skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.

Attention:

The NSF Public Access Repository (PAR) system and access will be unavailable from 10:00 PM ET on Friday, February 6 until 10:00 AM ET on Saturday, February 7 due to maintenance. We apologize for the inconvenience.

Explore Research Products in the PAR
It may take a few hours for recently added research products to appear in PAR search results.


Title: Unlocking the decoding of unknown magnetic nanobarcode signatures
Magnetic nanowires (MNWs) rank among the most promising multifunctional magnetic nanomaterials for nanobarcoding applications owing to their safety, nontoxicity, and remote decoding using a single magnetic excitation source. Until recently, coercivity and saturation magnetization have been proposed as encoding parameters. Herein, backward remanence magnetization (BRM) is used to decode unknown remanence spectra of MNWs-based nanobarcodes. A simple and fast expectation algorithm is proposed to decode the unknown remanence spectra with a success rate of 86% even though the MNWs have similar coercivities, which cannot be accomplished by other decoding schemes. Our experimental approach and analytical analysis open a promising direction towards reliably decoding magnetic nanobarcodes to expand their capabilities for security and labeling applications.  more » « less
Award ID(s):
1642268
PAR ID:
10209707
Author(s) / Creator(s):
;
Date Published:
Journal Name:
Nanoscale Advances
ISSN:
2516-0230
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. ; ; (, AIP Advances)
    Magnetic properties such as coercivity, remanence and saturation magnetization will determine the area enclosed by the hysteresis loop of a magnetic material, which also represents magnetic heating. Nanowarming of cryopreserved organs is a new application for magnetic heating using nanoparticles. In this paper, isolated Ni MNW of different sizes and shapes are studied via micromagnetic simulation to explore the optimization of heating using individual MNW. Ellipsoidal MNWs with small (30nm) diameters turn out to be most promising in heating ability due to their large hysteresis area and their potential to distribute uniformly in an organ that is being heated. In addition to optimized heating, a special switching pattern of magnetic moment was also observed for cylindrical large (200nm) MNW. This special switching pattern can trigger applications such as quantum computing. 
    more » « less
  2. ; ; ; (, Scientific Reports)
    null (Ed.)
    Abstract Magnetic nanoparticles have been proposed as contact-free minimal-background nanobarcodes, and yet it has been difficult to rapidly and reliably decode them in an assembly. Here, high aspect ratio nanoparticles, or magnetic nanowires (MNWs), are characterized using first-order reversal curves (FORC) to investigate quantitative decoding. We have synthesized four types of nanowires (differing in diameter) that might be used for barcoding, and identified four possible “signature” functions that might be used to quickly distinguish them. To test this, we have measured the signatures of several combination samples containing two or four different MNW types, and fit them to linear combinations of the individual type signatures to determine the volume ratios of the types. We find that the signature which determines the ratios most accurately involves only the slope of each FORC at its reversal field, which requires only 2–4 data points per FORC curve, reducing the measurement time by a factor of 10 to 50 compared to measuring the full FORC. 
    more » « less
  3. ; (, RSC Advances)
    null (Ed.)
    The unmet demand for cheap, accurate, and fast multiplexing of biomarkers has urged nanobiotechnology to prioritize the invention of new biomarkers that make feasible the remote detection, identification, and quantification of biological units, such as regenerative tissues. Here, we introduce a novel approach that highlights magnetic nanowires (MNWs) with such capabilities. This method employs the stable magnetization states of MNWs as a unique characteristic that can be realized by projecting the MNWs' switching field on the backward field ( P Hb ), also known as the irreversible switching field. Experimentally, several types of MNWs were directly synthesized inside polycarbonate tissues and their P Hb characteristics were measured and analyzed. Our results show that the P Hb gives an excellent identification and quantification characteristic for demultiplexing MNWs embedded in these tissues. Furthermore, this method significantly improves the characterization speed by a factor of 50×–100× that makes it superior to the current state of the art that ceased the progression of magnetic nanoparticles in multiplexing/demultiplexing applications. 
    more » « less
  4. ; ; (, Proceedings of the International Ocean Discovery Program Expedition reports)
    We measured the natural remanent magnetization (NRM) and rock magnetic properties of 57 sediment samples and 38 basalt samples from Tūranganui Knoll on the Hikurangi Plateau collected at Site U1526 during International Ocean Discovery Program Expedition 375. NRM was measured on all samples before and after either progressive alternating field or thermal demagnetization. Principal component analysis was conducted to provide estimates of the characteristic remanent magnetization direction. Rock magnetic observations include measurements on select samples of the bulk magnetic susceptibility, susceptibility versus heating for Curie temperature assessment, magnetic hysteresis, backfield for coercivity of remanence determinations, isothermal remanent magnetization, and first-order reversal curves. 
    more » « less
  5. ; ; ; ; (, Meteoritics & Planetary Science)
    Abstract We evaluate the relationship between the intensity of remanent magnetization andfO2in natural and synthetic Mars meteorites. The olivine‐phyric shergottite meteorite Yamato 980459 (Y‐980459) and a sulfur‐free synthetic analog (Y‐98*) of identical major element composition were analyzed to explore the rock magnetic and remanence properties of a basalt crystallized from a primitive melt, and to explore the role of magmatic and alteration environmentfO2on Mars crustal anomalies. The reducing conditions under which Y‐980459 is estimated to have formed (QFM‐2.5; Shearer et al. 2006) were replicated during the synthesis of Y‐98*. Y‐980459 contains pyrrhotite and chromite. Chromite is the only magnetic phase in Y‐98*. The remanence‐carrying capacity of Y‐980459 is comparable to other shergottites that formed in thefO2range of QFM‐3 to QFM‐1. The remanence‐carrying capacity of these lowfO2basalts is 1–2 orders of magnitude too weak to account for the intense crustal anomalies observed in Mars's southern cratered highlands. Moderately oxidizing conditions of >QFM‐1, which are more commonly observed in nakhlites and Noachian breccias, are key to generating either a primary igneous assemblage or secondary alteration assemblage capable of acquiring an intense remanent magnetization, regardless of the basalt character or thermal history. This suggests that if igneous rocks are responsible for the intensely magnetized crust, these oxidizing conditions must have existed in the magmatic plumbing systems of early Mars or must have existed in the crust during secondary processes that led to acquisition of a chemical remanent magnetization. 
    more » « less
  • Citation Formats
  • MLA
  • APA
  • Chicago
  • BibTeX
  • Text Encoded Conversion
  • XML
  • Save / Share this Record
  • Send to Email