Abstract The sustained interest in investigating magnetism in the 2D limit of insulating antiferromagnets is driven by the possibilities of discovering, or engineering, novel magnetic phases through layer stacking. However, due to the difficulty of directly measuring magnetic interactions in 2D antiferromagnets, it is not yet understood howintralayer magnetic interactions ininsulating, strongly correlated, materials can be modified through layer proximity. Herein, the impact of reduced dimensionality in the model van der Waals antiferromagnet NiPS3is explored by measuring electronic excitations in exfoliated samples using Resonant Inelastic X‐ray Scattering (RIXS). The resulting spectra shows systematic broadening of NiS6multiplet excitations with decreasing layer count from bulk down to three atomic layers (3L). It is shown that these trends originate from a decrease in transition metal‐ligand and ligand–ligand hopping integrals, and by charge‐transfer energy evolving from Δ = 0.83 eV in the bulk to 0.37 eV in 3L NiPS3. Relevant intralayer magnetic exchange integrals computed from the electronic parameters exhibit a decrease in the average interaction strength with thickness. This study underscores the influence ofinterlayer electronic interactions onintralayer ones in insulating magnets, indicating that magnetic Hamiltonians in few‐layer insulating magnets can greatly deviate from their bulk counterparts. 
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                            Architectural Archipelagos: Technical Debt in Long-Lived Software Research Platforms
                        
                    
    
            This paper identifies a model of software evolution that is prevalent in large, long-lived academic research tool suites (3L-ARTS). This model results in an "archipelago" of related but haphazardly organized architectural "islands", and inherently induces technical debt. We illustrate the archipelago model with examples from two 3L-ARTS archipelagos identified in literature. 
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                            - Award ID(s):
- 1823354
- PAR ID:
- 10293488
- Editor(s):
- Chatzigeorgiou, Alexander; Seaman, Carolyn
- Date Published:
- Journal Name:
- 2021 IEEE/ACM International Conference on Technical Debt (TechDebt)
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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