisotropic perovskite emitter may result in a maximum EQE of 36%.
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- Award ID(s):
- 1807397
- PAR ID:
- 10185662
- Publisher / Repository:
- Optical Society of America
- Date Published:
- Journal Name:
- Optics Letters
- Volume:
- 45
- Issue:
- 17
- ISSN:
- 0146-9592; OPLEDP
- Format(s):
- Medium: X Size: Article No. 4786
- Size(s):
- Article No. 4786
- Sponsoring Org:
- National Science Foundation
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