Optical manipulation of nanoparticles (NPs) in liquid has garnered increasing interest for various applications, ranging from biological systems to nanofabrication. A plane wave as an optical source has recently been shown to be capable of pushing or pulling an NP when the NP is encapsulated by a nanobubble (NB) in water. However, the lack of an accurate model to describe the optical force on NP-in-NB systems hinders a comprehensive understanding of NP motion mechanisms. In this study, we present an analytical model using vector spherical harmonics to accurately capture the optical force and the resultant trajectory of an NP in an NB. We test the developed model using a solid Au NP as an example. By visualizing the vector field line of the optical force, we reveal the possible moving paths of the NP in the NB. This study can provide valuable insights for designing experiments to manipulate supercaviting NPs using plane waves.
Long-distance optical pulling of nanoparticle in a low index cavity using a single plane wave
Optical pulling force (OPF) can make a nanoparticle (NP) move against the propagation direction of the incident light. Long-distance optical pulling is highly desired for nano-object manipulation, but its realization remains challenging. We propose an NP-in-cavity structure that can be pulled by a single plane wave to travel long distances when the spherical cavity wrapping the NP has a refractive index lower than the medium. An electromagnetic multipole analysis shows that NPs made of many common materials can receive the OPF inside a lower index cavity. Using a silica-Au core-shell NP that is encapsulated by a plasmonic nanobubble, we experimentally demonstrate that a single laser can pull the Au NP-in-nanobubble structure for ~0.1 mm. These results may lead to practical applications that can use the optical pulling of NP, such as optically driven nanostructure assembly and nanoswimmers.
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- Award ID(s):
- 1706039
- NSF-PAR ID:
- 10189601
- Date Published:
- Journal Name:
- Science Advances
- Volume:
- 6
- Issue:
- 21
- ISSN:
- 2375-2548
- Page Range / eLocation ID:
- eaaz3646
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
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Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1126/sciadv.aaz3646
