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1. Thermal-light heterodyne spectroscopy with frequency comb calibration

   https://doi.org/10.1364/OPTICA.440389  

   Fredrick, Connor ; Olsen, Freja ; Terrien, Ryan ; Mahadevan, Suvrath ; Quinlan, Franklyn ; Diddams, Scott A. ( February 2022 , Optica)

   Precision laser spectroscopy is key to many developments in atomic and molecular physics and the advancement of related technologies such as atomic clocks and sensors. However, in important spectroscopic scenarios, such as astronomy and remote sensing, the light is of thermal origin, and interferometric or diffractive spectrometers typically replace laser spectroscopy. In this work, we employ laser-based heterodyne radiometry to measure incoherent light sources in the near-infrared and introduce techniques for absolute frequency calibration with a laser frequency comb. Measuring the solar continuum, we obtain a signal-to-noise ratio that matches the fundamental quantum-limited prediction given by the thermal photon distribution and our system’s efficiency, bandwidth, and averaging time. With resolving power$R\sim <\#comment/>{10}^6$, we determine the center frequency of an iron line in the solar spectrum to sub-MHz absolute frequency uncertainty in under 10 min, a fractional precision 1/4000 the linewidth. Additionally, we propose concepts that take advantage of refractive beam shaping to decrease the effects of pointing instabilities by$100\times <\#comment/>$, and of frequency comb multiplexing to increase data acquisition rates and spectral bandwidths by comparable factors. Taken together, our work brings the power of telecommunications photonics and the precision of frequency comb metrology to laser heterodyne radiometry, with implications for solar and astronomical spectroscopy, remote sensing, and precise Doppler velocimetry.

    

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2. Passive frequency comb generation at radiofrequency for ranging applications

   https://doi.org/10.1038/s41467-024-46940-2  

   Hussein, Hussein M. E. ; Kim, Seunghwi ; Rinaldi, Matteo ; Alù, Andrea ; Cassella, Cristian ( April 2024 , Nature Communications)

   Optical frequency combs, featuring evenly spaced spectral lines, have been extensively studied and applied to metrology, signal processing, and sensing. Recently, frequency comb generation has been also extended to MHz frequencies by harnessing nonlinearities in microelectromechanical membranes. However, the generation of frequency combs at radio frequencies (RF) has been less explored, together with their potential application in wireless technologies. In this work, we demonstrate an RF system able to wirelessly and passively generate frequency combs. This circuit, which we name quasi-harmonic tag (qHT), offers a battery-free solution for far-field ranging of unmanned vehicles (UVs) in GPS-denied settings, and it enables a strong immunity to multipath interference, providing better accuracy than other RF approaches to far-field ranging. Here, we discuss the principle of operation, design, implementation, and performance of qHTs used to remotely measure the azimuthal distance of a UV flying in an uncontrolled electromagnetic environment. We show that qHTs can wirelessly generate frequency combs with μWatt-levels of incident power by leveraging the nonlinear interaction between an RF parametric oscillator and a high quality factor piezoelectric microacoustic resonator. Our technique for frequency comb generation opens new avenues for a wide range of RF applications beyond ranging, including timing, computing and sensing.

    

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3. Room temperature terahertz semiconductor frequency comb

   https://doi.org/10.1038/s41467-019-10395-7  

   Lu, Quanyong ; Wang, Feihu ; Wu, Donghai ; Slivken, Steven ; Razeghi, Manijeh ( June 2019 , Nature Communications)

   A terahertz (THz) frequency comb capable of high-resolution measurement will significantly advance THz technology application in spectroscopy, metrology and sensing. The recently developed cryogenic-cooled THz quantum cascade laser (QCL) comb has exhibited great potentials with high power and broadband spectrum. Here, we report a room temperature THz harmonic frequency comb in 2.2 to 3.3 THz based on difference-frequency generation from a mid-IR QCL. The THz comb is intracavity generated via down-converting a mid-IR comb with an integrated mid-IR single mode based on distributed-feedback grating without using external optical elements. The grating Bragg wavelength is largely detuned from the gain peak to suppress the grating dispersion and support the comb operation in the high gain spectral range. Multiheterodyne spectroscopy with multiple equally spaced lines by beating it with a reference Fabry-Pérot comb confirms the THz comb operation. This type of THz comb will find applications to room temperature chip-based THz spectroscopy.

    

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4. Nonlocal subpicosecond delay metrology using spectral quantum interference

   https://doi.org/10.1364/OPTICA.458565  

   Seshadri, Suparna ; Lingaraju, Navin ; Lu, Hsuan-Hao ; Imany, Poolad ; Leaird, Daniel E. ; Weiner, Andrew M. ( November 2022 , Optica)

   Precise knowledge of position and timing information is critical to support elementary protocols such as entanglement swapping on quantum networks. While approaches have been devised to use quantum light for such metrology, they largely rely on time-of-flight (ToF) measurements with single-photon detectors and, therefore, are limited to picosecond-scale resolution owing to detector jitter. In this work, we demonstrate an approach to distributed sensing that leverages phase modulation to map changes in the spectral phase to coincidence probability, thereby overcoming the limits imposed by single-photon detection. By extracting information about the joint biphoton phase, we measure a generalized delay—the difference in signal–idler arrival, relative to local radio frequency (RF) phase modulation. For nonlocal ranging measurements, we achieve ($2\mathrm{\sigma <\#comment/>}$) precision of$\pm <\#comment/>0.04\mathrm{p}\mathrm{s}$and for measurements of the relative RF phase, ($2\mathrm{\sigma <\#comment/>}$) precision of$\pm <\#comment/>{0.7}^{\circ <\#comment/>}$. We complement this fine timing information with ToF data from single-photon time-tagging to demonstrate absolute measurement of time delay. By relying on off-the-shelf telecommunications equipment and standard quantum resources, this approach has the potential to reduce overhead in practical quantum networks.

    

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5. Entanglement-enhanced dual-comb spectroscopy

   https://doi.org/10.1038/s41534-023-00758-w  

   Shi, Haowei ; Chen, Zaijun ; Fraser, Scott E. ; Yu, Mengjie ; Zhang, Zheshen ; Zhuang, Quntao ( September 2023 , npj Quantum Information)

   Dual-comb interferometry harnesses the interference of two laser frequency combs to provide unprecedented capability in spectroscopy applications. In the past decade, the state-of-the-art systems have reached a point where the signal-to-noise ratio per unit acquisition time is fundamentally limited by shot noise from vacuum fluctuations. To address the issue, we propose an entanglement-enhanced dual-comb spectroscopy protocol that leverages quantum resources to significantly improve the signal-to-noise ratio performance. To analyze the performance of real systems, we develop a quantum model of dual-comb spectroscopy that takes practical noises into consideration. Based on this model, we propose quantum combs with side-band entanglement around each comb lines to suppress the shot noise in heterodyne detection. Our results show significant quantum advantages in the uW to mW power range, making this technique particularly attractive for biological and chemical sensing applications. Furthermore, the quantum comb can be engineered using nonlinear optics and promises near-term experimentation.

    

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