More Like this

1. Electrostatic focusing of cold and heavy molecules for the ACME electron EDM search

   https://doi.org/10.1088/1367-2630/ac8014  

   Wu, X.; Hu, P.; Han, Z.; Ang, D. G.; Meisenhelder, C.; Gabrielse, G.; Doyle, J. M.; DeMille, D. (August 2022, New Journal of Physics)

   Abstract The current best upper limit for electron electric dipole moment (EDM), |d_e| < 1.1 × 10⁻²⁹e cm (90% confidence), was set by the ACME Collaboration in 2018. The ACME experiment uses a spin-precession measurement in a cold beam of thorium monoxide (ThO) molecules to detectd_e. An improvement in statistical uncertainty would be possible with more efficient use of molecules from the cryogenic buffer gas beam source. Here, we demonstrate electrostatic focusing of the ThO beam with a hexapole lens. This results in a factor of 16 enhancement in the molecular flux detectable downstream, in a beamline similar to that built for the next generation of ACME. We also demonstrate an upgraded rotational cooling scheme that increases the ground state population by 3.5 times compared to no cooling, consistent with expectations and a factor of 1.4 larger than previously in ACME. When combined with other demonstrated improvements, we project over an order of magnitude improvement in statistical sensitivity for the next generation ACME electron EDM search. 

   more » « less
2. The metastable Q ³ Δ ₂ state of ThO: a new resource for the ACME electron EDM search

   https://doi.org/10.1088/1367-2630/ab6a3a  

   Wu, X.; Han, Z.; Chow, J.; Ang, D. G.; Meisenhelder, C.; Panda, C. D.; West, E. P.; Gabrielse, G.; Doyle, J. M.; DeMille, D. (February 2020, New Journal of Physics)

   Abstract The best upper limit for the electron electric dipole moment was recently set by the ACME collaboration. This experiment measures an electron spin-precession in a cold beam of ThO molecules in their metastable $H{(}^3{\mathrm{\Delta }}_1)$state. Improvement in the statistical and systematic uncertainties is possible with more efficient use of molecules from the source and better magnetometry in the experiment, respectively. Here, we report measurements of several relevant properties of the long-lived $Q{(}^3{\mathrm{\Delta }}_2)$state of ThO, and show that this state is a very useful resource for both these purposes. TheQstate lifetime is long enough that its decay during the time of flight in the ACME beam experiment is negligible. The large electric dipole moment measured for theQstate, giving rise to a large linear Stark shift, is ideal for an electrostatic lens that increases the fraction of molecules detected downstream. The measured magnetic moment of theQstate is also large enough to be used as a sensitive co-magnetometer in ACME. Finally, we show that theQstate has a large transition dipole moment to the $C{(}^1{\mathrm{\Pi }}_1)$state, which allows for efficient population transfer between the ground state $X{(}^1{\mathrm{\Sigma }}^{+})$and theQstate via $X-C-Q$Stimulated Raman Adiabatic Passage (STIRAP). We demonstrate 90 % STIRAP transfer efficiency. In the course of these measurements, we also determine the magnetic moment ofCstate, the $X\to C$transition dipole moment, and branching ratios of decays from theCstate. 

   more » « less
3. Radio Scattering Horizons for Galactic and Extragalactic Transients

   https://doi.org/10.3847/1538-4357/ac75ba  

   Ocker, Stella Koch; Cordes, James M.; Chatterjee, Shami; Gorsuch, Miranda R. (July 2022, The Astrophysical Journal)

   Abstract Radio wave scattering can cause severe reductions in detection sensitivity for surveys of Galactic and extragalactic fast (∼ms duration) transients. While Galactic sources like pulsars undergo scattering in the Milky Way interstellar medium (ISM), extragalactic fast radio bursts (FRBs) can also experience scattering in their host galaxies and other galaxies intervening in their lines of sight. We assess Galactic and extragalactic scattering horizons for fast radio transients using a combination of NE2001 to model the dispersion measure and scattering time (τ) contributed by the Galactic disk, and independently constructed electron density models for the Galactic halo and other galaxies’ ISMs and halos that account for different galaxy morphologies, masses, densities, and strengths of turbulence. For source redshifts 0.5 ≤z_s≤ 1, an all-sky, isotropic FRB population has simulated values ofτ(1 GHz) ranging from ∼1μs to ∼2 ms (90% confidence, observer frame) that are dominated by host galaxies, althoughτcan be ≫2 ms at low Galactic latitudes. A population atz_s= 5 has 0.01 ≲τ≲ 300 ms at 1 GHz (90% confidence), dominated by intervening galaxies. About 20% of these high-redshift FRBs are predicted to haveτ> 5 ms at 1 GHz (observer frame), and ≳40% of FRBs betweenz_s∼ 0.5–5 haveτ≳ 1 ms forν≤ 800 MHz. Our scattering predictions may be conservative if scattering from circumsource environments is significant, which is possible under specific conditions. The percentage of FRBs selected against from scattering could also be substantially larger than we predict if circumgalactic turbulence causes more small-scale (≪1 au) density fluctuations than observed from nearby halos. 

