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1. High-pressure induced Weyl semimetal phase in 2D Tellurium

   https://doi.org/10.1038/s42005-023-01460-1  

   Niu, Chang ; Zhang, Zhuocheng ; Graf, David ; Lee, Seungjun ; Wang, Mingyi ; Wu, Wenzhuo ; Low, Tony ; Ye, Peide D. ( November 2023 , Communications Physics)

   Relativistic Weyl fermion quasiparticles in Weyl semimetal bring the electron’s chirality degree of freedom into the electrical transport and give rise to exotic phenomena. A topological phase transition from a topological trivial phase to a topological non-trivial phase offers a route to control electronic devices through its topological properties. Here, we report the Weyl semimetal phase in hydrothermally grown two-dimensional Tellurium (2D Te) induced by high hydrostatic pressure (up to 2.47 GPa). The unique chiral crystal structure gives rise to chiral fermions with different topological chiral charges ($${{C}}=-{{1}},+{{1}},{{and}}-{{2}}$$$C=-1,+1,and-2$). The highly tunable chemical potential in 2D Te provides comprehensive information for understanding the pressure-dependent electron band structure. The pressure-induced insulator-to-metal transition, two-carrier transport, and the non-trivial π Berry phase shift in quantum oscillations are observed in the 2D Te Weyl semimetal phase. Our work demonstrates the pressure-induced bandgap closing in the inversion asymmetric narrow bandgap semiconductor 2D Te.

    

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2. Perspectives on field-free spin–orbit torque devices for memory and computing applications

   https://doi.org/10.1063/5.0135185  

   Lopez-Dominguez, Victor ; Shao, Yixin ; Khalili Amiri, Pedram ( January 2023 , Journal of Applied Physics)

   The emergence of embedded magnetic random-access memory (MRAM) and its integration in mainstream semiconductor manufacturing technology have created an unprecedented opportunity for engineering computing systems with improved performance, energy efficiency, lower cost, and unconventional computing capabilities. While the initial interest in the existing generation of MRAM—which is based on the spin-transfer torque (STT) effect in ferromagnetic tunnel junctions—was driven by its nonvolatile data retention and lower cost of integration compared to embedded Flash (eFlash), the focus of MRAM research and development efforts is increasingly shifting toward alternative write mechanisms (beyond STT) and new materials (beyond ferromagnets) in recent years. This has been driven by the need for better speed vs density and speed vs endurance trade-offs to make MRAM applicable to a wider range of memory markets, as well as to utilize the potential of MRAM in various unconventional computing architectures that utilize the physics of nanoscale magnets. In this Perspective, we offer an overview of spin–orbit torque (SOT) as one of these beyond-STT write mechanisms for the MRAM devices. We discuss, specifically, the progress in developing SOT-MRAM devices with perpendicular magnetization. Starting from basic symmetry considerations, we discuss the requirement for an in-plane bias magnetic field which has hindered progress in developing practical SOT-MRAM devices. We then discuss several approaches based on structural, magnetic, and chiral symmetry-breaking that have been explored to overcome this limitation and realize bias-field-free SOT-MRAM devices with perpendicular magnetization. We also review the corresponding material- and device-level challenges in each case. We then present a perspective of the potential of these devices for computing and security applications beyond their use in the conventional memory hierarchy. 

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3. Strain‐Engineered Anisotropic Optical and Electrical Properties in 2D Chiral‐Chain Tellurium

   https://doi.org/10.1002/adma.202002342  

   Wang, Yixiu ; Yao, Shukai ; Liao, Peilin ; Jin, Shengyu ; Wang, Qingxiao ; Kim, Moon J. ; Cheng, Gary J. ; Wu, Wenzhuo ( June 2020 , Advanced Materials)

