Nonlinear photocurrent in time-reversal invariant noncentrosymmetric systems such as ferroelectric semimetals sparked tremendous interest of utilizing nonlinear optics to characterize condensed matter with exotic phases. Here we provide a microscopic theory of two types of second-order nonlinear direct photocurrents, magnetic shift photocurrent (MSC) and magnetic injection photocurrent (MIC), as the counterparts of normal shift current (NSC) and normal injection current (NIC) in time-reversal symmetry and inversion symmetry broken systems. We show that MSC is mainly governed by shift vector and interband Berry curvature, and MIC is dominated by absorption strength and asymmetry of the group velocity difference at time-reversedmore »
This content will become publicly available on December 3, 2022
- Award ID(s):
- 1734011
- Publication Date:
- NSF-PAR ID:
- 10326562
- Journal Name:
- Science
- Volume:
- 374
- Issue:
- 6572
- Page Range or eLocation-ID:
- 1242 to 1247
- ISSN:
- 0036-8075
- Sponsoring Org:
- National Science Foundation
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