   more » « less
4. Test of light-lepton universality in τ decays with the Belle II experiment

   https://doi.org/10.1007/JHEP08(2024)205  

   Adachi, I; Adamczyk, K; Aggarwal, L; Aihara, H; Akopov, N; Aloisio, A; Anh_Ky, N; Asner, D M; Atmacan, H; Aushev, V; et al (August 2024, Journal of High Energy Physics)

   A<sc>bstract</sc> We present a measurement of the ratio$$ {R}_{\mu }=\mathcal{B}\left({\tau}^{-}\to {\mu}^{-}{\overline{\nu}}_{\mu }{\nu}_{\tau}\right)/\mathcal{B}\left({\tau}^{-}\to {e}^{-}{\overline{\nu}}_e{\nu}_{\tau}\right) $$ $R_{\mu }=B\left({\tau }^{-}\to {\mu }^{-}{\overline{\nu }}_{\mu }{\nu }_{\tau }\right)/B\left({\tau }^{-}\to e^{-}{\overline{\nu }}_e{\nu }_{\tau }\right)$of branching fractions$$ \mathcal{B} $$ $B$of theτlepton decaying to muons or electrons using data collected with the Belle II detector at the SuperKEKBe⁺e⁻collider. The sample has an integrated luminosity of 362 ± 2 fb⁻¹at a centre-of-mass energy of 10.58 GeV. Using an optimised event selection, a binned maximum likelihood fit is performed using the momentum spectra of the electron and muon candidates. The result,R_μ= 0.9675 ± 0.0007 ± 0.0036, where the first uncertainty is statistical and the second is systematic, is the most precise to date. It provides a stringent test of the light-lepton universality, translating to a ratio of the couplings of the muon and electron to theWboson inτdecays of 0.9974 ± 0.0019, in agreement with the standard model expectation of unity. 

   more » « less
5. Unraveling the Solid-State Photoreactivity of Carbonylbis(4,1-Phenylene)dicarbonazidate with Laser Flash Photolysis

   https://doi.org/10.1021/acs.jpca.3c04867  

   Ahmed, Noha; Kavikarage, Janaka P.; Judkins, DeAnte F.; Mendis, W. Dinindu; Merugu, Rajkumar; Krause, Jeanette A.; Ault, Bruce S.; Gudmundsdottir, Anna D. (November 2023, The Journal of Physical Chemistry A)

   Solid-state photoreactions are generally controlled by the rigid and ordered nature of crystals. Herein, the solution and solid-state photoreactivities of carbonylbis(4,1-phenylene)dicarbonazidate (1) were investigated to elucidate the solid-state reaction mechanism. Irradiation of 1 in methanol yielded primarily the corresponding amine, whereas irradiation in the solid state gave a mixture of photoproducts. Laser flash photolysis in methanol showed the formation of the triplet ketone (TK) of 1 (τ ∼ 99 ns), which decayed to triplet nitrene 31N (τ ∼ 464 ns), as assigned by comparison to its calculated spectrum. Laser flash photolysis of a nanocrystalline suspension and diffuse reflectance laser flash photolysis also revealed the formation of TK of 1 (τ ∼ 106 ns) and 31N (τ ∼ 806 ns). Electron spin resonance spectroscopy and phosphorescence measurements further verified the formation of 31N and the TK of 1, respectively. In methanol, 31N decays by H atom abstraction. However, in the solid state, 31N is sufficiently long lived to thermally populate its singlet configuration (11N). Insertion of 11N into the phenyl ring to produce oxazolone competes with 31N cleavage to form a radical pair. Notably, 1 did not exhibit photodynamic behavior, likely because the photoreaction occurs only on the crystal surfaces. 

   more » « less