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Title: Second order Zeeman interaction and ferroquadrupolar order in TmVO4
Abstract TmVO 4 exhibits ferroquadrupolar order of the Tm 4f electronic orbitals at low temperatures, and is a model system for Ising nematicity. A magnetic field oriented along the c -axis constitutes a transverse effective field for the quadrupolar order parameter, continuously tuning the system to a quantum phase transition as the field is increased from zero. In contrast, in-plane magnetic fields couple to the order parameter only at second order, such that orienting along the primary axes of the quadrupole order results in an effective longitudinal field, whereas orienting at 45 degrees results in a second effective transverse field. Not only do in-plane fields engender a marked in-plane anisotropy of the critical magnetic and quadrupole fluctuations above the ferroquadrupolar ordering temperature, but in-plane transverse fields initially enhance the ferroquadrupolar order, before eventually suppressing it, an effect that we attribute to admixing of the higher crystalline electric field levels.  more » « less
Award ID(s):
1807889 1852581
PAR ID:
10341538
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ;
Date Published:
Journal Name:
npj Quantum Materials
Volume:
7
Issue:
1
ISSN:
2397-4648
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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