Ultracold molecules have been proposed as a candidate platform for quantum science and precision measurement because of their rich internal structures and interactions. Direct laser-cooling promises to be a rapid and efficient way to bring molecules to ultracold temperatures. However, for trapped molecules, laser-cooling to the quantum motional ground state remains an outstanding challenge. A technique capable of reaching the motional ground state is Raman sideband cooling, first demonstrated in trapped ions and atoms. Here we demonstrate Raman sideband cooling of CaF molecules trapped in an optical tweezer array. Our protocol does not rely on high magnetic fields and preserves the purity of molecular internal states. We measure a high ground-state fraction and achieve low motional entropy per particle. The low temperatures we obtain could enable longer coherence times and higher-fidelity molecular qubit gates, desirable for quantum information processing and quantum simulation. With further improvements, Raman sideband cooling will also provide a route to quantum degeneracy of large molecular samples, which could be extendable to polyatomic molecular species.
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Coherently Coupled Mechanical Oscillators in the Quantum Regime
Coupled harmonic oscillators are ubiquitous in physics and play a prominent role in quantum science. They are a cornerstone of quantum mechanics and quantum field theory, where second quantization relies on harmonic oscillator operators to create and annihilate particles. Descriptions of quantum tunneling, beamsplitters, coupled potential wells, "hopping terms", decoherence and many other phenomena rely on coupled harmonic oscillators. Despite their prominence, only a few experimental systems have demonstrated direct coupling between separate harmonic oscillators; these demonstrations lacked the capability for high-fidelity quantum control. Here, we realize coherent exchange of single motional quanta between harmonic oscillators -- in this case, spectrally separated harmonic modes of motion of a trapped ion crystal where the timing, strength, and phase of the coupling are controlled through the application of an oscillating electric field with suitable spatial variation. We demonstrate high-fidelity quantum state transfer, entanglement of motional modes, and Hong-Ou-Mandel-type interference. We also project a harmonic oscillator into its ground state by measurement and preserve that state during repetitions of the projective measurement, an important prerequisite for non-destructive syndrome measurement in continuous-variable quantum error correction. Controllable coupling between harmonic oscillators has potential applications in quantum information processing with continuous variables, quantum simulation, and precision measurements. It can also enable cooling and quantum logic spectroscopy involving motional modes of trapped ions that are not directly accessible.
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- Award ID(s):
- 2016244
- NSF-PAR ID:
- 10340299
- Date Published:
- Journal Name:
- ArXivorg
- ISSN:
- 2331-8422
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
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Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.21203/rs.3.rs-1774123/v1
