Abstract A pulling motion of supercavitating plasmonic nanoparticle (NP) by a single plane wave has received attention for the fundamental physics and potential applications in various fields ( e.g. , bio-applications, nanofabrication, and nanorobotics). Here, the supercavitating NP depicts a state where a nanobubble encapsulates the NP, which can be formed via the photo-thermal heating process in a liquid. In this letter, we theoretically study the optical force on a supercavitating titanium nitride (TiN) NP by a single plane wave at near-infrared wavelengths to explore optical conditions that can potentially initiate the backward motion of the NP against the wave-propagating direction. An analysis with vector spherical harmonics is used to quantify the optical force on the NP efficiently. Next, the vector field line of the optical force is introduced to visualize the light-driven motion of the NP in a nanobubble. Finally, we characterize the vector field lines at various optical conditions ( e.g. , various sizes of NP and nanobubble, and wavelength), and we find a suitable window of the optical state which can potentially activate the backward motion of the supercavitating TiN NP. 
                        more » 
                        « less   
                    
                            
                            Long-distance optical pulling of nanoparticle in a low index cavity using a single plane wave
                        
                    
    
            Optical pulling force (OPF) can make a nanoparticle (NP) move against the propagation direction of the incident light. Long-distance optical pulling is highly desired for nano-object manipulation, but its realization remains challenging. We propose an NP-in-cavity structure that can be pulled by a single plane wave to travel long distances when the spherical cavity wrapping the NP has a refractive index lower than the medium. An electromagnetic multipole analysis shows that NPs made of many common materials can receive the OPF inside a lower index cavity. Using a silica-Au core-shell NP that is encapsulated by a plasmonic nanobubble, we experimentally demonstrate that a single laser can pull the Au NP-in-nanobubble structure for ~0.1 mm. These results may lead to practical applications that can use the optical pulling of NP, such as optically driven nanostructure assembly and nanoswimmers. 
        more » 
        « less   
        
    
                            - Award ID(s):
- 1706039
- PAR ID:
- 10189601
- Date Published:
- Journal Name:
- Science Advances
- Volume:
- 6
- Issue:
- 21
- ISSN:
- 2375-2548
- Page Range / eLocation ID:
- eaaz3646
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
- 
            
- 
            Optical manipulation of nanoparticles (NPs) in liquid has garnered increasing interest for various applications, ranging from biological systems to nanofabrication. A plane wave as an optical source has recently been shown to be capable of pushing or pulling an NP when the NP is encapsulated by a nanobubble (NB) in water. However, the lack of an accurate model to describe the optical force on NP-in-NB systems hinders a comprehensive understanding of NP motion mechanisms. In this study, we present an analytical model using vector spherical harmonics to accurately capture the optical force and the resultant trajectory of an NP in an NB. We test the developed model using a solid Au NP as an example. By visualizing the vector field line of the optical force, we reveal the possible moving paths of the NP in the NB. This study can provide valuable insights for designing experiments to manipulate supercaviting NPs using plane waves.more » « less
- 
            Abstract Directed high-speed motion of nanoscale objects in fluids can have a wide range of applications like molecular machinery, nano robotics, and material assembly. Here, we report ballistic plasmonic Au nanoparticle (NP) swimmers with unprecedented speeds (~336,000 μm s−1) realized by not only optical pushing but also pulling forces from a single Gaussian laser beam. Both the optical pulling and high speeds are made possible by a unique NP-laser interaction. The Au NP excited by the laser at the surface plasmon resonance peak can generate a nanoscale bubble, which can encapsulate the NP (i.e., supercavitation) to create a virtually frictionless environment for it to move, like the Leidenfrost effect. Certain NP-in-bubble configurations can lead to the optical pulling of NP against the photon stream. The demonstrated ultra-fast, light-driven NP movement may benefit a wide range of nano- and bio-applications and provide new insights to the field of optical pulling force.more » « less
- 
            Newly, there has been significant research interest in the exact solution of the AC optimal power flow (AC-OPF) problem. A semideflnite relaxation solves many OPF problems globally. However, the real problem exists in which the semidefinite relaxation fails to yield the global solution. The appropriation of relaxation for AC-OPF depends on the success or unfulflllment of the SDP relaxation. This paper demonstrates a quadratic AC-OPF problem with a single negative eigenvalue in objective function subject to linear and conic constraints. The proposed solution method for AC-OPF model covers the classical AC economic dispatch problem that is known to be NP-hard. In this paper, by combining successive linear conic optimization (SLCO), convex relaxation and line search technique, we present a global algorithm for AC-OPF which can locate a globally optimal solution to the underlying AC-OPF within given tolerance of global optimum solution via solving linear conic optimization problems. The proposed algorithm is examined on modified IEEE 6-bus test system. The promising numerical results are described.more » « less
- 
            We propose to simulate bosonic pair creation using large arrays of long-lived dipoles with multilevel internal structure coupled to an undriven optical cavity. Entanglement between the atoms, generated by the exchange of virtual photons through a common cavity mode, grows exponentially fast and is described by two-mode squeezing (TMS) of effective bosonic quadratures. The mapping between an effective bosonic model and the natural spin description of the dipoles allows us to realize the analog of optical homodyne measurements via straightforward global rotations and population measurements of the electronic states, and we propose to exploit this for quantum-enhanced sensing of an optical phase (common and differential between two ensembles). We discuss a specific implementation based on Sr atoms and show that our sensing protocol is robust to sources of decoherence intrinsic to cavity platforms. Our proposal can open unique opportunities for the observation of continuous variable entanglement in atomic systems and associated applications in next-generation optical atomic clocks.more » « less
 An official website of the United States government
An official website of the United States government 
				
			 
					 
					
 
                                    