   Atomically thin materials, leveraging their low‐dimensional geometries and superior mechanical properties, are amenable to exquisite strain manipulation with a broad tunability inaccessible to bulk or thin‐film materials. Such capability offers unexplored possibilities for probing intriguing physics and materials science in the 2D limit as well as enabling unprecedented device applications. Here, the strain‐engineered anisotropic optical and electrical properties in solution‐grown, sub‐millimeter‐size 2D Te are systematically investigated through designing and introducing a controlled buckled geometry in its intriguing chiral‐chain lattice. The observed Raman spectra reveal anisotropic lattice vibrations under the corresponding straining conditions. The feasibility of using buckled 2D Te for ultrastretchable strain sensors with a high gauge factor (≈380) is further explored. 2D Te is an emerging material boasting attractive characteristics for electronics, sensors, quantum devices, and optoelectronics. The results suggest the potential of 2D Te as a promising candidate for designing and implementing flexible and stretchable devices with strain‐engineered functionalities.

    

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4. Recent Advances in Low‐Dimensional Nanomaterials for Photodetectors

   https://doi.org/10.1002/smtd.202300246  

   Kim, Jaehyun ; Lee, Junho ; Lee, Jong‐Min ; Facchetti, Antonio ; Marks, Tobin J. ; Park, Sung Kyu ( May 2023 , Small Methods)

   New emerging low‐dimensional such as 0D, 1D, and 2D nanomaterials have attracted tremendous research interests in various fields of state‐of‐the‐art electronics, optoelectronics, and photonic applications due to their unique structural features and associated electronic, mechanical, and optical properties as well as high‐throughput fabrication for large‐area and low‐cost production and integration. Particularly, photodetectors which transform light to electrical signals are one of the key components in modern optical communication and developed imaging technologies for whole application spectrum in the daily lives, including X‐rays and ultraviolet biomedical imaging, visible light camera, and infrared night vision and spectroscopy. Today, diverse photodetector technologies are growing in terms of functionality and performance beyond the conventional silicon semiconductor, and low‐dimensional nanomaterials have been demonstrated as promising potential platforms. In this review, the current states of progress on the development of these nanomaterials and their applications in the field of photodetectors are summarized. From the elemental combination for material design and lattice structure to the essential investigations of hybrid device architectures, various devices and recent developments including wearable photodetectors and neuromorphic applications are fully introduced. Finally, the future perspectives and challenges of the low‐dimensional nanomaterials based photodetectors are also discussed.

    

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5. Two-dimensional Dirac spin-gapless semiconductors with tunable perpendicular magnetic anisotropy and a robust quantum anomalous Hall effect

   https://doi.org/10.1039/d0mh00396d  

   Sun, Qilong ; Ma, Yandong ; Kioussis, Nicholas ( August 2020 , Materials Horizons)

   null (Ed.)

   A major recent breakthrough in materials science is the emergence of intrinsic magnetism in two-dimensional (2D) crystals, which opens the door to more cutting-edge fields in the 2D family and could eventually lead to novel data-storage and information devices with further miniaturization. Herein we propose an experimentally feasible 2D material, Fe 2 I 2 , which is an intrinsic room-temperature ferromagnet exhibiting perpendicular magnetic anisotropy (PMA). Using first-principles calculations, we demonstrate that single-layer (SL) Fe 2 I 2 is a spin-gapless semiconductor with a spin-polarized Dirac cone and linear energy dispersion in one spin channel, exhibiting promising dissipation-less transport properties with a Fermi velocity up to 6.39 × 10 5 m s −1 . Our results reveal that both strain and ferroelectric polarization switching could induce an out-of- to in-plane spin reorientation in the 2D Fe 2 I 2 layer, revealing its advantage in assembling spintronic devices. In addition, spin–orbit coupling (SOC) triggers a topologically nontrivial band gap of 301 meV with a nonzero Chern number (| C | = 2), giving rise to a robust quantum anomalous Hall (QAH) state. The 2D crystal also exhibits high carrier mobilites of 0.452 × 10 3 and 0.201 × 10 3 cm 2 V −1 s −1 for the electrons and holes, respectively. The combination of these unique properties renders the 2D Fe 2 I 2 ferromagnet a promising platform for high efficiency multi-functional spintronic applications. 

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